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Using femtosecond pump-probe spectroscopy with pulse shaping techniques, one can generate and detect coherent phonons in chirality-specific semiconducting single-walled carbon nanotubes. The signals are resonantly enhanced when the pump…

Mesoscale and Nanoscale Physics · Physics 2015-05-13 G. D. Sanders , C. J. Stanton , J. -H. Kim , K. -J. Yee , Y. -S. Lim , E. H. Haroz , L. G. Booshehri , J. Kono , R. Saito

Coherent phonons in single wall carbon nanotubes (SWNTs) are observed as oscillations of the differential absorption coefficient as a function of time by means of pump-probe spectroscopy. For the radial breathing mode (RBM) of a SWNT, the…

Mesoscale and Nanoscale Physics · Physics 2015-06-22 A. R. T. Nugraha , E. H. Hasdeo , G. D. Sanders , C. J. Stanton , R. Saito

We have investigated the polarization dependence of the generation and detection of radial breathing mode (RBM) coherent phonons (CP) in highly-aligned single-walled carbon nanotubes. Using polarization-dependent pump-probe…

Mesoscale and Nanoscale Physics · Physics 2015-05-19 L. G. Booshehri , C. L. Pint , G. D. Sanders , L. Ren , C. Sun , E. H. Haroz , J. -H. Kim , K. -J. Yee , Y. -S. Lim , R. H. Hauge , C. J. Stanton , J. Kono

We have observed large-amplitude coherent phonon oscillations of radial breathing modes (RBMs) in single-walled carbon nanotubes excited through the lowest-energy (E11) interband transitions. In contrast to the previously-studied coherent…

Mesoscale and Nanoscale Physics · Physics 2010-08-11 Y. -S. Lim , J. -G. Ahn , J. -H. Kim , K. -J. Yee , T. Joo , S. -H. Baik , E. H. Haroz , L. G. Booshehri , J. Kono

We review recent studies of coherent phonons (CPs) corresponding to the radial breathing mode (RBM) and G-mode in single-wall carbon nanotubes (SWCNTs) and graphene. Because of the bandgap-diameter relationship, RBM-CPs cause bandgap…

Mesoscale and Nanoscale Physics · Physics 2013-03-28 J. -H. Kim , A. R. T. Nugraha , L. G. Booshehri , E. H. Hároz , K. Sato , G. D. Sanders , K. -J. Yee , Y. -S. Lim , C. J. Stanton , R. Saito , J. Kono

We have used a femtosecond pump-probe impulsive Raman technique to explore the ultrafast dynamics of micelle suspended single walled carbon nanotubes (SWNTs) in various pH environments. The structures of coherent phonon spectra of the…

Mesoscale and Nanoscale Physics · Physics 2010-11-17 Kotaro Makino , Atsushi Hirano , Kentaro Shiraki , Yutaka Maeda , Muneaki Hase

The pulse-train technique within ultrafast pump-probe spectroscopy is theoretically investigated to enhance a specific coherent phonon mode while suppressing the other phonon modes generated in single wall carbon nanotubes (SWNTs). In…

Mesoscale and Nanoscale Physics · Physics 2016-12-20 Ahmad R. T. Nugraha , Eddwi H. Hasdeo , Riichiro Saito

With the empirical bond polarizability model, the nonresonant Raman spectra of the chiral and achiral single-wall carbon nanotubes (SWCNTs) under uniaxial and torsional strains have been systematically studied by \textit{ab initio} method.…

Mesoscale and Nanoscale Physics · Physics 2007-07-31 Gang Wu , Jian Zhou , Jinming Dong

We have studied the coherent dynamics of G-band phonons in single-walled carbon nanotubes through impulsive stimulated Stokes and anti-Stokes Raman scattering. The probe energy dependence of phonon amplitude as well as preferential…

Mesoscale and Nanoscale Physics · Physics 2012-11-13 J. -H. Kim , K. -J. Yee , Y. -S. Lim , L. G. Booshehri , E. H. Haroz , J. Kono

The Raman spectra of two G-bands and a radial breathing mode (RBM) of unfilled and filled single-wall semiconducting and metallic carbon nanotubes have been investigated theoretically, in the presence of electron-phonon and phonon-phonon…

Other Condensed Matter · Physics 2009-11-13 S. Gayen , S. N. Behera , S. M. Bose

We discuss how excitons can affect the generation of coherent radial breathing modes in ultrafast spectroscopy of single wall carbon nanotubes. Photoexcited excitons can be localized spatially and give rise to a spatially distributed…

In this work we investigate the role of exciton resonances in coherent anti-Stokes Raman scattering (er-CARS) in single walled carbon nanotubes (SWCNTs). We drive the nanotube system in simultaneous phonon and excitonic resonances, where we…

Mesoscale and Nanoscale Physics · Physics 2023-11-06 Georgy Gordeev , Lucas Lafeta , Benjamin Scott Flavel , Ado Jorio , Leandro M. Malard

We report on the impulsive generation of coherent optical phonons in CdTe0.68Se0.32 nanocrystallites embedded in a glass matrix. Pump probe experiments using femtosecond laser pulses were performed by tuning the laser central energy to…

Mesoscale and Nanoscale Physics · Physics 2009-11-10 A. V. Bragas , C. Aku-Leh , S. Costantino , Alka Ingale , J. Zhao , R. Merlin

We use the energy analysis as a perturbative method to study the effect of electron-radial breathing mode (RBM) phonon interaction on the electrical conductivity of long metallic zigzag carbon nanotubes (CNTs). The band structure of zigzag…

Mesoscale and Nanoscale Physics · Physics 2018-05-29 Reyhaneh Taj , Afshin Namiranian

We have investigated excitons in highly-aligned single-walled carbon nanotubes (SWCNTs) through optical spectroscopy at low temperature (1.5 K) and high magnetic fields ($\textbf{\textit{B}}$) up to 55 T. SWCNT/polyacrylic acid films were…

Mesoscale and Nanoscale Physics · Physics 2009-11-13 J. Shaver , S. A. Crooker , J. A. Fagan , E. K. Hobbie , N. Ubrig , O. Portugall , V. Perebeinos , Ph. Avouris , J. Kono

We have studied photoluminescence (PL) and resonant Raman scatterings of single-walled carbon nanotubes (SWNTs) consisting of carbon-13 (SW13CNTs) synthesized from a small amount of isotopically modified ethanol. There was almost no change…

Materials Science · Physics 2009-11-11 Yuhei Miyauchi , Shigeo Maruyama

We report on an optical method to directly measure electron-phonon coupling in carbon nanotubes by correlating the first and second harmonic of the resonant Raman excitation profile. The method is applicable to 1D and 0D systems and is not…

Materials Science · Physics 2007-05-23 Y. Yin , A. Vamivakas , A. Walsh , S. Cronin , M. S. Unlu , B. B Goldberg , A. K. Swan

We employed femtosecond pump probe technique to investigate the dynamics of coherent optical phonons in iron garnet. A phenomenological symmetry-based consideration reveals that oscillations of the terahertz T2g mode are excited. Selective…

Excitation of four coherent phonon modes of different symmetries has been realized in copper metaborate CuB$_2$O$_4$ via impulsive stimulated Raman scattering (ISRS). Phonons were detected by monitoring changes in the linear optical…

We study the optical properties of a single, semiconducting single-walled carbon nanotube (CNT) that is partially suspended across a trench and partially supported by a SiO2-substrate. By tuning the laser excitation energy across the E33…

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