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Theoretical rotational quenching cross sections and rate coefficients of ortho- and para-H$_2$O due to collisions with He atoms are presented. The complete angular momentum close-coupling approach as well as the coupled-states approximation…

Solar and Stellar Astrophysics · Physics 2015-06-15 Benhui Yang , M. Nagao , W. Satomi , M. Kimura , P. C. Stancil

Rate coefficients for rotational transitions in H_2 induced by H_2 impact are presented. Extensive quantum mechanical coupled-channel calculations based on a recently published (H_2)_2 potential energy surface were performed. The potential…

Rate coefficients for state-to-state rotational transitions in CO induced by both para- and ortho-H$_2$ collisions are presented. The results were obtained using the close-coupling method and the coupled-states approximation, with the…

Solar and Stellar Astrophysics · Physics 2015-05-18 Benhui Yang , P. C. Stancil , N. Balakrishnan , R. C. Forrey

We report rotational quenching cross sections and rate coefficients of HCl due to collisions with He. The close-coupling method and the coupled-states approximation are applied in quantum-mechanical scattering calculations of state-to-state…

Solar and Stellar Astrophysics · Physics 2015-06-18 Benhui Yang , Phillip C. Stancil

Cross sections for the rotational (de)excitation of CO by ground state para- and ortho-H_2 are obtained using quantum scattering calculations for collision energies between 1 and 520 cm^{-1}. A new CO-H_2 potential energy surface is…

Astrophysics · Physics 2008-11-26 M. Wernli , P. Valiron , A. Faure , L. Wiesenfeld , P. Jankowski , K. Szalewicz

Theoretical cross sections for the pressure broadening by hydrogen of rotational transitions of water are compared to the latest available measurements in the temperature range 65-220 K. A high accuracy interaction potential is employed in…

Chemical Physics · Physics 2015-05-19 Laurent Wiesenfeld , Alexandre Faure

Rotational transitions in molecular hydrogen collisions are computed. The two most recently developed potential energy surfaces for the H2-H2 system are used from the following works: 1) A.I. Boothroyd, P.G. Martin, W.J. Keogh, M.J.…

Chemical Physics · Physics 2009-11-11 Renat A. Sultanov , Dennis Guster

We present quantum dynamical calculations that describe the rotational excitation of H$_2$O due to collisions with H atoms. We used a recent, high accuracy potential energy surface, and solved the collisional dynamics with the…

Astrophysics of Galaxies · Physics 2015-06-23 F. Daniel , A. Faure , P. J. Dagdigian , M. -L. Dubernet , F. lique , G. Pineau des forêts

The interpretation of water line emission from existing observations and future HIFI/Herschel data requires a detailed knowledge of collisional rate coefficients. Among all relevant collisional mechanisms, the rotational (de)excitation of…

Astrophysics · Physics 2009-11-13 A. Faure , N. Crimier , C. Ceccarelli , P. Valiron , L. Wiesenfeld , M. -L. Dubernet

New calculations for rotational excitation of cyanoacetylene by collisions with hydrogen molecules are performed to include the lowest 38 rotational levels of HC3N and kinetic temperatures to 300 K. Calculations are based on the interaction…

Astrophysics of Galaxies · Physics 2016-06-15 A. Faure , F. Lique , L. Wiesenfeld

We report pressure broadening coefficients for the 21 electric-dipole transitions between the eight lowest rotational levels of ortho-H$_2$O and para-H$_2$O molecules by collisions with He at temperatures from 20 to 120 K. These…

Chemical Physics · Physics 2016-06-07 M. I. Hernández , J. M. Fernández , G. Tejeda , E. Moreno , S. Montero

Rates of conversions of molecular internal energy to and from kinetic energy by means of molecular collision allows to compute collisional line shapes and transport properties of gases. Knowledge of ro-vibrational quenching rates is…

Chemical Physics · Physics 2022-07-27 Laurent Wiesenfeld

We extend our recent theoretical work on the bending relaxation of H$_2$O in collisions with H$_2$ by including the three water modes of vibration coupled with rotation, as well as the rotation of H$_2$. Our full quantum close-coupling…

Chemical Physics · Physics 2023-11-16 Ricardo Manuel Garcia-Vazquez , Alexandre Faure , Thierry Stoecklin

In this work we report the results concerning calculations for quantum-mechanical rotational transitions in molecular hydrogen, H$_2$, induced by an ultra-cold ground state anti-hydrogen atom $\bar{H}_{1s}$. The calculations are…

Atomic Physics · Physics 2015-05-14 Renat A. Sultanov , Sadhan K. Adhikari , Dennis Guster

Carbon monoxide is a simple molecule present in many astrophysical environments, and collisional excitation rate coefficients due to the dominant collision partners are necessary to accurately predict spectral line intensities and extract…

Astrophysics of Galaxies · Physics 2015-11-17 Kyle M. Walker , L. Song , B. H. Yang , G. C. Groenenboom , A. van der Avoird , N. Balakrishnan , R. C. Forrey , P. C. Stancil

New quantum scattering calculations for rotational deexcitation transitions of CO induced by H collisions using two CO-H potential energy surfaces (PESs) from Shepler et al. (2007) are reported. State-to-state rate coefficients are computed…

Solar and Stellar Astrophysics · Physics 2015-06-15 Benhui Yang , P. C. Stancil , N. Balakrishnan , R. C. Forrey , J. M. Bowman

We present the first accurate rate coefficients for the rotational excitation of CO by H2O in the kinetic temperature range 5-100 K. The statistical adiabatic channel method (SACM) is combined with a high-level rigid-rotor CO-H2O…

Earth and Planetary Astrophysics · Physics 2020-02-13 A. Faure , F. Lique , J. Loreau

Results for quantum mechanical calculations of the integral cross sections and corresponding thermal rate coefficients for para-/ortho-H2+HD collisions are presented. Because of significant astrophysical interest in regard to the cooling of…

Chemical Physics · Physics 2015-05-13 Renat A. Sultanov , Avas V. Khugaev , Dennis Guster

The molecular anion C$_2^-$ has been of interest in the last few years as a candidate for laser cooling due to its electronic structure and favourable branching ratios to the ground electronic and vibrational state. Molecular hydrogen has…

The relative orientation of colliding molecules plays a key role in determining the rates of chemical processes. Here we examine in detail a prototypical example: rotational quenching of HD in cold collisions with H2. We show that the…

Chemical Physics · Physics 2020-09-21 J. F. E. Croft , N. Balakrishnan
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