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It is shown that adsorption energy at semiconductor surfaces critically depends on the charge transfer to or from the adsorbed species. For the processes without the charge transfer, such as molecular adsorption of closed shell systems, the…

Materials Science · Physics 2013-08-23 Paweł Kempisty , Paweł Strak , Konrad Sakowski , Stanisław Krukowski

We studied the electron transfer from excitons in adsorbed indoline dye layers across the organic-inorganic interface. The hybrids consist of indoline derivatives on the one hand and different inorganic substrates (TiO$_2$, ZnO,…

Radiative and nonradiative resonant couplings between defects are ubiquitous phenomena in photonic devices used in classical and quantum information technology applications. In this work we present a first principles approach to enable…

Optics · Physics 2025-09-10 Swarnabha Chattaraj , Giulia Galli

The possibility for controlling the probe-field optical gain and absorption switching and photon conversion by a surface-plasmon-polariton near field is explored for a quantum dot above the surface of a metal. In contrast to the linear…

Mesoscale and Nanoscale Physics · Physics 2023-07-19 Danhong Huang , Michelle Easter , Godfrey Gumbs , A. A. Maradudin , Shawn-Yu Lin , Dave Cardimona , Xiang Zhang

We have investigated the conditions necessary to achieve stronger Cherenkov-like instability of plasma waves leading to emission in the terahertz (THz) regime for semiconductor quantum wells (QWs). The surface response function is…

Mesoscale and Nanoscale Physics · Physics 2015-05-18 Antonios Balassis , Godfrey Gumbs

Surface plasmons on metals can concentrate light into sub-nanometric volumes and on these near atomic length scales the electronic response at the metal interface is smeared out over a Thomas-Fermi screening length. This nonlocality is a…

Mesoscale and Nanoscale Physics · Physics 2015-06-16 Yu Luo , A. I. Fernandez-Dominguez , Aeneas Wiener , S. A. Maier , J. B. Pendry

It has recently been demonstrated that difference frequency mixing (DFM) can generate surface plasmons in graphene [1]. Here, we present detailed calculations comparing the contributions to this effect from substrate and from graphene…

When a semiconductor absorbs light, the resulting electron-hole superposition amounts to a uncontrolled quantum ripple that eventually degenerates into diffusion. If the conformation of these excitonic superpositions could be engineered,…

Mesoscale and Nanoscale Physics · Physics 2017-05-31 Xiaoning Zang , Simone Montangero , Lincoln D. Carr , Mark T. Lusk

Understanding the differences between photon-induced and plasmon-induced hot electrons is essential for the construction of devices for plasmonic energy conversion. The mechanism of the plasmonic enhancement in photochemistry,…

Closely-spaced quantum emitters coherently sharing excitation can release their energy faster than suggested by a simple sum over their individual emission rates - a phenomenon known as superradiance. Here, we show that the assumption of…

Quantum Physics · Physics 2019-12-13 Severin Bang , Stefan Yoshi Buhmann , Robert Bennett

Atomically thin two-dimensional crystals have revolutionized materials science. In particular, monolayer transition metal dichalcogenides promise novel optoelectronic applications, due to their direct energy gaps in the optical range. Their…

Generalizing recent work, the Raman scattering intensity from a semi-infinite superconducting superlattice is calculated taking into account the surface contribution to the density response functions. Our work makes use of the formalism of…

Condensed Matter · Physics 2009-10-28 W. C. Wu , A. Griffin

Studies of different experimental groups that explore the properties of a two-dimensional electron gas in silicon semiconductor systems ((100) Si metal-oxide-semiconductor field-effect transistors (MOSFETs) and (100) SiGe/Si/SiGe quantum…

Strongly Correlated Electrons · Physics 2019-10-15 V. T. Dolgopolov

The interaction between light and matter is fundamental to developments in quantum optics and information. Over recent years enormous progress has been made in controlling the interface between light and single emitters including ions,…

Evidence is presented for energy exchange between surface plasmon polaritons (SPPs) excited in waveguide-coupled Ag/Si3N4/Au structures and CdSe/ZnS quantum dot (QD) emitters. The QD dispersion is coated on the surface of Ag/Si3N4/Au…

Applied Physics · Physics 2020-07-09 Kunal Tiwari , Suresh C Sharma , Hussein Akafzade , Nader Hozhabri

We describe a strategy for conversion of optical power into DC electrical power using resonant absorption in plasmonic nanostructures. A thermodynamic analysis of the underlying mechanism motivates our description of the phenomenon, which…

Mesoscale and Nanoscale Physics · Physics 2012-02-03 Matthew T. Sheldon , Harry A. Atwater

Quenching of fluorescence (FL) at the vicinity of conductive surfaces, and in particular, near a 2-D graphene layer has become an important biochemical sensing tool. The quenching is attributed to fast non-radiative energy transfer between…

Mesoscale and Nanoscale Physics · Physics 2023-07-19 X. Miao , D. J. Gosztola , X. Ma , D. Czaplewski , L. Stan , H. Grebel

The effect of screening of the coulomb interaction between two layers of two-dimensional electrons, such as in graphene, by a highly doped semiconducting substrate is investigated. We employ the random-phase approximation to calculate the…

Mesoscale and Nanoscale Physics · Physics 2014-10-15 Godfrey Gumbs , Andrii Iurov , Danhong Huang

We investigate three-dimensional rolled-up metamaterials containing optically active quantum wells and metal gratings supporting surface plasmon polarition resonances. Finite-difference time-domain simulations show that by matching the…

Materials Science · Physics 2011-09-09 Andreas Rottler , Stephan Schwaiger , Anuen Koitmäe , Detlef Heitmann , Stefan Mendach

The electron transfer in different solvents is investigated for systems consisting of donor, bridge and acceptor. It is assumed that vibrational relaxation is much faster than the electron transfer. Electron transfer rates and final…

Soft Condensed Matter · Physics 2016-09-28 D. Kilin , U. Kleinekathoefer , M. Schreiber
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