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We report the optical absorption characteristics and the photocurrent spectra for large-area molecular junctions containing different molecular structures and thicknesses. Through experimental assessment of the optical absorption of…

Chemical Physics · Physics 2021-04-12 V Mukundan , J A Fereiro , R L McCreery , A J Bergren

Recent optical studies of monolayer transition metal dechalcogenides have demonstrated that their excitonic absorption feature splits into two widely separated peaks at finite carrier densities. The additional peak is usually attributed to…

Mesoscale and Nanoscale Physics · Physics 2017-01-25 Dmitry K. Efimkin , Allan H. MacDonald

We present an ab initio description of optical and shallow-core x-ray absorption spectroscopies in a unified formalism based on the pseudopotential plane-wave method at the level of the Bethe-Salpeter equation (BSE) within Green's functions…

Materials Science · Physics 2023-06-07 M. Laura Urquiza , Matteo Gatti , Francesco Sottile

Techniques for coherent multidimensional optical spectroscopy have been developed and utilised to understand many different processes, including energy transfer in photosynthesis and many-body effects in semiconductor nanostructures.…

Optics · Physics 2017-01-24 Jonathan Tollerud , Jeffrey Davis

The optical properties of two-dimensional transition metal dichalcogenide monolayers such as MoS$_2$ or WSe$_2$ are dominated by excitons, Coulomb bound electron-hole pairs. Screening effects due the presence of hexagonal-BN surrounding…

Materials Science · Physics 2018-12-26 Iann C. Gerber , Xavier Marie

A first-principles study on the quasiparticles energy and optical absorption spectrum of fluorographene is presented by employing the GW + Bethe-Salpeter Equation (BSE) method with many-electron effects included. The calculated band gap is…

Mesoscale and Nanoscale Physics · Physics 2019-06-05 Yufeng Liang , Li Yang

Optical responses in an excitonic insulating (EI) system with strong electron correlation are studied. We adopt the two-orbital Hubbard model with a finite energy difference between the two orbitals where the spin state degree of freedom…

Strongly Correlated Electrons · Physics 2020-03-25 Hengyue Li , Junya Otsuki , Makoto Naka , Sumio Ishihara

In the Mott-Hubbard insulators YTiO3 and SmTiO3 we study optical excitations from the lower to the upper Hubbard band, d^1d^1 -> d^0d^2. The multi-peak structure observed in the optical conductivity reflects the multiplet structure of the…

Strongly Correlated Electrons · Physics 2024-11-05 A. Gössling , R. Schmitz , H. Roth , M. W. Haverkort , T. Lorenz , J. A. Mydosh , E. Müller-Hartmann , M. Grüninger

Based on \emph{ab initio} theoretical calculations of the optical spectra of vertical heterostructures of MoSe$_2$ (or MoS$_2$) and WSe$_2$ sheets, we reveal two spin-orbit-split Rydberg series of excitonic states below the \textsl{A}…

Mesoscale and Nanoscale Physics · Physics 2018-04-18 Roland Gillen , Janina Maultzsch

Reflectance and magneto-reflectance experiments together with theoretical modelling based on the $\mathbf{k\cdot p}$ approach have been employed to study the evolution of direct bandgap excitons in MoS$_2$ layers with a thickness ranging…

Mesoscale and Nanoscale Physics · Physics 2019-03-01 A. O. Slobodeniuk , Ł. Bala , M. Koperski , M. R. Molas , P. Kossacki , K. Nogajewski , M. Bartos , K. Watanabe , T. Taniguchi , C. Faugeras , M. Potemski

It is important to study absorption spectrum in film dosimetry because the spectral absorbance of the film relates to the film's total absorption dose. We investigated the absorption spectra of Gafchromic EBT2 film with various rotational…

We investigate the excitonic transitions in single- and few-layer MoSe2 phototransistors by photocurrent spectroscopy. The measured spectral profiles show a well-defined peak at the optically active (bright) A0 exciton resonance. More…

We present a systematic study of the variables affecting the electronic and optical properties of two-dimensional(2D) crystals within \textit{ab initio} GW and GW plus Bethe Salpeter Equation (GW-BSE) calculations. As a prototypical 2D…

Materials Science · Physics 2016-07-20 Diana Y. Qiu , Felipe H. da Jornada , Steven G. Louie

Mott transition has been realized in atomically thin monolayer (ML) of two dimensional semiconductors (WS$_2$) via optically excited carriers above a critical carrier density through many body interactions. The above nonlinear optical…

Materials Science · Physics 2021-10-12 Shreyasi Das , Rup K. Chowdhury , Debjani Karmakar , Soumen Das , Samit K. Ray

We have studied the absorption of electromagnetic radiation of an anisotropic quantum dot taking into account the spin-flip processes that is associated with the interaction of the electrons with optical phonons. It is shown that these…

Mesoscale and Nanoscale Physics · Physics 2009-11-13 V. A. Margulis , A. V. Shorokhov

In this article, we use a many-body approach to study the absorption spectra of electron-doped two-dimensional semiconductors. Optical absorption is modeled by a many-body scattering Hamiltonian which describes an exciton immersed in a…

Mesoscale and Nanoscale Physics · Physics 2019-03-27 Yao-Wen Chang , David R. Reichman

Optoelectronic excitations in monolayer MoS2 manifest from a hierarchy of electrically tunable, Coulombic free-carrier and excitonic many-body phenomena. Investigating the fundamental interactions underpinning these phenomena - critical to…

We have measured the electric field modulated absorption of a sample of single-walled nanotubes (SWNT) suspended in a solid polyvinyl alcohol matrix. The electroabsorption (EA) spectrum roughly follows the first derivative of the absorption…

Materials Science · Physics 2007-05-23 J. W. Kennedy , Z. V. Vardeny , S. Collins , R. H. Baughman , H. Zhao , S. Mazumdar

Floquet engineering of electronic states by light is a central topic in modern experiments. However, the impact of many-body interactions on the single-electron properties remains unclear in this non-equilibrium situation. We propose that…

Other Condensed Matter · Physics 2025-10-07 Teng Xiao , Tsan Huang , Changhua Bao , Zhiyuan Sun

The conservation of the photon total angular momentum in the incident direction in an axially symmetric scattering process is a very well known fact. Nonetheless, the re-distribution of this conserved magnitude into its spin and orbital…