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We study the linewidth of the surface plasmon resonance in the optical absorption spectrum of metallic nanoparticles, when the decay into electron-hole pairs is the dominant channel. Within a semiclassical approach, we find that the…

Mesoscale and Nanoscale Physics · Physics 2009-11-07 Rafael A. Molina , Dietmar Weinmann , Rodolfo A. Jalabert

Localized-surface plasmon resonance is of importance in both fundamental and applied physics for the subwavelength confinement of optical field, but realization of quantum coherent processes is confronted with challenges due to strong…

Quantum Physics · Physics 2017-12-13 Pai Peng , Yong-Chun Liu , Da Xu , Qi-Tao Cao , Qihuang Gong , Yun-Feng Xiao

The coherent oscillations of mobile charge carriers near the surface of good conductors-surface plasmons-are been exploited in many applications in information technologies, clean energy, high-density data storage, photovoltaics, chemistry,…

Mesoscale and Nanoscale Physics · Physics 2023-12-20 Jacob Khurgin , Anton Yu. Bykov , Anatoly V. Zayats

Generation of energetic (hot) electrons is an intrinsic property of any plasmonic nanostructure under illumination. Simultaneously, a striking advantage of metal nanocrystals over semiconductors lies in their very large absorption cross…

Mesoscale and Nanoscale Physics · Physics 2017-08-31 Lucas V. Besteiro , Xiang-Tian Kong , Zhiming Wang , Gregory V. Hartland , Alexander O. Govorov

We consider theoretically the spaser excited electrically via a nanowire with ballistic quantum conductance. We show that in the extreme quantum regime, i.e., for a single conductance-quantum nanowire, the spaser with the core made of…

Mesoscale and Nanoscale Physics · Physics 2015-06-12 Dabing Li , Mark I. Stockman

We present a theoretical study of the resonance fluorescence spectra of an optically driven quantum dot placed near a single metal nanoparticle. The metallic reservoir coupling is calculated for an 8-nm metal nanoparticle using a…

Mesoscale and Nanoscale Physics · Physics 2013-05-22 Rong-Chun Ge , C. Van Vlack , P. Yao , Jeff. F. Young , S. Hughes

We develop a theory of cooperative emission of light by an ensemble of emitters, such as fluorescing molecules or semiconductor quantum dots, located near a metal nanostructure supporting surface plasmon. The primary mechanism of…

Mesoscale and Nanoscale Physics · Physics 2015-05-14 Vitaliy N. Pustovit , Tigran V. Shahbazyan

The fluorescence of organic fluorophore molecules is enhanced when they are placed in contact with certain metals (Al, Ag, Cu, Au, etc.) whose surface plasmon waves couple into the radiative modes of the molecules and increase the radiative…

Mesoscale and Nanoscale Physics · Physics 2015-04-21 S. Sarkar , B. Kanchibotla , J. D. Nelson , J. D. Edwards , J. Anderson , G. C. Tepper , S. Bandyopadhyay

The random-phase-approximation semiclassical scheme for description of plasmon excitations in large metallic nanospheres (with radius 10--100 nm) is developed for a case of presence of dynamical electric field. The spectrum of plasmons in…

Mesoscale and Nanoscale Physics · Physics 2015-05-18 W. Jacak , J. Krasnyj , J. Jacak , A. Chepok , L. Jacak , W. Donderowicz , D. Z. Hu , D. M. Schaadt

Molecular aggregates on plasmonic nanoparticles have emerged as attractive systems for the studies of cavity quantum electrodynamics. They are highly tunable, scalable, easy to synthesize and offer sub-wavelength confinement, all while…

Quantum emitters coupled to plasmonic nanoantennas produce single photons at unprecedentedly high rates in ambient conditions. This enhancement of quantum emitters' radiation rate is based on the existence of optical modes with highly…

The field of plasmonics is capable of enabling interesting applications in the different wavelength ranges, spanning from the ultraviolet up to the infrared. The choice of plasmonic material and how the material is nanostructured have…

We systematically investigated and quantified how gold (Au) metal nanoparticles (NPs) optical spectra change upon introduction into biological tissue phantoms environment, in which the AuNPs can agglomerate. Quantitative knowledge of how…

Applied Physics · Physics 2021-03-17 J. C. R. Araujo , A. F. G. Monte , R. L. Serrano , W. Iwamoto , A. Antunes , O. Brener , M. Foschini

In this work, the plasmon coupling effect between two gold nanospheres on a gold slab is investigated. At plasmon resonance frequencies, electrons on the surface of the slab are absorbed into spheres and contribute to plasmon oscillation.…

Optics · Physics 2015-05-30 H. Liu , J. Ng , S. B. Wang , Z. H. Hang , C. T. Chan , S. N. Zhu

We study the plasmonic properties of coupled noble-metal nanochains in the case of different number of coupled chains and doping by different transition-metal (TM) atoms within the time-dependent density-functional theory (TDDFT) approach.…

Mesoscale and Nanoscale Physics · Physics 2014-09-12 Neha Nayyar , Volodymyr Turkowski , Talat S. Rahman

Plasmons in nanostructured metals are widely utilized to trigger strong light--matter interactions with quantum light sources. While the nonclassical behavior of such quantum emitters (QEs) is well-understood in this context, the role of…

The electronic environment causes decoherence and dissipation of the collective surface plasmon excitation in metallic nanoparticles. We show that the coupling to the electronic environment influences the width and the position of the…

Mesoscale and Nanoscale Physics · Physics 2007-05-23 Guillaume Weick , Gert-Ludwig Ingold , Rodolfo A. Jalabert , Dietmar Weinmann

We study theoretically the emission and lasing properties of a single nanoshell spaser nanoparticle, or plasmonic nanolaser, made of an active core (gain material) and a plasmonic metal shell. Based on an analytical framework coupling…

Plasmonic nanoantenna is of promising applications in optical sensing, single-molecular detection, and enhancement of optical nonlinear effect, surface optical spectroscopy, photochemistry, photoemission, photovoltaics, etc. Here we show…

Optics · Physics 2015-08-14 Qiang Zhang , Jun-Jun Xiao , Meili Li , Dezhuan Han , Lei Gao

Steady-state plasmonic lasing is studied theoretically for a system consisting of many dye molecules arranged regularly around a gold nano-sphere. A three-level model with realistic molecular dissipation is employed to analyze the…

Optics · Physics 2018-01-31 Yuan Zhang , Klaus Mølmer
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