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Graphene is expected to complement todays Si-based information technology. In particular, magnetic molecules in contact with graphene constitute a tantalizing approach towards organic spin electronics because of the reduced conductivity…

Materials Science · Physics 2013-04-18 C. F. Hermanns , K. Tarafder , M. Bernien , A. Krüger , Y. -M. Chang , P. M. Oppeneer , W. Kuch

We show that strong coupling between graphene and the substrate is mitigated when 0.8 monolayer of Na is adsorbed and consolidated on top graphene-on-Ni(111). Specifically, the {\pi} state is partially restored near the K-point and the…

Electronic decoupling of graphene from metallic and semiconducting substrates via intercalation of different species is one of the widely used approaches in studies of graphene. In the present work the modification of the electronic and…

Materials Science · Physics 2021-12-24 Yong Zhou , Roman Ovcharenko , Beate Paulus , Yuriy Dedkov , Elena Voloshina

We perform systematic first-principles calculations of the proximity exchange coupling, induced by cobalt (Co) and nickel (Ni) in graphene, via a few (up to three) layers of hexagonal boron nitride (hBN). We find that the induced spin…

Mesoscale and Nanoscale Physics · Physics 2016-10-26 Klaus Zollner , Martin Gmitra , Tobias Frank , Jaroslav Fabian

The combination of the surface science techniques (STM, XPS, ARPES) and density-functional theory calculations was used to study the decoupling of graphene from Ni(111) by oxygen intercalation. The formation of the antiferromagnetic (AFM)…

Materials Science · Physics 2017-05-26 Yuriy Dedkov , Wolfgang Klesse , Andreas Becker , Florian Späth , Christian Papp , Elena Voloshina

In this paper, we establish the existence of both compressive stress and charge transfer process in hydrothermally synthesized cobalt ferrite-graphene oxide (CoFe2O4/GO) nanocomposites. Transmission electron microscopy (TEM) results reveal…

Mesoscale and Nanoscale Physics · Physics 2017-05-24 Amodini Mishra , Vikash Kumar Singh , Tanuja Mohanty

Superconductivity in graphite intercalated compounds has been studied for more than 40 years and it is still not fully understood, despite the recent progress and the discovery of relatively high Tc superconductivity in CaC6 and YbC6.…

Superconductivity · Physics 2009-04-14 T. Valla , J. Camacho , Z-H. Pan , A. V. Fedorov , A. C. Walters , C. A. Howard , M. Ellerby

We study the magnetic coupling between different ferromagnetic metals (FMs) across a graphene (G) layer, and the role of graphene as a thin covalent spacer. Starting with G grown on a FM substrate (Ni or Co), we deposit on top at room…

Materials Science · Physics 2017-03-08 I. Grimaldi , M. Papagno , L. Ferrari , P. M. Sheverdyaeva , S. K. Mahatha , D. Pacilé , C. Carbone

Measuring the transport of electrons through a graphene sheet necessarily involves contacting it with metal electrodes. We study the adsorption of graphene on metal substrates using first-principles calculations at the level of density…

Materials Science · Physics 2015-05-13 P. A. Khomyakov , G. Giovannetti , P. C. Rusu , G. Brocks , J. van den Brink , P. J. Kelly

This study theoretically investigated the magnetic properties and electronic structure of a graphene-based nano-spin-valve-like structure. Magnetic nickel layers on both sides of the graphene were considered. A spin-polarized…

Mesoscale and Nanoscale Physics · Physics 2019-05-30 Yusuf Wicaksono , Shingo Teranishi , Kazutaka Nishiguchi , Koichi Kusakabe

The induction of unconventional superconductivity by twisting two layers of graphene a small angle was groundbreaking1, and since then has attracted widespread attention to novel phenomena caused by lattice or angle mismatch between…

Mesoscale and Nanoscale Physics · Physics 2020-09-21 Yuqi Wang , Soroush Arabi , Klaus Kern , Markus Ternes

We report an advanced organic spin-interface architecture with magnetic remanence at room temperature, constituted by metal phthalocyanine molecules magnetically coupled with Co layer(s), mediated by graphene. Fe- and Cu-phthalocyanines…

The electronic structure and magnetic properties of the graphene/Fe/Ni(111) system were investigated via combination of the density functional theory calculations and electron-spectroscopy methods. This system was prepared via intercalation…

Materials Science · Physics 2017-09-13 M. Weser , E. N. Voloshina , K. Horn , Yu. S. Dedkov

Magnetic properties of nanometer thick Co films intercalated at the graphene/Ir(111) interface are investigated using spin-polarized low-energy electron microscopy (SPLEEM) and Auger electron spectroscopy. We show that the graphene top…

Materials Science · Physics 2014-04-04 N. Rougemaille , A. T. N'Diaye , J. Coraux , C. Vo-Van , O. Fruchart , A. K. Schmid

Using low-energy electron microscopy, we study Co intercalation under graphene grown on Ir(111). Depending on the rotational domain of graphene on which it is deposited, Co is found intercalated at different locations. While intercalated Co…

Materials Science · Physics 2014-03-14 S. Vlaic , A. Kimouche , J. Coraux , B. Santos , A. Locatelli , N. Rougemaille

First-principles calculations of the effect of carbon coverage on the atomic, electronic and magnetic structure of nickel and iron substrates demonstrate insignificant changes in the interatomic distances and magnetic moments on the atoms…

Materials Science · Physics 2014-12-24 D. W. Boukhvalov , Yu. N. Gornostyrev , M. A. Uimin , A. V. Korolev , A. Ye Yermakov

The in-plane lattice constants of close-packed planes of fcc and hcp Ni and Co match that of graphite almost perfectly so that they share a common two dimensional reciprocal space. Their electronic structures are such that they overlap in…

Here we report the photoemission studies of intercalation process of Fe underneath graphene layer on Ni(111). The process of intercalation was monitored via XPS of corresponding core levels and UPS of the graphene-derived $\pi$ states in…

Materials Science · Physics 2009-11-13 Yu. S. Dedkov , M. Fonin , U. Rüdiger , C. Laubschat

CO$_2$ capture using carbon-based materials, particularly graphene and graphene-like materials, is a promising strategy to deal with CO$_2$ emissions. However, significant gaps remain in our understanding of the molecular-level interaction…

The exceptional electronic properties of monoatomic thin graphene sheets triggered numerous original transport concepts, pushing quantum physics into the realm of device technology for electronics, optoelectronics and thermoelectrics. At…

Materials Science · Physics 2016-04-21 M. Vondracek , M. Kucera , L. Fekete , J. Kopecek , J. Lancok , D. Kalita , J. Coraux , V. Bouchiat , J. Honolka
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