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We present the results of a muon-spin relaxation (muSR) investigation into magnetic ordering in several families of layered quasi-two-dimensional molecular antiferromagnets based on transition metal ions such as S=1/2 Cu2+ bridged with…

We present the results of muon-spin relaxation measurements of spin excitations in the one-dimensional quantum Heisenberg antiferromagnet Cu(pyz)(NO$_{3}$)$_{2}$. Using density-functional theory we propose muon sites and assess the degree…

Strongly Correlated Electrons · Physics 2015-05-20 F. Xiao , J. S. Möller , T. Lancaster , R. C. Williams , F. L. Pratt , S. J. Blundell , D. Ceresoli , A. M. Barton , J. L. Manson

Low-dimensional magnetic materials with spin-$\frac{1}{2}$ moments can host a range of exotic magnetic phenomena due to the intrinsic importance of quantum fluctuations to their behavior. Here, we report the structure, magnetic structure…

We present the results of muon-spin spectroscopy ($\mu^{+}$SR) measurements on the molecular spin ladder system (Hpip)$_{2}$CuBr$_{4(1-x)}$Cl$_{4x}$, [Hpip=(C$_{5}$H$_{12}$N)]. Using transverse field $\mu^{+}$SR we are able to identify…

Muon spin relaxation measurements are reported on samples of dimethylammonium metal formates containing magnetic divalent nickel, cobalt, manganese, and copper ions. These hybrid organic-inorganic perovskites exhibit weak ferromagnetism and…

Strongly Correlated Electrons · Physics 2015-05-19 P. J. Baker , T. Lancaster , I. Franke , W. Hayes , S. J. Blundell , F. L. Pratt , P. Jain , Z. -M. Wang , M. Kurmoo

We present the first evidence of magnetic order in the quasi-one-dimensional spin 1/2 molecular chain compound, copper pyrazine dinitrate Cu(C4H4N2)(NO3)2}. Zero field muon-spin relaxation measurements made at dilution refrigerator…

Strongly Correlated Electrons · Physics 2007-11-14 T. Lancaster , S. J. Blundell , M. L. Brooks , P. J. Baker , F. L. Pratt , J. L. Manson , C. P. Landee , C. Baines

Magnetic properties of a one-dimensional frustrated quantum spin system Rb2Cu2Mo3O12 is investigated by the muon spin relaxation (muSR) technique. Although this system shows an incommensurate spin correlation in neutron scattering, it has…

Strongly Correlated Electrons · Physics 2018-04-04 Seiko Ohira-Kawamura , Keisuke Tomiyasu , Akihiro Koda , Dita P. Sari , Retno Asih , Sungwon Yoon , Isao Watanabe , Kenji Nakajima

We investigate the structural and magnetic properties of two molecule-based magnets synthesized from the same starting components. Their different structural motifs promote contrasting exchange pathways and consequently lead to markedly…

We have performed magnetic susceptibility, heat capacity, muon spin relaxation, and neutron scattering measurements on three members of the family Ba3MRu2O9, where M = In, Y and Lu. These systems consist of mixed-valence Ru dimers on a…

Strongly Correlated Electrons · Physics 2017-05-31 D. Ziat , A. A. Aczel , R. Sinclair , Q. Chen , H. D. Zhou , T. J. Williams , M. B. Stone , A. Verrier , J. A. Quilliam

Metal organic magnets have enormous potential to host a variety of electronic and magnetic phases that originate from a strong interplay between the spin, orbital and lattice degrees of freedom. We control this interplay in the quantum…

Strongly Correlated Electrons · Physics 2017-08-14 M. Skoulatos , M. Månsson , C. Fiolka , K. W. Krämer , J. Schefer , J. S. White , Ch. Rüegg

We have performed elastic and inelastic neutron experiments on single crystal samples of the coordination polymer compound CuF2(H2O)2(pyz) (pyz=pyrazine) to study the magnetic structure and excitations. The elastic neutron diffraction…

Within a first principles framework, we study the electronic structure of the recently synthesized polymeric coordination compound Cu(II)-2,5-bis(pyrazol-1-yl)-1,4-dihydroxybenzene (CuCCP), which has been suggested to be a good realization…

The magnetic dynamic structure factor of the one-dimensional S = 1/2 chain system BaCu2(Si0.5Ge0.5)2O7 is studied in a wide range of energy transfers and temperatures. Contrary to previous erroneous reports [T. Masuda et al., Phys. Rev.…

Strongly Correlated Electrons · Physics 2015-06-25 A. Zheludev , T. Masuda , G. Dhalenne , A. Revcolevschi , C. Frost , T. Perring

In this work we study the interplay between the crystal structure and magnetism of the pyroarsenate \alpha-Cu_2As_2O_7 by means of magnetization, heat capacity, electron spin resonance and nuclear magnetic resonance measurements as well as…

Zero-field muon spin relaxation (ZF-$\mu$SR) measurements were undertaken on under- and overdoped samples of superconducting YBa$_2$Cu$_3$O$_{6+x}$ to determine the origin of the weak static magnetism recently reported in this system. The…

A large variety of materials can be approximately described by means of spin-1/2 Heisenberg ladders. Here, the Density Matrix Renormalization Group (DMRG) algorithm together with a previously established numerical self-consistent mean-field…

Strongly Correlated Electrons · Physics 2026-02-18 Mateo Cárdenes Wuttig , Andrew J. Millis

The interplay of crystal electric field, temperature, and spin-orbit coupling can yield a Kramers ion and thus an effective S = 1/2 ground state for Co2+ ions (3d7), which is often the case for low dimensional materials. This is because a…

Materials Science · Physics 2025-04-01 Lun Jin , Robert J. Cava

We investigated the crystal and magnetic structures of the spin-1/2 frustrated antiferromagnet Cu3Mo2O9 in which the spin system consists of antiferromagnetic chains and dimers. The space group at room temperature has been reported to be…

Using the exact solution in terms of the generalized classical transfer matrix method we presented a detailed analysis of the magnetic properties and ground state structure of the simplified model of the single-chain magnet, trimetallic…

Statistical Mechanics · Physics 2014-03-12 Stefano Bellucci , Vadim Ohanyan , Onofre Rojas

Muon spin rotation measurements have been performed on a powder sample of a-RuCl3, a layered material which previously has been proposed to be a quantum magnet on a honeycomb lattice close to a quantum spin liquid ground state. Our data…

Strongly Correlated Electrons · Physics 2016-07-20 F. Lang , P. J. Baker , A. A. Haghighirad , Y. Li , D. Prabhakaran , R. Valenti , S. J. Blundell
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