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We explore the relaxation of photo-excited graphene by solving a transient Boltzmann transport equation with electron-phonon (e-ph) and electron-electron (e-e) scattering. Simulations show that when the excited carriers are relaxed by e-ph…

Mesoscale and Nanoscale Physics · Physics 2011-09-15 Raseong Kim , Vasili Perebeinos , Phaedon Avouris

Ultrafast optical pump-probe spectroscopy measurement on monolayer graphene observes significant optical nonlinearities. We show that strongly photoexcited graphene monolayers with 35 fs pulses quasi-instantaneously build up a broadband,…

Mesoscale and Nanoscale Physics · Physics 2015-06-15 Junhua Zhang , Joerg Schmalian , Tianqi Li , Jigang Wang

The transient evolution of carriers in an intrinsic graphene under ultrafast excitation, which is caused by the collisionless interband transitions, is studied theoretically. The energy relaxation due to the quasielastic acoustic phonon…

Mesoscale and Nanoscale Physics · Physics 2015-05-14 P. N. Romanets , F. T. Vasko

We present here a general formulation for the interband dynamical optical conductivity in the nonlinear regime of graphene in the presence of a quantum bath comprising phonons and electrons. Our main focus is the relaxation behavior of the…

Mesoscale and Nanoscale Physics · Physics 2023-07-10 Bristi Ghosh , Sushanta Dattagupta , Malay Bandyopadhyay

Mechanism of transient population inversion in graphene with multi-splitted (interdigitated) top-gate and grounded back gate is suggested and examined for the mid-infrared (mid-IR) spectral region. Efficient stimulated emission after fast…

Mesoscale and Nanoscale Physics · Physics 2015-06-16 A. Satou , F. T. Vasko , T. Otsuji , V. V. Mitin

We study inelastic energy relaxation in graphene for low energies to find out how electrons scatter with acoustic phonons and other electrons. By coupling the graphene to superconductors, we create a strong dependence of the measured…

Mesoscale and Nanoscale Physics · Physics 2015-05-27 Juha Voutilainen , Aurelien Fay , Pasi Häkkinen , Janne K. Viljas , Tero T. Heikkilä , Pertti J. Hakonen

We study the characteristics of photogenerated electron-hole plasma in optically pumped graphene layers at elevated (room) temperatures when the interband and intraband processes of emission and absorption of optical phonons play a crucial…

Mesoscale and Nanoscale Physics · Physics 2015-05-27 V. Ryzhii , M. Ryzhii , V. Mitin , A. Satou , T. Otsuji

We study the effect of population inversion associated with the electron and hole injection in graphene p-i-n structures at the room and slightly lower temperatures. It is assumed that the recombination and energy relaxation of electrons…

Mesoscale and Nanoscale Physics · Physics 2015-05-30 V. Ryzhii , M. Ryzhii , V. Mitin , T. Otsuji

Since graphene has no band gap, photoluminescence is not expected from relaxed charge carriers. We have, however, observed significant light emission from graphene under excitation by ultrashort (30-fs) laser pulses. Light emission was…

Mesoscale and Nanoscale Physics · Physics 2010-09-20 Chun Hung Lui , Kin Fai Mak , Jie Shan , Tony F. Heinz

We present a new paradigm for understanding optical absorption and hot electron dynamics experiments in graphene. Our analysis pivots on assigning proper importance to phonon assisted indirect processes and bleaching of direct processes. We…

Materials Science · Physics 2017-11-22 Yuan Yang , Grigory Kolesov , Lucas Kocia , Eric J. Heller

We present an experimental observation of non-linear up- and down-converted optical luminescence of graphene and thin graphite subject to picosecond infrared laser pulses. We show that the excitation yields to a high density electron-hole…

Materials Science · Physics 2010-10-01 Rainer J. Stoehr , Roman Kolesov , Jens Pflaum , Joerg Wrachtrup

We investigate the energy relaxation of hot carriers produced by photoexcitation of graphene through coupling to both intrinsic and remote (substrate) surface polar phonons using the Boltzmann equation approach. We find that the energy…

Mesoscale and Nanoscale Physics · Physics 2012-08-15 Tony Low , Vasili Perebeinos , Raseong Kim , Marcus Freitag , Phaedon Avouris

We compute the electronic component of the thermal conductivity (TC) and the thermoelectric power (TEP) of monolayer graphene, within the hydrodynamic regime, taking into account the slow rate of carrier population imbalance relaxation.…

Mesoscale and Nanoscale Physics · Physics 2009-11-13 Matthew S. Foster , Igor L. Aleiner

We theoretically study the population inversion and negative dynamic conductivity in intrinsic graphene in the terahertz (THz) frequency range upon pulse photoexcitation with near-/mid-infrared wavelength. The threshold pulse energy…

Mesoscale and Nanoscale Physics · Physics 2015-06-11 A. Satou , V. Ryzhii , Y. Kurita , T. Otsuji

We study the relaxation dynamics of laser-excited non-equilibrium electron distributions in the valence- and conduction band of a dielectric. We apply Boltzmann collision integrals to trace the influence of different scattering mechanisms…

Statistical Mechanics · Physics 2023-04-28 Nils Brouwer , Steffen Hirtle , Baerbel Rethfeld

A short overview of theoretical models for the description of the relaxation processes in metals excited by a short laser pulse is presented. The main effort is given to description of different processes which are taking place after…

Strongly Correlated Electrons · Physics 2020-05-20 V. V. Kabanov

Using transient absorption (TA) microscopy as a hot electron thermometer we show disorder-assisted acoustic-phonon supercollisions (SCs) best describes the rate-limiting relaxation step in graphene over a wide range of lattice temperatures…

Materials Science · Physics 2013-10-25 Matt W. Graham , Su-Fei Shi , Zenghui Wang , Daniel C. Ralph , Jiwoong Park , Paul L. McEuen

Creating non-equilibrium states of matter with highly unequal electron and lattice temperatures allows unsurpassed insight into the dynamic coupling between electrons and ions through time-resolved energy relaxation measurements. Recent…

We examine the photoconductivity of an intrinsic graphene associated with far- and mid-infrared irradiation at low temperatures. The model under consideration accounts for the excitation of the electron-hole pairs by incident radiation, the…

Materials Science · Physics 2008-05-27 F. T. Vasko V. Ryzhii

Using optical-pump terahertz-probe spectroscopy, we study the relaxation dynamics of photoexcited carriers in graphene at different temperatures. We find that at lower temperatures the tail of the relaxation transients as measured by the…

Mesoscale and Nanoscale Physics · Physics 2015-05-30 Jared H. Strait , Haining Wang , Shriram Shivaraman , Virgil B. Shields , Michael G. Spencer , Farhan Rana
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