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Coupled pairs of spin-1/2 nuclei support one singlet state and three triplet states. In many circumstances the nuclear singlet order, defined as the difference between the singlet population and the mean of the triplet populations, is a…

Quantum Physics · Physics 2022-10-19 Mohamed Sabba , Nino Wili , Christian Bengs , Lynda J. Brown , Malcolm H. Levitt

Dynamic nuclear polarization transfers spin polarization from electrons to nuclei. We have achieved this by a new method, simultaneously exciting transitions of electronic and nuclear spins. The efficiency of this technique improves with…

Quantum Physics · Physics 2008-09-11 G. W. Morley , K. Porfyrakis , A. Ardavan , J. van Tol

Spin squeezing, a form of many-body entanglement, is a crucial resource in quantum metrology and information processing. While experimentally viable protocols for generating stable spin squeezing have been proposed in quantum optics setups,…

Quantum Physics · Physics 2025-09-16 Jayakrishnan M. P. Nair , Benedetta Flebus

The hyperpolarization of nuclear spins can enable powerful imaging and sensing techniques provided the hyperpolarization is sufficiently long-lived. Recent experiments on nanodiamond $^{13}$C nuclear spins demonstrate that relaxation times…

Mesoscale and Nanoscale Physics · Physics 2024-02-20 Gargee Sharma , Torsten Gaebel , Ewa Rej , David J. Reilly , Sophia E. Economou , Edwin Barnes

Most materials freeze when cooled to sufficiently low temperature. We find that magnetic dipoles randomly distributed in a solid matrix condense into a spin liquid with spectral properties on cooling that are the diametric opposite of those…

Condensed Matter · Physics 2009-11-10 S. Ghosh , R. Parthasarathy , T. F. Rosenbaum , G. Aeppli

We investigate the performance of dynamical decoupling methods at suppressing electron spin decoherence from a low-temperature nuclear spin reservoir in a quantum dot. The controlled dynamics is studied through exact numerical simulation,…

Mesoscale and Nanoscale Physics · Physics 2009-11-13 Wenxian Zhang , V. V. Dobrovitski , Lea F. Santos , Lorenza Viola , B. N. Harmon

We show how to divide a coupled multi-spin system into a small subset of ``active'' spins that evolve under chemical shift or scalar coupling operators, and a larger subset of ``spectator'' spins which are returned to their initial states,…

Quantum Physics · Physics 2009-10-31 N Linden , H Barjat , RJ Carbajo , R Freeman

States with long coherence are a crucial requirement for qubits and quantum memories. Nuclear spins in epitaxial quantum dots are a great candidate, offering excellent isolation from external environments and on-demand coupling to optical…

Mesoscale and Nanoscale Physics · Physics 2025-02-18 Harry E. Dyte , Santanu Manna , Saimon F. Covre da Silva , Armando Rastelli , Evgeny A. Chekhovich

The dominant source of decoherence for an electron spin in a quantum dot is the hyperfine interaction with the surrounding bath of nuclear spins. The decoherence process may be slowed down by subjecting the electron spin to suitable…

Mesoscale and Nanoscale Physics · Physics 2017-08-23 Wenxian Zhang , V. V. Dobrovitski , Lea F. Santos , Lorenza Viola , B. N. Harmon

The phase coherence relaxation times as long as $T_2\sim830-1030\pm20$ ns were measured for the [2Fe-2S] cluster in the intrinsic protein environment. This relaxation corresponds to a relatively long lasting coherence of the low-spin…

Biomolecules · Quantitative Biology 2015-04-02 Amgalanbaatar Baldansuren

Spins in solids and molecules are promising for applications of quantum sensing technology. The sensitivity of the quantum sensing depends on how precisely spin observables can be determined in the measurement, and is intrinsically limited…

Quantum Physics · Physics 2025-11-21 Yifan Song , Nabiha Hasan , Susumu Takahashi

Metastable states arise in a range of quantum systems and can be observed in various dynamical scenarios, including decay, bubble nucleation, and long-lived oscillations. The phenomenology of metastable states has been examined in quantum…

Multiple quantum (MQ) NMR with a dipolar ordered initial state opens new possibilities for the exploration of many-spin entanglement. In this paper, we investigate many-spin entanglement in a gas of spin-carrying molecules (atoms) in…

Quantum Physics · Physics 2021-02-03 Ilia D. Lazarev , Edward. B. Feldman

In pulsed dynamic nuclear polarization (DNP), enhancement of the polarization of bulk nuclei requires the repeated application of a microwave pulse sequence. So far, analysis of a one-time transfer of electron spin polarization to a…

Chemical Physics · Physics 2025-07-24 Shebha Anandhi Jegadeesan , Yujie Zhao , Graham M. Smith , Ilya Kuprov , Guinevere Mathies

We measure the transverse relaxation of the spin state of an ensemble of ground-state rubidium atoms trapped in solid parahydrogen at cryogenic temperatures. We find the spin dephasing time of the ensemble (T$_2^*$) is limited by…

We propose a strategy to generate a many-body entangled state in a collection of randomly placed, dipolarly coupled electronic spins in the solid state. By using coherent control to restrict the evolution into a suitable collective…

Quantum Physics · Physics 2009-09-12 Paola Cappellaro , Mikhail D. Lukin

Nuclear spins and paramagnetic centers in a solid randomly group to form clusters featuring nearly-degenerate, hybrid states whose dynamics are central to processes involving nuclear spin-lattice relaxation and diffusion. Their…

Previous heat-capacity measurements of our group had shown the possible existence of an anomalous quantum phase containing the zero-point vacancies (ZPVs) in 2D $^{3}$He. The system is monolayer $^{3}$He adsorbed on graphite preplated with…

Strongly Correlated Electrons · Physics 2009-11-13 S. Takayoshi , K. Obata , D. Sato , T. Matsui , Hiroshi Fukuyama

We develop an efficient package for the simulation of nuclear magnetic resonance spin echo experiments to study the effects of strong electronic spin correlations on the dynamics of the nuclear spin ensemble. A mean-field model is used to…

Strongly Correlated Electrons · Physics 2026-02-09 Charles Snider , Stephen Carr , D. E. Feldman , Chandrasekhar Ramanathan , V. F. Mitrović

We analyze two approaches to quantum state transfer in solid-state spin systems. First, we consider unpolarized spin-chains and extend previous analysis to various experimentally relevant imperfections, including quenched disorder,…

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