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Models for the evolution of dust are used to show that the observed trend of the abundance of polycyclic aromatic hydrocarbons (PAHs) with metallicity is the result of the delayed injection of carbon dust that formed in low mass asymptotic…
We investigate the evolution of polycyclic aromatic hydrocarbon (PAH) abundance in a galaxy, which is a crucial step to understand the evolution of bright emission features in the mid-infrared range. We calculate the evolution of dust grain…
Hydrogenated amorphous carbon materials, a-C(:H), are heterogeneous structures consisting of carbon atoms in different hybridisation states and bonding configurations and are thought to constitute a significant and observationally important…
A majority of early-type galaxies contain interstellar dust, yet the origin of this dust, and why the dust sometimes exhibits unusual polycyclic aromatic hydrocarbon (PAH) ratios, remains a mystery. If the dust is internally produced, it…
We investigate to what degree local physical and chemical conditions are related to the evolutionary status of various objects in star-forming media. rho Oph A displays the entire sequence of low-mass star formation in a small volume of…
Molecular hydrogen (H2) is the main constituent of the gas in the planet-forming disks that surround many PMS stars. H2 can be incorporated in the atmosphere of the giant planets. HD has been detected in a few disks and can be considered…
Hydrogen depleted environments are considered an essential requirement for the formation of fullerenes. The recent detection of C60 and C70 fullerenes in what was interpreted as the hydrogen-poor inner region of a post-final helium shell…
Recent observations indicate potentially carbon-rich exoplanet atmospheres. Spectral fitting methods for brown dwarfs and exoplanets have invoked the C/O ratio as additional parameter but carbon-rich cloud formation modeling is a challenge…
Observational evidence seems to indicate that the depletion of interstellar carbon into dust shows rather wide variations and that carbon undergoes rather rapid recycling in the interstellar medium (ISM). Small hydrocarbon grains are…
Aims. Interstellar dust grains, because of their catalytic properties, are crucial to the formation of H2, the most abundant molecule in the Universe. The formation of molecular hydrogen strongly depends on the ability of H atoms to stick…
On galactic scales, the surface density of star formation appears to be well correlated with the surface density of molecular gas. This has lead many authors to suggest that there exists a causal relationship between the chemical state of…
The formation of polycyclic aromatic hydrocarbons (PAHs) and their methyl derivatives occurs mainly in the dust shells of asymptotic giant branch (AGB) stars. The bands at 3.3 and 3.4 $\mu$m, observed in infrared emission spectra of several…
Cosmic dust is mainly formed in the atmospheres of evolved stars. In carbon rich stars, amorphous carbon along with silicon carbide are the main constituents of dust grains yet the mechanisms involved in the formation of these grains are…
The radical hydrocarbon molecule C$_2$H is widely detected in various stages of star and planet formation, and has emerged as a useful tracer of high-C/O gas within the photochemically active surface layers of mature (Class II)…
Context. The compositional properties of hydrogenated amorphous carbons are known to evolve in response to the local conditions. Aims. To present a model for low-temperature, amorphous hydrocarbon solids, based on the microphysical…
Context. The presence of dust in the interstellar medium has profound consequences on the chemical composition of regions where stars are forming. Recent observations show that many species formed onto dust are populating the gas phase,…
The temperature of newly forming dust is controlled by the radiation field. As dust forms around stars, stellar transients, quasars or supernovae, the grains must grow through a regime where they are stochastically heated by individual…
We describe a phenomenological model for molecular hydrogen formation suited for applications in galaxy formation simulations, which includes on-equilibrium formation of molecular hydrogen on dust and approximate treatment of both its…
Fragmentation is an important decay mechanism for polycyclic aromatic hydrocarbons (PAHs) under harsh interstellar conditions and represents a possible formation pathway for small molecules such as H2, C2H2, C2H4. Our aim is to investigate…
The study of cyclic hydrocarbons is of utmost relevance in current astrochemical research, as they are considered to be among the most significant reservoirs of carbon in the interstellar medium. However, while unsaturated cyclic…