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The nucleation and growth of two--dimensional islands is studied with Monte Carlo simulations of a pair--bond solid--on--solid model of epitaxial growth. The conventional description of this problem in terms of a well--defined critical…

Condensed Matter · Physics 2009-10-28 C. Ratsch , P. Šmilauer , A. Zangwill , D. D. Vvedensky

We generalize the level set approach to model epitaxial growth to include thermal detachment of atoms from island edges. This means that islands do not always grow and island dissociation can occur. We make no assumptions about a critical…

Materials Science · Physics 2009-11-07 M. Petersen , C. Ratsch , R. E. Caflisch , A. Zangwill

We study statistical properties of the Kolmogorov-Avrami-Johnson-Mehl nucleation-and-growth model in one dimension. We obtain exact results for the gap density as well as the island distribution. When all nucleation events occur…

Condensed Matter · Physics 2009-10-28 E. Ben-Naim , P. L. Krapivsky

We reexamine the density of two dimensional islands in the submonolayer regime of a homoepitaxially growing surface using the coarse grained Monte Carlo simulation with random sequential updating rather than parallel updating. It turns out…

Statistical Mechanics · Physics 2015-06-25 H. Jeong , B. Kahng , D. E. Wolf

We study irreversible dimer nucleation on top of terraces during epitaxial growth in one and two dimensions, for all values of the step-edge barrier. The problem is solved exactly by transforming it into a first passage problem for a random…

Statistical Mechanics · Physics 2007-05-23 Paolo Politi , Claudio Castellano

We study the configurational structure of the point-island model for epitaxial growth in one dimension. In particular, we calculate the island gap and capture zone distributions. Our model is based on an approximate description of…

Statistical Mechanics · Physics 2012-03-12 Diego Luis Gonzalez Cabrera , Alberto Pimpinelli , T. L. Einstein

We introduce a new equation describing epitaxial growth processes. This equation is derived from a simple variational geometric principle and it has a straightforward interpretation in terms of continuum and microscopic physics. It is also…

Statistical Mechanics · Physics 2009-11-13 Carlos Escudero

We develop a theory for nucleation on top of islands in epitaxial growth based on the derivation of lifetimes and rates governing individual microscopic processes. These processes are strongly affected by the additional step edge barrier…

Materials Science · Physics 2009-10-31 S. Heinrichs , J. Rottler , Ph. Maass

Understanding surface dynamics during epitaxial film growth is key to growing high quality materials with controllable properties. X-ray photon correlation spectroscopy (XPCS) using coherent x-rays opens new opportunities for in situ…

In the electrochemical deposition of thin films the measurement of the current-time curve does not allow for a direct determination of the nucleus growth law, electrode surface coverage and mean film thickness. In this work we present a…

Soft Condensed Matter · Physics 2018-03-07 S. Politi , M. Tomellini

We develop a theory of nucleation on top of two-dimensional islands bordered by steps with an additional energy barrier $\Delta E_S$ for descending atoms. The theory is based on the concept of the residence time of an adatom on the…

Materials Science · Physics 2007-05-23 Joachim Krug , Paolo Politi , Thomas Michely

We investigate submonolayer epitaxial growth with a fixed monomer flux and irreversible aggregation of adatom islands due to their effective diffusion. When the diffusivity D_k of an island of mass k is proportional to k^{-\mu}, a…

Statistical Mechanics · Physics 2009-10-30 P. L. Krapivsky , J. F. F. Mendes , S. Redner

The capture numbers entering the rate equations (RE) for submonolayer film growth are determined from extensive kinetic Monte Carlo (KMC) simulations for simple representative growth models yielding point, compact, and fractal island…

Statistical Mechanics · Physics 2012-08-16 Martin Körner , Mario Einax , Philipp Maass

In this thesis we present a kinetic Monte Carlo model for the description of epitaxial graphene growth. Experimental results suggest a growth mechanism by which clusters of 5 carbon atoms are an intermediate species necessary for nucleation…

Mesoscale and Nanoscale Physics · Physics 2012-04-03 B. Monserrat

The self-consistency of the distributional fixed-point equation (DFPE) approach to understanding the statistical properties of island nucleation and growth during submonolayer deposition is explored. We perform kinetic Monte Carlo…

Mesoscale and Nanoscale Physics · Physics 2018-11-21 Hrvojka Krcelic , Michael Grinfeld , Paul Mulheran

The formation of stable dimers on top of terraces during epitaxial growth is investigated in detail. In this paper we focus on mean-field theory, the standard approach to study nucleation. Such theory is shown to be unsuitable for the…

Statistical Mechanics · Physics 2007-05-23 Paolo Politi , Claudio Castellano

The effects of adsorbates on nucleation and growth of two-dimensional islands is investigated by kinetic Monte Carlo simulations and rate equation theory. The variation of island morphology with adsorbate parameters is discussed and the…

Materials Science · Physics 2007-05-23 Miroslav Kotrla , Joachim Krug , Pavel Smilauer

We simulated the growth of 2D islands with 2 kinds of diffusion atoms using the kinetic Monte- Carlo (kMC) method. As a result, we found that the slow atoms tend to create nuclei and determine the island volume distribution, along with…

Atomic and Molecular Clusters · Physics 2015-03-17 R. Yamauchi , X. M. Lu , M. Koyama , H. Sasakura , Y. Nakata , S. Muto

The distributions of inter-island gaps and captures zones for islands nucleated on a one-dimensional substrate during submonolayer deposition are considered using a novel retrospective view. This provides an alternative perspective on why…

Statistical Mechanics · Physics 2015-03-20 Paul A. Mulheran , Kenneth P. O'Neill , Michael Grinfeld , Wilson Lamb

In studies of island nucleation and growth, the distribution of capture zones, essentially proximity cells, can give more insight than island-size distributions. In contrast to the complicated expressions, ad hoc or derived from rate…

Statistical Mechanics · Physics 2009-10-27 Alberto Pimpinelli , T. L. Einstein
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