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We show that the lack of inversion symmetry in monolayer MoS2 allows strong optical second harmonic generation. Second harmonic of an 810-nm pulse is generated in a mechanically exfoliated monolayer, with a nonlinear susceptibility on the…

Materials Science · Physics 2015-06-15 Nardeep Kumar , Sina Najmaei , Qiannan Cui , Frank Ceballos , Pulickel M. Ajayan , Jun Lou , Hui Zhao

Anomalously high generation efficiency of coherent higher field-harmonics in collisions between {\em oppositely charged particles} in the field of femtosecond lasers is predicted. This is based on rigorous numerical solutions of a quantum…

Condensed Matter · Physics 2009-10-31 H. Haberland , M. Bonitz , D. Kremp

In present paper, we describe a theoretical model of generation of harmonic emissions of type III solar radio bursts. The goal of our study is to fully take into account the most efficient physical processes participating in generation of…

Plasma Physics · Physics 2021-02-24 Anna Tkachenko , Vladimir Krasnoselskikh , Andrii Voshchepynets

We study cascaded harmonic generation of hybrid surface plasmons in integrated planar waveguides composed of a graphene layer and a doped-semiconductor slab. We derive a comprehensive model of cascaded third harmonic generation through…

Optics · Physics 2015-10-14 Daria A. Smirnova , Alexander S. Solntsev

Integrated nonlinear photonic technologies, even with state-of-the-art fabrication with only a few nanometer geometry variations, face significant challenges in achieving wafer-scale yield of functional devices. A core limitation lies in…

We study the phase matching of resonant high-harmonic generation (HHG) and high-order frequency mixing (HFM) in plasma. We solve numerically the propagation equations coupled with the time-dependent Schr\"odinger equation for the nonlinear…

Optics · Physics 2024-04-30 Vasily V. Strelkov , Margarita A. Khokhlova

Plasmon resonances are known to amplify the electromagnetic fields near metallic nanostructures. Therefore, they are considered to provide a promising scheme to generate extreme-ultraviolet harmonics, using low power drivings. During…

Optical frequency conversion processes in nonlinear materials are limited in wavelength by the accessible phase matching and the required high pump powers. In this letter, we report a novel broadband phase matching (PM) technique in high…

Optics · Physics 2013-03-18 Guoping Lin , Josef U. Fürst , Dmitry V. Strekalov , Nan Yu

The effect of slow light on second harmonic generation in a periodically poled $\chi^{(2)}$ nonlinear medium is investigated theoretically. A linear $\pi$ phase shifted grating is used to slow the group velocity of the fundamental frequency…

Optics · Physics 2022-02-02 Thomas E. Maybour , Devin H. Smith , Peter Horak

Hyperbolic plasmonic metamaterials provide numerous opportunities for designing unusual linear and nonlinear optical properties. We show that the modal overlap of fundamental and second-harmonic light in an anisotropic plasmonic…

Second-order nonlinear effects, such as second-harmonic generation, can be strongly enhanced in nanofabricated photonic materials when both fundamental and harmonic frequencies are spatially and temporally confined. Practically designing…

Harmonic generation is a general characteristic of driven nonlinear systems, and serves as an efficient tool for investigating the fundamental principles that govern the ultrafast nonlinear dynamics. In atomic gases, high-harmonic radiation…

Second-order nonlinear optical response allows to detect different properties of the system associated with the inversion symmetry breaking. Here, we use a second harmonic generation effect to investigate the alignment of a…

Mesoscale and Nanoscale Physics · Physics 2020-07-03 E. A. Stepanov , S. V. Semin , C. R. Woods , M. Vandelli , A. V. Kimel , K. S. Novoselov , M. I. Katsnelson

Efficient nonlinear wave mixing is of paramount importance for a wide range of applications. However, weak optical nonlinearities pose significant challenges for accessing nonlinear light-matter interaction in compact systems. Here, we…

High-harmonic generation in solids allows probing and controlling electron dynamics in crystals on few femtosecond timescales, paving the way to lightwave electronics. In the spatial domain, recent advances in the real-space interpretation…

In this Letter, it is experimentally and theoretically shown that weak odd harmonics generated during the propagation of an infrared ultrashort ultra-intense pulse unexpectedly modify the nonlinear properties of the medium and lead to a…

Optics · Physics 2015-06-18 P. Béjot , G. Karras , F. Billard , E. Hertz , B. Lavorel , E. Cormier , O. Faucher

We experimentally and theoretically investigate the second order nonlinear optical response of metallo-dielectric multilayer structures composed of Ag and Ta2O5 layers, deposited by magnetron sputtering. Second harmonic generation…

We aim to clarify the role that absorption plays in nonlinear optical processes in a variety of metallic nanostructures and show how it relates to emission and conversion efficiency. We define a figure of merit that establishes the…

We report on the fabrication of what we believe is the first example of a two dimensional nonlinear periodic crystal\cite{berger}, where the refractive index is constant but in which the 2nd order nonlinear susceptibility is spatially…

Spatial and spectral properties of the pulsed second harmonic generation in a periodically-poled KTP waveguide exploiting simultaneously the first, second, and third harmonics of periodic nonlinear modulation are analyzed. Experimental…

Quantum Physics · Physics 2013-01-30 Radek Machulka , Jiří Svozilík , Jan Soubusta , Jan Peřina , Ondřej Haderka