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Deterministic control of coupled ferroelectric and antiferromagnetic orders remains a central challenge in multiferroics, limiting their integration into functional magnetoelectrics and magnonic-devices. (111)pc BiFeO3 with a robust single…

Magnetic phase transitions in multiferroic bismuth ferrite (BiFeO3) induced by magnetic field, epitaxial strain, and composition modification are considered. These transitions from a spatially modulated spin spiral state to a homogenous…

Strongly Correlated Electrons · Physics 2008-12-28 A. M. Kadomtseva , Yu. F. Popov , A. P. Pyatakov , G. P. Vorob'ev , A. K. Zvezdin , D. Viehland

The effects of high magnetic fields applied perpendicular to the spontaneous ferroelectric polarization on single crystals of BiFeO$_3$ were investigated through magnetization, magnetostriction, and neutron diffraction measurements. The…

The magnetic-field-dependent spin ordering of strained BiFeO3 films is determined using nuclear resonant scattering and Raman spectroscopy. The critical field required to destroy the cycloidal modulation of the Fe spins is found to be…

Epitaxial strain has emerged as a powerful tool to tune magnetic and ferroelectric properties in functional materials such as in multiferroic perovskite oxides. Here, we use first-principles calculations to explore the evolution of magnetic…

Materials Science · Physics 2023-11-23 Sebastian Meyer , Bin Xu , Laurent Bellaiche , Bertrand Dupé

A morphotropic phase boundary driven by epitaxial strain has been observed in a lead-free multiferroic BiFeO3 thin films and the strain-driven phase transitions were widely reported to be iso-symmetric Cc-Cc ones by recent works. In this…

Non-collinear spin order that breaks space inversion symmetry and allows efficient electric-field control of magnetism makes BiFeO$_3$ a promising candidate for applications in low-power spintronic devices. Epitaxial strain effects have…

We study the electrical behavior of multiferroic BiFeO$_3$ by means of first-principles calculations. We do so by constraining a specific component of the electric displacement field along a variety of structural paths, and by monitoring…

Materials Science · Physics 2016-01-20 Massimiliano Stengel , Jorge Íñiguez

The magnetic field induced rearrangement of the cycloidal spin structure in ferroelectric mono-domain single crystals of the room-temperature multiferroic BiFeO$_3$ is studied using small-angle neutron scattering (SANS). The cycloid…

Strongly Correlated Electrons · Physics 2018-04-11 S. Bordács , D. G. Farkas , J. S. White , R. Cubitt , L. DeBeer-Schmitt , T. Ito , I. Kézsmárki

The ZFC and FC magnetization dependence on temperature was measured for BiFeO3 ceramics at the applied magnetic field up to H=10T in 2K-1000K range. The antiferromagnetic order was detected from the hysteresis loops below the Neel…

Materials Science · Physics 2013-05-15 B. Andrzejewski , A. Molak , B. Hilczer , A. Budziak , R. Bujakiewicz-Koronska

The presence of domains in ferroic materials can negatively affect their macroscopic properties and hence their usefulness in device applications. From an experimental perspective, measuring materials comprising multiple domains can…

Strongly Correlated Electrons · Physics 2019-02-20 N. Waterfield Price , A. M. Vibhakar , R. D. Johnson , J. Schad , W. Saenrang , A. Bombardi , F. P. Chmiel , C. B. Eom , P. G. Radaelli

We discuss theoretically phase transitions in frustrated antiferromagnets with biaxial anisotropy or dipolar forces in magnetic field applied along the easy axis at $T=0$. There are well-known sequences of phase transitions upon the field…

Strongly Correlated Electrons · Physics 2019-09-04 O. I. Utesov , A. V. Syromyatnikov

Multiferroic oxides, such as BiFeO3, have garnered significant attention due to their coupled ferroelectric, magnetic, and elastic properties, offering exciting opportunities for multifunctional device applications. Controlling phase…

Materials Science · Physics 2025-02-19 Fei Sun , Chao Chen , Deyang Chen , Minghui Qin , Xubing Lu , Xingsen Gao , Christopher T Nelson , Jun-Ming Liu

A key challenge in antiferromagnetic spintronics is the control of spin configuration on nanometer scales applicable to solid-state technologies. Bismuth ferrite (BiFeO3) is a multiferroic material that exhibits both ferroelectricity and…

In the effective Ising spin-1/2 antiferromagnetic chain system BaCo$_2$V$_2$O$_8, the magnetic-field influence is highly anisotropic. For magnetic fields along the easy axis $c$, the N\'{e}el order is strongly suppressed already for low…

Strongly Correlated Electrons · Physics 2015-06-15 S. K. Niesen , G. Kolland , M. Seher , O. Breunig , M. Valldor , M. Braden , B. Grenier , T. Lorenz

The physical properties of epitaxial films can fundamentally differ from those of bulk single crystals even above the critical thickness. By a combination of non-resonant x-ray magnetic scattering, neutron diffraction and vector-mapped…

Strongly Correlated Electrons · Physics 2016-10-26 N. Waterfield Price , R. D. Johnson , W. Saenrang , F. Maccherozzi , S. S. Dhesi , A. Bombardi , F. P. Chmiel , C. -B. Eom , P. G. Radaelli

We have studied the magnetic field dependence of far-infrared active magnetic modes in a single ferroelectric domain \BFO/ crystal at low temperature. The modes soften close to the critical field of 18.8\,T along the [001] (pseudocubic)…

Strongly Correlated Electrons · Physics 2013-06-26 U. Nagel , Randy S. Fishman , T. Katuwal , H. Engelkamp , D. Talbayev , Hee Taek Yi , S. -W. Cheong , T. Rõõm

A theoretical description of the sequence of magnetic phases in Co3TeO6 is presented. The strongly first-order character of the transition to the commensurate multiferroic ground state, induced by coupled order parameters corresponding to…

Strongly Correlated Electrons · Physics 2012-07-06 Pierre Tolédano , Vera Carolus , Matthias Hudl , Thomas Lottermoser , Dmitry D. Khalyavin , Sergey A. Ivanov , Manfred Fiebig

Magnetoelectric multiferroics, materials with intrinsically coupled electric polarization and magnetic order, promise ultralow-power switching, nonvolatile memory, and energy-efficient signal transduction. Yet practical deployment demands…

A current challenge in the field of magnetoelectric multiferroics is to identify systems that allow a controlled tuning of states displaying distinct magnetoelectric responses. Here we show that the multiferroic ground state of the…

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