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We use first-principles calculations to study the effect of magnetic disorder and electron correlations on the structural and thermodynamic properties of CrN. We illustrate the usability of a special quasirandom structure supercell…

Strongly Correlated Electrons · Physics 2010-12-14 B. Alling , T. Marten , I. A. Abrikosov

An ab initio study of magnetic exchange interactions in antiferromagnetic and strongly correlated 3d transition metal monoxides is presented. Their electronic structure is calculated using the local self-interaction correction approach,…

An efficient method to compute magnetic exchange interactions in systems with strong correlations is introduced. It is based on a magnetic force theorem which evaluates linear response due to rotations of magnetic moments and uses a novel…

Strongly Correlated Electrons · Physics 2007-05-23 Xiangang Wan , Quan Yin , Sergej Y. Savrasov

We present a novel approach to calculate the effective exchange interaction parameters based on the realistic electronic structure of correlated magnetic crystals in local approach with the frequency dependent self energy. The analog of…

Strongly Correlated Electrons · Physics 2009-10-31 M. I. Katsnelson , A. I. Lichtenstein

We introduce a theoretical framework for computaions of anisotropic multipolar exchange interactions found in many spin--orbit coupled magnetic systems and propose a method to extract these coupling constants using a density functional…

Strongly Correlated Electrons · Physics 2014-08-01 Shu-Ting Pi , Ravindra Nanguneri , Sergey Savrasov

Estimates of the exchange interaction parameter (J) between electronic magnetic momenta residing in the d-shells of several divalent first row transition metal ions, and those residing on the [TCNE]$^-$. anion-radicals (TCNE =…

Chemical Physics · Physics 2011-12-07 A. L. Tchougréeff

We report a study of the anisotropic exchange interactions in bulk CrO_2 calculated from first principles within density functional theory. We determine the exchange coupling energies, using both the experimental lattice parameters and…

Materials Science · Physics 2015-03-13 H. Sims , S. J. Oset , W. H. Butler , James M. MacLaren , Martijn Marsman

We unify the method of exchange perturbation theory for multicenter systems. For the case of exchange degeneracy in the total spin of the system we give a secular equation that is more compact and convenient for calculations than those…

Strongly Correlated Electrons · Physics 2015-03-25 Elena V. Orlenko , Tatiana Latychevskaia

Because of large spatial separation of the Mn atoms in Heusler alloys the Mn 3d states belonging to different atoms do not overlap considerably. Therefore an indirect exchange interaction between Mn atoms should play a crucial role in the…

Materials Science · Physics 2009-11-13 E. Sasioglu , L. M. Sandratskii , P. Bruno

We consider mechanism of exchange coupling based on interaction between electrons in nonmagnetic layer. Depending on ratio of inverse time of diffusion of electrons between ferromagnetic layers and ferromagnetic splitting of conducting…

Mesoscale and Nanoscale Physics · Physics 2009-09-29 Zyuzin A. Yu

It is demonstrated that the magnetic interactions can be drastically different for nano-sized systems compared to those of bulk or surfaces. Using a real-space formalism we have developed a method to calculate non-collinear magnetization…

We propose a method for the evaluation of magnetic exchange couplings based on noncollinear spin-density functional calculations. The method employs the second derivative of the total Kohn-Sham energy of a single reference state, in…

Materials Science · Physics 2009-11-13 Juan E. Peralta , Veronica Barone

We analyze the effective electron-electron interaction in a two dimensional polarized paramagnetic system. The spin degree of freedom, s, is manifestly present in the expressions of spin dependent local field factors that describe the short…

Strongly Correlated Electrons · Physics 2007-05-23 Juana Moreno , D. C. Marinescu

Incommensurate magnetism in CrB$_2$ is studied in terms of a spin model based on density functional theory calculations. Heisenberg exchange interactions derived from the paramagnetic phase using the disordered local moment theory show…

Strongly Correlated Electrons · Physics 2022-10-12 András Deák , Jerome Jackson , Bendegúz Nyári , László Szunyogh

A new method of computing multipolar exchange interaction in spin-orbit coupled systems is developed using multipolar tensor expansion of the density matrix in LDA+U electronic structure calculation. Within mean-field approximation,…

Strongly Correlated Electrons · Physics 2014-03-06 Shu-Ting Pi , Ravindra Nanguneri , Sergey Savrasov

We present a computational method to determine the exchange constants in isotropic spin models. The method uses the Hamiltonian and overlap matrices computed from density functional schemes that are based on nonorthogonal basis sets. We…

Mesoscale and Nanoscale Physics · Physics 2019-06-19 László Oroszlány , Jaime Ferrer , András Deák , László Udvardi , László Szunyogh

We study the dependence of magnetic interactions and Curie temperature in Ni(1+x)MnSb system on the Ni concentration within the framework of the density-functional theory. The calculation of the exchange parameters is based on the…

Materials Science · Physics 2009-11-11 E. Sasioglu , L. M. Sandratskii , P. Bruno

We present calculations of magnetic exchange interactions and critical temperature T_c in Mn:GaAs, Cr:GaAs and Cr:GaN. The local spin density approximation is combined with a linear-response technique to map the magnetic energy onto a…

Materials Science · Physics 2009-11-10 J. L. Xu , M. van Schilfgaarde , G. D. Samolyuk

Despite serious effort, the nature of the magnetic interactions and the role of electron-correlation effects in magnetic two-dimensional (2D) van der Waals materials remain elusive. Using CrI$_3$ as a model system, we show that the…

Materials Science · Physics 2021-02-04 Liqin Ke , Mikhail I. Katsnelson

We present a controlled method for computing the exchange coupling in correlated one-dimensional electron systems based on the relation between the exchange constant and the pair-correlation function of spinless electrons. This relation is…

Strongly Correlated Electrons · Physics 2007-05-23 Michael M. Fogler , Eugene Pivovarov
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