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Interatomic Coulombic decay (ICD) plays a crucial role in weakly bound complexes exposed to intense or high-energy radiation. So far, neutral or ionic atoms or molecules have been prepared in singly excited electron or hole states which can…

Interatomic Coulombic decay (ICD) is induced in helium (He) nanodroplets by photoexciting the n=2 excited state of He^+ using XUV synchrotron radiation. By recording multiple coincidence electron and ion images we find that ICD occurs in…

Atomic and Molecular Clusters · Physics 2017-07-24 M. Shcherbinin , A. C. LaForge , V. Sharma , M. Devetta , R. Richter , R. Moshammer , T. Pfeifer , M. Mudrich

Interatomic Coulombic decay (ICD) processes play a crucial role in weakly bound complexes exposed to intense or high-energy radiation. Using large helium nanodroplets, we demonstrate that ICD is efficient even when the droplets are…

An ultrafast mechanism belonging to the family of interatomic Coulombic decay (ICD) phenomena is proposed. When two excited species are present, an ultrafast energy transfer can take place bringing one of them to its ground state and…

Ionization of matter by energetic radiation generally causes complex secondary reactions which are hard to decipher. Using large helium nanodroplets irradiated by XUV photons, we show that the full chain of processes ensuing primary…

Atomic and Molecular Clusters · Physics 2023-07-26 L. Ben Ltaief , K. Sishodia , S. Mandal , S. De , S. R. Krishnan , C. Medina , N. Pal , R. Richter , T. Fennel , M. Mudrich

Irradiation of condensed matter with ionizing radiation generally causes direct photoionization as well as secondary processes that often dominate the ionization dynamics. Here, large helium (He) nanodroplets with radius >40 nm doped with…

Atomic and Molecular Clusters · Physics 2024-12-06 L. Ben Ltaief , K. Sishodia , J. D. Asmussen , A. R. Abid , S. R. Krishnan , H. B. Pedersen , N. Sisourat , M. Mudrich

Molecular mechanisms that enable collective and upconverted energy transfer from multiple photoacceptors to a non-absorbing spectator reaction center are highly desirable for efficient light-energy utilization. Here, we show that…

Chemical Physics · Physics 2026-03-05 Saroj Barik , Pratikkumar Thakkar , Siddhartha S. Payra , Yash Lenka , Y. Sajeev , G. Aravind

Photoexcitation of van der Waals complexes can lead to several decay pathways depending on the nature of the potential energy surfaces. Upon excitation of a chromophore in a complex, ionization of its weakly bound neighbour via energy…

Chemical Physics · Physics 2022-01-14 Namitha Brijit Bejoy , Nitin. K Singh , Balanarayan Pananghat , G. Naresh Patwari

Excited atoms and molecules can utilize their excess energy to ionize a neighboring system by a process named interatomic and intermolecular Coulombic decay (ICD). ICD is ultrafast, in the femtosecond regime, and has many modes of…

Chemical Physics · Physics 2026-03-10 Alan G. Falkowski , Alexander I. Kuleff , Lorenz S. Cederbaum

We report theory for time-resolved spectator resonant Interparticle Coulombic Decay (ICD) processes. Following excitation by a short extreme ultraviolet pulse, the spectrum of the resonant ICD electron develops. Strong-field ionization is…

Quantum Physics · Physics 2020-04-29 Elke Fasshauer , Lars Bojer Madsen

The electron removal and excitation channels in argon dimer target and helium ion projectile collision systems that facilitate interatomic Coulombic decay (ICD) are investigated. We implement an independent-atom and independent-electron…

Atomic and Molecular Clusters · Physics 2026-03-25 Darij Starko , Tom Kirchner

We investigate the onset of photoionization shakeup induced interatomic Coulombic decay (ICD) in He2 at the He+*(n = 2) threshold by detecting two He+ ions in coincidence. We find this threshold to be shifted towards higher energies…

Low-energy-electron emission from resonant Auger final states via intermolecular Coulombic decay (RA-ICD) has been previously described as a promising scenario for controlling radiation damage for medical purposes, but has so far only been…

We report the first observation of intermolecular Coulombic decay (ICD) in liquid water following inner-valence ionization. By combining a monochromatized table-top high-harmonic source with a liquid micro-jet, we recorded electron-electron…

Atomic and Molecular Clusters · Physics 2022-04-05 Pengju Zhang , Conaill Perry , Tran Trung Luu , Danylo Matselyukh , Hans Jakob Wörner

We report on the experimental observation of interatomic Coulombic decay (ICD) in pure $^4$He nanoclusters of mean sizes between $N \approx$ 5000 and 30000 and the subsequent scattering of energetic He$^+$ fragments inside the neutral…

When weakly-bound complexes are multiply excited by intense electromagnetic radiation, energy can be exchanged between neighboring atoms through a type of resonant interatomic Coulombic decay (ICD). This decay mechanism due to multiple…

Interatomic coulombic decay (ICD) is a relaxation process induced by electronic correlation. In this work we study the ICD process in a two coupled Quantum wells (QWs) nano-structure. We study a simple one-dimensional effective potential…

Mesoscale and Nanoscale Physics · Physics 2015-06-11 Tamar Goldzak , Liron Gantz , Ido Gilary , Gad Bahir , Nimrod Moiseyev

To exploit the high intensity of laser radiation, we propose to select frequencies at which single-photon absorption is of too low energy and two or more photons are needed to produce states of an atom that can undergo interatomic Coulombic…

Atomic and Molecular Clusters · Physics 2012-01-04 Philipp V. Demekhin , Spas D. Stoychev , Alexander I. Kuleff , Lorenz S. Cederbaum

Single strand breaks are induced in DNA plasmids, pBR322 and pUC19, in aqueous media by intense ultrashort laser pulses (820 nm wavelength, 45 fs pulse duration, 1 kHz repetition rate) at intensities of 1-12 TW cm$^{-2}$. The intense laser…

Biological Physics · Physics 2010-06-03 J. S. D'Souza , J. A. Dharmdhikari , A. K. Dharmdhikair , B. J. Rao , D. Mathur

The elucidation of fundamental mechanisms underlying ion-induced radiation damage of biological systems is crucial for the advancement of radiotherapy with ion beams and for radiation protection in space. The study of ion-induced biodamage…

Biological Physics · Physics 2023-09-06 Ida Friis , Alexey V. Verkhovtsev , Ilia A. Solov'yov , Andrey V. Solov'yov
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