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One way for solar cell efficiencies to overcome the Shockley-Queisser limit is downconversion of high-energy photons using singlet fission (SF) in polyacenes like tetracene (Tc). SF enables generation of multiple excitons from the…

Applied Physics · Physics 2018-01-31 S. W. Tabernig , B. Daiber , T. Wang , B. Ehrler

A simple refluxing wet-chemical approach is employed for fabricating In2S3/Pt-TiO2 heterogeneous catalysts for hydrogen generation under visible light irradiation. When the mass ratio between Pt-TiO2 and cubic-phased In2S3 (denoted as…

The concept of the effective one-electron potentials (OEP) has been useful for many decades in efficient description of electronic structure of chemical systems, especially extended molecular aggregates such as interacting molecules in…

Chemical Physics · Physics 2020-02-04 Bartosz Błasiak , Joanna D. Bednarska , Marta Chołuj , Wojciech Bartkowiak

Transparent photovoltaic (TPV) devices have the great potential to apply as smart windows in the construction and agriculture field. The efficiencies of TPVs are growing up quickly in recent years and the champion efficiency even exceeds…

Applied Physics · Physics 2021-05-07 Ruiqian Meng , Qianqing Jiang , Dianyi Liu

A novel diad composed of a diaminoterephthalate scaffold, covalently linked to a Fullerene derivative, is explored as a nanosized charge separation unit powered by solar energy. Its opto-electronic properties are studied and the charge…

Halide perovskites have emerged as promising candidates for high-performance solar cells. This study investigates the temperature-dependent optoelectronic properties of mixed-cation mixed-halide perovskite solar cells using…

Electron-hole pairs in organic photovoltaics dissociate efficiently despite their Coulomb-binding energy exceeding thermal energy at room temperature. The electronic states involved in charge separation couple to structured vibrational…

Mesoscale and Nanoscale Physics · Physics 2023-08-15 Alejandro D. Somoza , Nicola Lorenzoni , James Lim , Susana F. Huelga , Martin B. Plenio

Electron paramagnetic resonance (EPR) study of air-physisorbed defective carbon nano-onions evidences in favor of microwave assisted formation of weakly-bound paramagnetic complexes comprising negatively-charged O2- ions and edge carbon…

Mesoscale and Nanoscale Physics · Physics 2016-06-10 D. W. Boukhvalov , V. Yu. Osipov , A. I. Shames , K. Takai , T. Hayashi , T. Enoki

The feasibility of an experimental determination of the parton distributions of virtual photons at high energy $ep$ colliders is studied in the context of the DESY-HERA collider. Recently proposed parton densities of virtual photons are…

High Energy Physics - Phenomenology · Physics 2011-01-25 M. Gluck , E. Reya , M. Stratmann

Excitonic semiconductors such as transition metal dichalcogenides (TMDCs) are attractive for next-generation photovoltaics (PVs) with low cost, light weight, and low material consumption. In WS2 and other TMDCs, the simultaneous large…

Optics · Physics 2024-10-22 Adam D. Alfieri , Tobia Ruth , Cheryl Lim , Jason Lynch , Deep Jariwala

Power sector decarbonization plays a vital role in the upcoming energy transition towards a more sustainable future. Decentralized energy resources, such as Electric Vehicles (EV) and solar photovoltaic systems (PV), are continuously…

Solar water splitting provides a promising path for sustainable hydrogen production and solar energy storage. One of the greatest challenges towards large-scale utilization of this technology is reducing the hydrogen production cost. The…

Different computational methods are employed to evaluate elastic (rotationally summed) integral and differential cross sections for low energy (below about 10 eV) positron scattering off gas-phase C$_2$H$_2$ molecules. The computations are…

Chemical Physics · Physics 2009-11-13 J. Franz , F. A. Gianturco , K. L. Baluja , J. Tennyson , R. Carey , R. Montuoro , R. R. Lucchese , T. Stoecklin

We present a neutron spectroscopy based method to study quantitatively the partial miscibility and phase behaviour of an organic photovoltaic active layer made of conjugated polymer:small molecule blends, presently illustrated with the…

Materials Science · Physics 2021-09-20 Mohamed Zbiri , Peter A. Finn , Christian B. Nielsen , Anne A. Y. Guilbert

Distributed energy resources (DERs) installed at electric distribution networks create different opportunities and challenges for the distribution system operator (DSO). By increasing the penetration level of DERs, the impacts of these…

Systems and Control · Electrical Eng. & Systems 2022-06-29 Abbas Rabiee , Andrew Keane , Alireza Soroudi

The high recombination rate of photogenerated carriers is the bottleneck of photocatalysis, severely limiting the photocatalytic efficiency. Here, we develop a dipole-scheme (D-scheme for short) photocatalytic model and materials…

Materials Science · Physics 2022-07-13 Xu Gao , Yanqing Shen , Jiajia Liu , Lingling Lv , Min Zhou , Zhongxiang Zhou , Yuan Ping Feng , Lei Shen

We compare three representative high performance PV materials: halide perovskite MAPbI3, CdTe, and GaAs, in terms of photoluminescence (PL) efficiency, PL lineshape, carrier diffusion, and surface recombination, over multiple orders of…

Experimental/theoretical evidence for sustained vibration-assisted electronic (vibronic) coherence in the Photosystem II Reaction Center (PSII RC) indicates that photosynthetic solar-energy conversion might be optimized through the…

We present a density functional theory (DFT) based supercell approach for modeling small polarons with proper account for the long-range elastic response of the material. Our analysis of the supercell dependence of the polaron properties…

Materials Science · Physics 2018-04-18 Sebastian Kokott , Sergey V Levchenko , Patrick Rinke , Matthias Scheffler

While silicon solar cells dominate global photovoltaic energy production, their continued improvement is hindered by the single junction limit. One potential solution is to use molecular singlet exciton fission to generate two electrons…