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Photo-acoustic spectroscopy (PAS) is one of the most sensitive non-destructive analysis techniques for gases, fluids and solids. It can operate background-free at any wavelength and is applicable to microscopic and even non-transparent…

Two-dimensional (2D) layered materials have been extensively studied owing to their fascinating and technologically relevant properties. Their functionalities can be often tailored by the interlayer stacking pattern. Low-frequency (LF)…

Mesoscale and Nanoscale Physics · Physics 2017-10-06 Liangbo Liang , Alexander A. Puretzky , Bobby G. Sumpter , Vincent Meunier

Raman spectroscopy is a well established tool for the analysis of vibration spectra, which then allow for the determination of individual substances in a chemical sample, or for their phase transitions. In the…

Numerical Analysis · Mathematics 2020-07-15 Konstantin Fackeldey , Jonas Röhm , Amir Niknejad , Surahit Chewle , Marcus Weber

Currently, no light source exists which is both narrow-band and speckle-free with sufficient brightness for full-field imaging applications. Light emitting diodes (LEDs) are excellent spatially incoherent sources, but are tens of nanometers…

Many imaging applications require increasingly bright illumination sources, motivating the replacement of conventional thermal light sources with light emitting diodes (LEDs), superluminescent diodes (SLDs) and lasers. Despite their…

Optics · Physics 2017-04-05 Brandon Redding , Michael A. Choma , Hui Cao

Stokes Raman scattering is known to be a particularly robust nonlinearity, occurring in virtually every material, with spectra defined by the material and strengths dependent on the material as well as light intensities. This ubiquity has…

Optics · Physics 2021-08-10 Xiao Liu , Zelin Ma , Aku Antikainen , Siddharth Ramachandran

Raman scattering signal can be enhanced through localization of incident field into sub-wavelength hot-spots through plasmonic nano-structures (Surface-enhanced Raman scattering-SERS). Recently, further enhancement of SERS signal via…

An accurate, closed-form expression evaluating the nonlinear interference (NLI) power in coherent optical transmission systems in the presence of inter-channel stimulated Raman scattering (ISRS) is derived. The analytical result enables a…

Signal Processing · Electrical Eng. & Systems 2019-05-22 Daniel Semrau , Robert I. Killey , Polina Bayvel

Raman spectroscopy can provide insight into the molecular composition of cells and tissue. Consequently, it can be used as a powerful diagnostic tool, e.g. to help identify changes in molecular contents with the onset of disease. But robust…

Medical Physics · Physics 2023-08-02 Ciaran Bench , Mads S. Bergholt , Mohamed Ali al-Badri

We employ dual-probe 1-d fs/ps hybrid rotational coherent anti-Stokes Raman spectroscopy to investigate simultaneous temperature, pressure, and O2/N2 measurements for gas-phase diagnostics. The dual-probe HRCARS technique allows for…

We present a simple method and its experimental implementation to completely determine the characteristics of the pump-and-probe pulse and the Stokes pulse in a coherent anti-Stokes Raman scattering microscope at sample level without…

With the wave interferometric approach, we study how extrinsically multiple coherent waves excitation can dramatically alter the overall scattering states, resulting in tailoring the energy assignment among radiation and dissipation. To…

We demonstrate the generation of coherent Stokes pulses with randomized linear-polarization in diamond, when the pump wave-vector and linear polarization were oriented along the $[110]$ and $[1\bar{1}0]$ axes respectively. In this…

We introduce the first method to enable an optical amplification of a coherent Raman spectroscopy signal called radio frequency Doppler Raman spectroscopy. Doppler Raman measurements amplify the optical signals in coherent Raman…

We demonstrate orientation-sensitive multimodal nonlinear optical polarizing microscopy capable of probing orientational, polar, and biaxial features of mesomorphic ordering in soft matter. This technique achieves simultaneous imaging in…

Soft Condensed Matter · Physics 2015-05-19 Taewoo Lee , Rahul P. Trivedi , Ivan I. Smalyukh

Nonlinear interferometry with entangled photons allows for characterizing a sample without detecting the photons interacting with it. This method enables highly sensitive optical sensing in the wavelength regions where efficient detectors…

Optics · Physics 2025-08-11 Kazuki Hashimoto , Dmitri B. Horoshko , Maria V. Chekhova

Strain engineering in semiconductor transistor devices has become vital in the semiconductor industry due to the ever increasing need for performance enhancement at the nanoscale. Raman spectroscopy is a non-invasive measurement technique…

Optics · Physics 2021-06-17 V. Prabhakara , T. Nuytten , H. Bender , W. Vandervorst , S. Bals , J. Verbeeck

We focus on an alignment-free method to estimate the underlying signal from a large number of noisy randomly shifted observations. Specifically, we estimate the mean, power spectrum, and bispectrum of the signal from the observations. Since…

Signal Processing · Electrical Eng. & Systems 2018-07-04 Hua Chen , Mona Zehni , Zhizhen Zhao

Phonon polaritons enable waveguiding and localization of infrared light with extreme confinement and low losses. The spatial propagation and spectral resonances of such polaritons are usually probed with complementary techniques such as…

Spectroscopic stimulated Raman scattering (SRS) imaging has become a useful tool finding a broad range of applications. Yet, wider adoption is hindered by the bulky and environmentally-sensitive solid-state optical parametric oscillator…

Optics · Physics 2021-08-20 Hongli Ni , Peng Lin , Yifan Zhu , Meng Zhang , Yuying Tan , Yuewei Zhan , Ji-Xin Cheng