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In our theoretical study where we combine a nonequilibrium Green's function (NEGF) approach with density functional theory (DFT) we investigate compounds containing a ferrocene moiety which is connected to i) thiol anchor groups on both…

Chemical Physics · Physics 2019-01-30 Xin Zhao , Robert Stadler

We cure the lack of spin torque in semilocal exchange-correlation (XC) functionals by treating XC effects in the framework of spin-current-density-functional theory (SCDFT), and present the implementation of the first kind of this novel…

Materials Science · Physics 2025-01-09 Marie-Therese Huebsch , Fabien Tran , Martijn Marsman

We study new superconductor candidates in functionalized MXenes Zr$_2$NS$_2$, Zr$_2$NCl$_2$, and Sc$_2$NCl$_2$ with $\textit{ab initio}$ calculations based on density functional theory for superconductors (SCDFT). The superconducting…

Superconductivity · Physics 2025-09-29 Alpin N. Tatan , Osamu Sugino

The density functional theory (DFT) interaction energy of a dimer is rigorously derived from the monomer densities. To this end, the supermolecular energy bifunctional is formulated in terms of mutually orthogonal sets of orbitals of the…

Finite-temperature DFT has become of topical interest, partly due to the increasing ability to create novel states of warm-correlated matter (WCM). Subclasses of WCM are Warm-dense matter (WDM), ultra-fast matter (UFM), and high-energy…

Chemical Physics · Physics 2016-03-15 M. W. C. Dharma-wardana

In this thesis we study the strongly-correlated-electron physics of the longstanding H-Tc-superconductivity problem using a non-perturbative method, the Dynamical Mean Field Theory (DMFT), capable to go beyond standard perturbation-theory…

Strongly Correlated Electrons · Physics 2007-10-16 Marcello Civelli

Quantum--Mechanical methods that are both computationally fast and accurate are not yet available for electronic excitations having charge transfer character. In this work, we present a significant step forward towards this goal for those…

Chemical Physics · Physics 2015-06-12 Michele Pavanello , Troy Van Voorhis , Lucas Visscher , Johannes Neugebauer

The density of states of the disordered s-wave superconductor is calculated perturbatively. The effect of Coulomb interaction on diffusively moving electrons in the normal state has been known before, but in the superconducting state both…

Superconductivity · Physics 2019-10-03 Takanobu Jujo

The self consistent version of the density functional theory (DFT) is presented, which allows to calculate the ground state and dynamic properties of finite multi-electron systems such as atoms, molecules and clusters. The exact functional…

Condensed Matter · Physics 2007-05-23 M. Ya. Amusia , V. R. Shaginyan

We develop a semiclassical density functional theory in the context of quantum dots. Coulomb blockade conductance oscillations have been measured in several experiments using nanostructured quantum dots. The statistical properties of these…

Mesoscale and Nanoscale Physics · Physics 2009-10-31 Denis Ullmo , Tatsuro Nagano , Steven Tomsovic , Harold U. Baranger

A model of a strongly correlated electron liquid based on the fermion condensation (FC) is extended to high-temperature superconductors. Within our model, the appearance of FC presents a boundary separating the region of a strongly…

Strongly Correlated Electrons · Physics 2009-10-31 S. A. Artamonov , V. R. Shaginyan

Density functional theory is the workhorse of modern electronic structure calculations, with wide-ranging applications in chemistry, physics, materials science, and machine learning. At its heart lies the exchange-correlation functional, a…

Chemical Physics · Physics 2026-02-20 Fabien Tran , Susi Lehtola , Stefano Pittalis , Miguel A. L. Marques

This work explores the use of joint density-functional theory, a new form of density-functional theory for the ab initio description of electronic systems in thermodynamic equilibrium with a liquid environment, to describe electrochemical…

Materials Science · Physics 2015-06-05 Kendra Letchworth-Weaver , T. A. Arias

The combination of isochoric heating of solids by free electron lasers (FEL) and in situ diagnostics by X-ray Thomson scattering (XRTS) allows for measurements of material properties at warm dense matter (WDM) conditions relevant for…

A system of soft ellipsoid molecules confined between two planar walls is studied using classical Density Functional Theory (DFT). Both the isotropic and nematic phases are considered. The excess free energy is evaluated using two different…

Materials Science · Physics 2009-11-10 David Cheung , Friederike Schmid

The time-dependent density functional theory (TDDFT) is the leading computationally feasible theory to treat excitations by strong electromagnetic fields. Here the theory is applied to coherent optical phonon generation produced by intense…

Materials Science · Physics 2015-06-05 Y. Shinohara , S. A. Sato , K. Yabana , J. -I. Iwata , T. Otobe , G. F. Bertsch

We have introduced a Coulomb correlated normal state to study the superconducting pairing with a Fermi liquid like normal phase background in a 3 dimensional system. The role of the Coulomb correlation has been actively incorporated by…

Superconductivity · Physics 2022-07-20 Koushik Mandal , Ranjan Chaudhury

We have calculated the ground state electronic structure of He under pressure from 0 to 1500 GPa using both all-electron full-potential and pseudopotential methods based on the density functional theory (DFT). We find that throughout this…

Materials Science · Physics 2012-01-10 W. Xiao , Z. X. Tian , W. T. Geng

We study thermal conductivity in the disordered two-dimensional electron liquid in the presence of long-range Coulomb interactions. We describe a microscopic analysis of the problem using as a starting point the partition function defined…

Mesoscale and Nanoscale Physics · Physics 2016-06-22 G. Schwiete , A. M. Finkel'stein

Electronic Coulomb excitations in monolayer silicene are investigated by using the Lindhard dielectric function and a newly developed generalized tight-binding model (G-TBM). G-TBM simultaneously contains the atomic interactions, the…

Mesoscale and Nanoscale Physics · Physics 2015-10-07 Jhao-Ying Wu , Szu-Chao Chen , Godfrey Gumbs , Ming-Fa Lin