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We present an ab initio computational approach for the calculation of resonant Raman intensities, including both excitonic and non-adiabatic effects. Our diagrammatic approach, which we apply to two prototype, semiconducting layered…

Mesoscale and Nanoscale Physics · Physics 2020-10-01 Sven Reichardt , Ludger Wirtz

Effects of coupling between an molecular exciton and a surface plasmon (exciton-plasmon coupling) on the luminescence properties of the molecule and the surface plasmons are investigated using nonequilibrium Green's function method.…

Materials Science · Physics 2013-11-12 Kuniyuki Miwa , Mamoru Sakaue , Hideaki Kasai

Applying the novel exact-exchange (EXX) Kohn-Sham method within time-dependent density-functional theory, we obtained the optical absorption spectrum of bulk silicon in good agreement with experiments including excitonic features. Analysis…

Materials Science · Physics 2016-01-01 Yong-Hoon Kim , Andreas Goerling

We investigate high resolution laser absorption spectroscopy of a single InGaAs/GaAs self-assembled quantum dot embedded in a field-effect structure. We show experimentally that the interband optical absorption to the lower Zeeman branch of…

Mesoscale and Nanoscale Physics · Physics 2016-08-16 A. Högele , M. Kroner , S. Seidl , K. Karrai , M. Atatüre , J. Dreiser , A. Imamoğlu , R. J. Warburton , A. Badolato , B. D. Gerardot , P. M. Petroff

We show how to correctly extract from the ellipsometric data the surface susceptibility and the surface conductivity that describe the optical properties of monolayer $\rm MoS_2$. Theoretically, these parameters stem from modelling a…

We investigated the $ab$-plane absorption spectra of $R$MnO$%_{3}$ ($R$ = La, Pr, Nd, Gd, and Tb) thin films. As the $R$-ion size decreases, we observed a drastic suppression of the 2 eV peak, \textit{i.e.} the inter-site optical transition…

Strongly Correlated Electrons · Physics 2007-05-23 M. W. Kim , S. J. Moon , J. H. Jung , Jaejun Yu , Sachin Parashar , P. Murugavel , T. W. Noh

We review vibrational and electronic properties of single and a few layer MoS$_2$ relevant to understand their resonant and non-resonant Raman scattering results. In particular, the optical modes and low frequency shear and layer breathing…

Mesoscale and Nanoscale Physics · Physics 2015-02-13 Achintya Bera , A. K. Sood

We systematically measure the dielectric function of atomically thin MoS2 films with different layer numbers and demonstrate that excitonic effects play a dominant role in the dielectric function when the films are less than 5-7 layers…

Optical responses of atomically thin 2D materials are greatly influenced by electron-hole interactions. It is by far established that exciton signatures can be well-identified in the optical absorption spectrum of quasi-2D materials.…

Mesoscale and Nanoscale Physics · Physics 2023-10-30 Yu-Tzu Chang , Yang-Hao Chan

We show that spin-orbit coupling (SOC) in InSe enables the optical transition across the principal band gap to couple with in-plane polarized light. This transition, enabled by $p_{x,y}\leftrightarrow p_z$ hybridization due to intra-atomic…

Mesoscale and Nanoscale Physics · Physics 2017-11-21 S. J. Magorrian , V. Zólyomi , V. I. Fal'ko

We investigate phase-dependent electronic and excitonic phenomena in monolayer Y2TeO2 MOenes in the 1T and 2H polymorphs using first-principles theory and an effective many-body framework. Phonon spectra and elastic stability criteria…

It is well-known that exciton effects are determinant to understand the optical absorption spectrum of low-dimensional materials. However, the role of excitons in nonlinear optical responses has been much less investigated at an…

Mesoscale and Nanoscale Physics · Physics 2024-06-21 J. J. Esteve-Paredes , M. A. García-Blázquez , A. J. Uría-Álvarez , M. Camarasa-Gómez , J. J. Palacios

The photoluminescence spectrum of a single-layer boron nitride remains elusive, marked by enigmatic satellites that hint at a significant but unidentified exciton-phonon coupling.Here, by employing a first principles approach based on the…

Materials Science · Physics 2024-06-03 Giovanni Marini , Matteo Calandra , Pierluigi Cudazzo

We demonstrate here that the dipole-allowed optical absorption spectrum of a parabolic quantum dot subjected to an external magnetic field reflects the inter-electron interaction effects when the spin-orbit interaction is also taken into…

Mesoscale and Nanoscale Physics · Physics 2009-11-11 Tapash Chakraborty , Pekka Pietiläinen

We measure the optical absorption spectra and optical conductivities of excitons and trions in monolayers of metal dichalcogenide MoS$_{2}$ and compare the results with theoretical models. Our results show that the Wannier-Mott model for…

Mesoscale and Nanoscale Physics · Physics 2014-06-04 Changjian Zhang , Haining Wang , Weimin Chan , Christina Manolatou , Farhan Rana

The real part of optical conductivity $\text{Re}\sigma(\omega)$ of the Mott insulators has a large amount of information on how spin and charge degrees of freedom interact with each other. By using the time-dependent density-matrix…

Strongly Correlated Electrons · Physics 2021-11-23 Kazuya Shinjo , Yoshiki Tamaki , Shigetoshi Sota , Takami Tohyama

The recent advances in angle resolved photoemission techniques allowed the unambiguous experimental confirmation of spin charge decoupling in quasi one dimensional (1D) Mott insulators. This opportunity stimulates a quantitative analysis of…

Strongly Correlated Electrons · Physics 2015-05-14 Valeria Lante , Alberto Parola

We combine linear and non-linear optical spectroscopy at 4K with ab initio calculations to study the electronic bandstructure of MoSe2 monolayers. In 1-photon photoluminescence excitation (PLE) and reflectivity we measure a separation…

Materials Science · Physics 2015-11-05 G. Wang , I. C. Gerber , L. Bouet , D. Lagarde , A. Balocchi , M. Vidal , E. Palleau , T. Amand , X. Marie , B. Urbaszek

Monolayers of ReS2 were grown by a chemical vapor deposition technique on SiO2/Si substrates and investigated at room temperature by using micro-Raman, micro-photoluminescence (PL) and absorbance spectroscopies. The Raman scattering…

Materials Science · Physics 2024-04-23 Solomon Ojo , Juwon Onasanya , Morad Benamara , Bothina Hamad , M. O. Manasreh

A set of theoretical results [1-10] is reviewed, which concern calculations of energy spectra, density of energy levels, spin polarization, transport and optical properties (infrared absorption, luminescence) of semiconductor quantum dots…

Mesoscale and Nanoscale Physics · Physics 2007-05-23 Augusto Gonzalez