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Measurements and a theoretical interpretation of the excitation spectrum of a two-electron quantum dot fabricated on a parabolic Ga[Al]As quantum well are reported. Experimentally, excited states are found beyond the well-known lowest…

Mesoscale and Nanoscale Physics · Physics 2021-12-30 T. Ihn , C. Ellenberger , K. Ensslin , Constantine Yannouleas , Uzi Landman , D. C. Driscoll , A. C. Gossard

Electron-hole correlation in quantum-dot quantum wells (QDQW's) is investigated by incorporating Coulomb and exchange interactions into an empirical tight-binding model. Sufficient electron and hole single-particle states close to the band…

Materials Science · Physics 2009-11-10 Rui-Hua Xie , Garnett W. Bryant , Seungwon Lee , W. Jaskolski

We present an ab initio study of core excitations of solid-state materials focussing on the role of electron-hole correlation. In the framework of an all-electron implementation of many-body perturbation theory into the exciting code, we…

Materials Science · Physics 2017-04-21 Christian Vorwerk , Caterina Cocchi , Claudia Draxl

The adiabatic approximation in time-dependent density functional theory (TDDFT) yields reliable excitation spectra with great efficiency in many cases, but fundamentally fails for states of double excitation character. We discuss how…

Chemical Physics · Physics 2015-05-27 Peter Elliott , Sharma Goldson , Chris Canahui , Neepa T. Maitra

We present experimental coherent two-dimensional Fourier transform spectra of the exciton resonances in semiconductor quantum wells for a pulse sequence that isolates two-quantum coherences. By measuring the real part of the spectra, we can…

Mesoscale and Nanoscale Physics · Physics 2011-11-29 Denis Karaiskaj , Alan D. Bristow , Lijun Yang , Xingcan Dai , Richard P. Mirin , Shaul Mukamel , Steven T. Cundiff

We propose a three-pulse coherent ultrafast optical technique that is particularly sensitive to two-exciton correlations. Two Liouville-space pathways for the density matrix contribute to this signal which reveals double quantum coherences…

Mesoscale and Nanoscale Physics · Physics 2009-11-13 Lijun Yang , Shaul Mukamel

The excitation spectrum of a two-electron quantum dot is investigated by tunneling spectroscopy in conjuction with theoretical calculations. The dot made from a material with negligible Zeeman splitting has a moderate spatial anisotropy…

Mesoscale and Nanoscale Physics · Physics 2007-05-23 C. Ellenberger , T. Ihn , C. Yannouleas , U. Landman , K. Ensslin , D. Driscoll , A. C. Gossard

We show the ferro-rotational nature of the commensurate charge density wave (CCDW) in $1T$-$\mathrm{TaS}_2$ and track its dynamic modulations by temperature-dependent and time-resolved electric quadrupole rotation anisotropy-second harmonic…

We demonstrate how dynamic correlations of heavy-hole and light-hole excitons in semiconductor quantum wells may be investigated by two dimensional correlation spectroscopy (2DCS). The coherent response to three femtosecond optical pulses…

Mesoscale and Nanoscale Physics · Physics 2007-05-23 Lijun Yang , Igor V. Schweigert , Steven T. Cundiff , Shaul Mukamel

Excitons are electron-hole pairs appearing below the band gap in insulators and semiconductors. They are vital to photovoltaics, but are hard to obtain with time-dependent density-functional theory (TDDFT), since most standard…

Materials Science · Physics 2013-05-22 Zeng-hui Yang , Carsten A. Ullrich

Excitons in the weakly interacting regime can be well-described by many-body perturbation theories such as the Bethe-Salpeter equation formalism. However, for materials such as transition metal dichalcogenides moir\'e heterostructures under…

Materials Science · Physics 2026-03-16 Fangzhou Zhao , Carlos Mejuto-Zaera , Angel Rubio , Vojtěch Vlček

The energy spectrum of a two-dimensional electron gas (2DEG) in the fractional quantum Hall regime interacting with an optically injected valence band hole is studied as a function of the filling factor $\nu$ and the separation $d$ between…

Mesoscale and Nanoscale Physics · Physics 2009-10-31 Arkadiusz Wojs , John J. Quinn

Harnessing the optoelectronic response of organic semiconductors requires a thorough understanding of the fundamental light-matter interaction that is dominated by the excitation of correlated electron-hole pairs, i.e. excitons. The nature…

The extension of nonlinear spectroscopic techniques into the x-ray domain is in its infancy but holds the promise to provide unique insight into the dynamics of charges in photoexcited processes, which are of fundamental as well as applied…

Excitons, Coulomb-bound electron-hole pairs, are the fundamental excitations governing the optoelectronic properties of semiconductors. While optical signatures of excitons have been studied extensively, experimental access to the excitonic…

The structure appearance in exciton density distribution in semiconductor double quantum well with transverse electric field applied is studied, in the case when the metal electrode contains a round window. It is suggested that there is…

Mesoscale and Nanoscale Physics · Physics 2007-05-23 A. A. Chernyuk , V. S. Kopp , V. I. Sugakov

Time-resolved soft-X-ray photoemission spectroscopy is used to simultaneously measure the ultrafast dynamics of core-level spectral functions and excited states upon excitation of excitons in WSe$_2$. We present a many-body approximation…

Core-excitations on different atoms are highly localized and therefore decoupled. By placing molecules in an X-ray cavity the core-transitions become coupled via the exchange of cavity photons and form delocalized hybrid light-matter…

Quantum Physics · Physics 2021-02-08 Bing Gu , Artur Nenov , Francesco Segatta , Marco Garavelli , Shaul Mukamel

The energy spectrum of a two-dimensional electron gas (2DEG) interacting with a valence-band hole is studied in the high magnetic field limit as a function of the filling factor nu and the separation d between the electron and hole layers.…

Mesoscale and Nanoscale Physics · Physics 2009-10-31 Arkadiusz Wojs , Kyung-Soo Yi , John J. Quinn

Non-collinear four-wave mixing (FWM) techniques at near-infrared (NIR), visible, and ultraviolet frequencies have been widely used to map vibrational and electronic couplings, typically in complex molecules. However, correlations between…