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The interaction of a short, few-cycle light pulse and an atom which is prepared initially in a superposition of two stationary states is shown to exhibit strong signatures of atomic coherence. For a given waveform of the laser pulse,…

Atomic Physics · Physics 2017-01-04 Viktor Ayadi , Mihaly G. Benedict , Peter Dombi , Peter Foldi

Theoretical study on H$_2^+$ in an intense infrared laser field on the attosecond time-scale reveals that the molecular ion shows multiple bursts of ionization within a half-cycle of the laser field oscillation, in contrast to the widely…

Chemical Physics · Physics 2010-12-10 Norio Takemoto , Andreas Becker

In conditions where the interaction betweeen an atom and a short high-frequency extreme ultraviolet laser pulse is a perturbation, we show that a simple theoretical approach, based on Coulomb-Volkov-type states, can make reliable…

Atomic Physics · Physics 2009-11-07 Guillaume Duchateau , Eric Cormier , Robert Gayet

We report the breakdown of the electric dipole approximation in the long-wavelength limit in strong-field ionization with linearly polarized few-cycle mid-infrared laser pulses at intensities on the order of 10$^{13}$ W/cm$^2$.…

Atomic Physics · Physics 2014-12-16 A. Ludwig , J. Maurer , B. W. Mayer , C. R. Phillips , L. Gallmann , U. Keller

Ultraintense pulses from X-ray free-electron lasers can drive, within femtoseconds, multiple processes in the inner shells of atoms and molecules in all phases of matter. The ensuing complex ionization pathways of outer-shell electrons from…

Propagation of short and ultra-intense laser pulses in a semi-infinite space of overdense hydrogen plasma is analyzed via fully-relativistic, real geometry particle-in-cell (PIC) simulations including radiation friction. The relativistic…

Plasma Physics · Physics 2019-10-02 Masahiro Yano , Alexei Zhidkov , James Koga , Tomonao Hosokai , Ryosuke Kodama

We predict new end-of-pulse behavior in high-field atomic double ionization. Calculations of atomic electron trajectories in short intense laser pulses confirm our analysis of elliptical polarization. We exhibit a four-band structure in ion…

Atomic Physics · Physics 2010-08-20 Xu Wang , J. H. Eberly

Ionization by relativistically intense laser pulses of finite duration is considered in the framework of strong-field quantum electrodynamics. Our main focus is on the formation of ionization supercontinua. More specifically, when studying…

Atomic Physics · Physics 2016-07-13 K. Krajewska , J. Z. Kamiński

We demonstrate how the shape of femtosecond laser pulses can be tailored in order to obtain maximal ionization of atoms or molecules. For that purpose, we have overlayed a direct-optimization scheme on top of a fully unconstrained…

Computational Physics · Physics 2015-05-13 A. Castro , E. Rasanen , A. Rubio , E. K. U. Gross

We investigate electron correlation effects in internuclear-distance-dependent enhanced ionization of $\mathrm{H}_2$, $\mathrm{LiH}$, and $\mathrm{HF}$ molecules by intense near-infrared laser pulses using a 3D description of the systems…

Atomic Physics · Physics 2019-02-27 Siddhartha Chattopadhyay , Lars Bojer Madsen

We extend the semiclassical two-step model [Phys. Rev. A 94, 013415 (2016)] to include a multielectron polarization-induced dipole potential. Using this model we investigate the imprints of multielectron effects in the momentum…

Atomic Physics · Physics 2018-08-22 N. I. Shvetsov-Shilovski , M. Lein , L. B. Madsen

The uncorrelated (``sequential'') and correlated (``nonsequential'') double ionization of the H2 molecule in strong laser pulses is investigated using the tools of nonlinear dynamics. We focus on the phase-space dynamics of this system,…

Chaotic Dynamics · Physics 2009-11-30 François Mauger , Cristel Chandre , T. Uzer

Intense, ultrashort pulses of 800 nm laser light (12 fs, $\sim$4 optical cycles) of peak intensity 5$\times$10$^{14}$ W cm$^{-2}$ have been used to irradiate gas-phase Xe$_n$ clusters ($n$=500-25,000) so as to induce multiple ionization and…

Atomic and Molecular Clusters · Physics 2015-05-19 D. Mathur , F. A. Rajgara

The photoionization of a helium atom by short intense laser pulses is studied theoretically in the vicinity of the $2s2p\,^1P$ doubly-excited state with the intention to investigate the impact of the intensity and duration of the exciting…

Atomic Physics · Physics 2017-09-20 Anton N. Artemyev , Lorenz S. Cederbaum , Philipp V. Demekhin

We consider the classical dynamics of a two-electron system subjected to an intense bichromatic linearly polarized laser pulse. By varying the parameters of the field, such as the phase lag and the relative amplitude between the two colors…

Chaotic Dynamics · Physics 2011-04-04 Adam Kamor , Francois Mauger , Cristel Chandre , Turgay Uzer

The ionization of two-active-electron systems by intense laser fields is investigated theoretically. In comparison with time-dependent Hartree-Fock and exact two electron simulation, we show that the ionization rate is overestimated in SAE…

Atomic Physics · Physics 2015-06-18 Zengxiu Zhao , Jianmin Yuan

Two-color laser fields offer significantly enhanced control over electron excitation dynamics under ultrashort intense laser pulses compared to monochromatic fields. However, their strong nonlinearity necessitates computationally expensive…

Optics · Physics 2025-07-03 Mizuki Tani , Kenichi L. Ishikawa , Tomohito Otobe

Joint electron-ion energy spectra for the dissociative ionization of a model H$_2^+$ in few-cycle, infrared laser pulses are calculated via the numerical ab initio solution of the time-dependent Schr\"odinger equation. A strong,…

Atomic Physics · Physics 2017-11-21 V. Mosert , D. Bauer

In a previous publication, procedures were proposed for unambiguously extracting amplitudes for single and double ionization from a time-dependent wavepacket by effectively propagating for an infinite time following a radiation pulse. Here…

Atomic Physics · Physics 2009-11-13 A. Palacios , T. N. Rescigno , C. W. McCurdy

The acceleration of ions in the interaction of high intensity laser pulses with overdense plasmas is investigated with particle-in-cell simulations. For circular polarization of the laser pulses, high-density ion bunches moving into the…

Plasma Physics · Physics 2009-11-10 Andrea Macchi , Federica Cattani , Tatiana V. Liseykina , Fulvio Cornolti