Related papers: Metal nanoparticle plasmons operating within quant…
Self-oscillators are intriguing due to their ability to sustain periodic motion without periodic stimulus. They remain rare as achieving such behavior requires a balance of energy input, dissipation and non-linear feedback mechanism. Here,…
Quantum resources can enhance the sensitivity of a device beyond the classical shot noise limit and, as a result, revolutionize the field of metrology through the development of quantum-enhanced sensors. In particular, plasmonic sensors,…
The key component of nanoplasmonics is metals. For a long time, gold and silver have been the metals of choice for constructing plasmonic nanodevices because of their excellent optical properties. However, these metals possess a common…
We used high order harmonics of a femtosecond titanium-doped sapphire system (pulse duration 25 fs) to realise Ultraviolet Photoelectron Spectroscopy (UPS) measurements on diamond. The UPS spectra were measured for harmonics in the range 13…
We show that the dynamics of the surface plasmon in metallic nanoparticles damped by its interaction with particle-hole excitations can be modelled by a single degree of freedom coupled to an environment. In this approach, the fast decrease…
We develop a theoretical model of the surface plasmon resonance of metallic nanospheres in the size range down to the single nanometer size. Within this model we explicitly show how different microscopic mechanisms, namely quantization due…
The interaction of light with matter has triggered the interest of scientists for long time. The area of plasmonics emerges in this context through the interaction of light with valence electrons in metals. The random phase approximation in…
Plasmonic molecular nanojunctions exhibit opto-mechanical coupling at the nanoscale, enabling intertwined optical, vibrational and electronic phenomena. Here, we demonstrate plasmon-mediated phonon pumping, driven by inelastic electron…
Gold nanorod has generated great research interest due to its tunable longitudinal plasmon resonance. However, little progress has been made in the understanding of the effect. A major reason is that, except for metallic spheres and…
We investigate theoretically the non-Markovian dynamics of a degenerate V-type quantum emitter in the vicinity of a metallic nanosphere, a system that exhibits quantum interference in spontaneous emission due to the anisotropic Purcell…
We present experiments in which the interaction of a single gold nanoparticle with glass substrates or with another gold particle can be tuned by in-situ control of their separations using scanning probe technology. We record the plasmon…
Using time-resolved pump-probe spectroscopy we have performed the first investigation of the vibrational modes of gold nanoshells. The fundamental isotropic mode launched by a femtosecond pump pulse manifests itself in a pronounced…
Regular arrays of metal nanoparticles on metal films have tuneable optical resonances that can be applied for surface enhanced Raman scattering or biosensing. With the aim of developing more surface selective geometries we investigate…
Combining miniaturization and good operating speed is a compelling yet crucial task for our society. Plasmonic waveguides enable the possibility of carrying information at optical operating speed while maintaining the dimension of the…
With the help of a theoretical model and finite-difference-time-domain simulations based on the hydrodynamic-Maxwell model, we examine the effect of difference frequency generation in an array of L-shaped metal nano-particles characterized…
The optical response of a coupled nanowire dimer is studied using a fully quantum mechanical approach. The translational invariance of the system allows to apply the time--dependent density functional theory for the plasmonic dimer with the…
We use ultrafast pump-probe transmission spectroscopy to measure the electronic relaxation time for electrons in cobalt nanoparticles embedded on glass substrate using femtosecond laser pulses. We found that the plasmon excitation is…
We present a theoretical study of the radiative and nonradiative decay rates of an optical emitter in close proximity to a prolate-shaped metal nanoparticle. We use the model developed by Gersten and Nitzan, that we correct for radiative…
We report the enhancement of the optical second harmonic signal in non-centrosymmetric semiconductor CdS quantum dots, when they are placed in close contact with isolated silver nanoparticles. The intensity enhancement is about 1000. We…
We present a quantum mechanical approach to calculate broadening of plasmonic resonances in metallic nanostructures due to collisions of electrons with the surface of the structure. The approach is applicable if the characteristic size of…