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We report on high resolution Fourier-transform spectroscopy of fluorescence to the a^3\Sigma_u^+ state excited by two-photon or two-step excitation from the X^1\Sigma_g^+ state to the 2^3\Pi_g state in the molecule K_2. These spectroscopic…

Atomic Physics · Physics 2009-11-13 A. Pashov , P. Popov , H. Knöckel , E. Tiemann

The sodium monoxide radical (NaO) is observed in night glow in the Earth's mesosphere and likely has astronomical importance. This study concerns the optical transitions within the ground X $^2\Pi$ state and to the very low-lying…

Chemical Physics · Physics 2022-10-26 G. B. Mitev , S. Taylor , Jonathan Tennyson , S. N. Yurchenko , A. A. Buchachenko , A. V. Stolyarov

We consider the impurity problem in an orbital Feshbach resonance (OFR), with a single excited clock state $|e\uparrow\rangle$ atom immersed in a Fermi sea of electronic ground state $|g\downarrow\rangle$. We calculate the polaron effective…

Quantum Gases · Physics 2018-04-23 Junjun Xu , Ran Qi

We show that ultracold polar diatomic or linear molecules, oriented in an external electric field and mutually coupled by dipole-dipole interactions, can be used to realize the exact Heisenberg XYZ, XXZ and XY models without invoking any…

Quantum Physics · Physics 2022-11-09 Wenjing Yue , Qi Wei , Sabre Kais , Bretislav Friedrich , Dudley Herschbach

We examine dark quantum superposition states of weakly bound Rb2 Feshbach molecules and tightly bound triplet Rb2 molecules in the rovibrational ground state, created by subjecting a pure sample of Feshbach molecules in an optical lattice…

We report on the creation of heterospecies bosonic molecules, associated from an ultracold Bose-Bose mixture of 41K and 87Rb, by using a resonantly modulated magnetic field close to two Feshbach resonances. We measure the binding energy of…

Other Condensed Matter · Physics 2009-01-29 C. Weber , G. Barontini , J. Catani , G. Thalhammer , M. Inguscio , F. Minardi

We predict the existence of stable bound states between pairs of ultracold diatomic molecules with the aid of a static electric field and 1D harmonic confinement. We focus on collisions of NaK-NaK identical fermions, for which we find that…

Atomic Physics · Physics 2024-09-25 Reuben R. W. Wang , John L. Bohn

Quantum communication testbeds provide a useful resource for experimentally investigating a variety of communication protocols. Here we demonstrate a superconducting circuit testbed with bidirectional multi-photon state transfer capability…

Nuclear spin exchange occurs in ultracold collisions of fermionic alkaline-earth-like atoms due to a difference between s- and p-wave phase shifts. We study the use of an optical Feshbach resonance, excited on the ${}^1S_0 \to {}^3P_1$…

Quantum Physics · Physics 2013-05-29 Iris Reichenbach , Paul S. Julienne , Ivan H. Deutsch

We consider two-color heteronuclear photoassociation of atoms into dipolar molecules in the J=1 electro-vibrational ground state, where a free-ground laser couples atoms directly to the ground state and a free-bound laser couples the atoms…

Quantum Gases · Physics 2009-11-19 Matt Mackie , Catherine DeBrosse

We report on a high-resolution spectroscopic survey of ${}^{6}\textrm{Li}{}^{40}\textrm{K}$ molecules near the $2\textrm{S}+4\textrm{P}$ dissociation threshold and produce a fully empirical representation for the $\textrm{B}^{1}\Pi$…

Atomic Physics · Physics 2022-02-23 Sofia Botsi , Anbang Yang , Mark M. Lam , Sambit B. Pal , Sunil Kumar , Markus Debatin , Kai Dieckmann

Stimulated Raman adiabatic passage (STIRAP) allows to efficiently transferring the populations between two discrete quantum states and has been used to prepare molecules in their rovibrational ground state. In realistic molecules, a…

Atomic Physics · Physics 2019-07-24 Lan Liu , De-Chao Zhang , Huan Yang , Ya-Xiong Liu , Jue Nan , Jun Rui , Bo Zhao , Jian-Wei Pan

Ultracold paramagnetic and polar diatomic molecules are among the promising systems for quantum simulation of lattice-spin models. Unfortunately, their experimental observation is still challenging. Based on our recent \textit{ab-initio}…

Ultracold polar and magnetic ${}^{23}$Na${}^6$Li molecules in the rovibrational ground state of the lowest triplet $a^3\Sigma^+$ electronic state have been recently produced. Here, we calculate the electronic and rovibrational structure of…

Atomic Physics · Physics 2021-02-16 Marcin Gronowski , Adam M. Koza , Michał Tomza

We present a detailed study of interspecies Feshbach resonances of the bosonic $^{23}\mathrm{Na}+$$^{39}\mathrm{K}$ mixture for magnetic fields up to $750 \, \mathrm{G}$ in various collision channels. A total of fourteen Feshbach resonances…

A STIRAP-like scheme is proposed to exploit a three-photon resonance taking place in alkaline-earth-metal ions. This scheme is designed for state transfer between the two fine structure components of the metastable D-state which are two…

Many experimental platforms for quantum science depend on state control via laser fields. Frequently, however, the control fidelity is limited by optical phase noise. This is exacerbated in stabilized laser systems where high-frequency…

We demonstrate that it is possible to efficiently control ultracold chemical reactions of alkali-metal atoms colliding with open-shell alkali-metal dimers in their metastable triplet states by choosing the internal hyperfine and…

Chemical Physics · Physics 2021-09-08 Rebekah Hermsmeier , Jacek Klos , Svetlana Kotochigova , Timur V. Tscherbul

Cold and ultracold polar molecules with nonzero electronic angular momentum are of great interest for studies in quantum chemistry and control, investigations of novel quantum systems, and precision measurement. However, in mixed electric…

Atomic Physics · Physics 2015-05-30 Benjamin K. Stuhl , Mark Yeo , Brian C. Sawyer , Matt Hummon , Jun Ye

Modeling the underlying pairing mechanism of charge carriers in strongly correlated electrons, starting from a microscopic theory, is among the central challenges of condensed-matter physics. Hereby, the key task is to understand what…

Strongly Correlated Electrons · Physics 2024-03-21 Lukas Homeier , Pit Bermes , Fabian Grusdt
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