Related papers: Nonlinear light scattering in molecules triggered …
In nonlinear Thomson scattering, a relativistic electron reflects and re-radiates the photons of a laser pulse, converting optical light to x rays or beyond. While this extreme frequency conversion offers a promising source for probing…
Conventional nonlinear spectroscopy uses classical light to detect matter properties through the variation of its response with frequencies or time delays. Quantum light opens up new avenues for spectroscopy by utilizing parameters of the…
We study coherent backscattering of a monochromatic laser by a dilute gas of cold two-level atoms in the weakly nonlinear regime. The nonlinear response of the atoms results in a modification of both the average field propagation (nonlinear…
We examine x-ray scattering from an isolated organic molecule from the linear to nonlinear absorptiveregime. In the nonlinear regime, we explore the importance of both the elastic and inelastic channelsand observe the onset of nonlinear…
Optical signals obtained by the material response to classical laser fields are given by nonlinear response functions which can be expressed by sums over various quantum pathways of matter. We show that some pathways can be selected by…
This paper theoretically treats the spontaneous resonant inelastic scattering of Laguerre-Gauss (LG) beams from the totally symmetric vibrations of complex polyatomic molecules within the semi-classical framework. We develop an interaction…
Effects of nonlinearity in Thomson scattering of a high intensity laser pulse from electrons are analyzed. Analytic expressions for laser pulse shaping in amplitude and frequency are obtained which control spectrum broadening for…
The rotational dynamics of particles subject to external illumination is found to produce light amplification and inelastic scattering at high rotation velocities. Light emission at frequencies shifted with respect to the incident light by…
We study coherent backscattering of a quasi-monochromatic laser by a dilute gas of cold two-level atoms. We consider the perturbative regime of weak intensities, where nonlinear effects arise from {\em inelastic} two-photon scattering…
Accelerated charges emit electromagnetic radiation and the consequent energy-momentum loss alters their trajectory. This phenomenon is known as radiation reaction and the Landau-Lifshitz (LL) equation is the classical equation of motion of…
We study theoretically the quantum dynamics of nitrogen molecules (N$_2$) exposed to intense and ultrafast x-rays at a wavelength of 1.1 nm (1100 eV photon energy) from the Linac Coherent Light Source (LCLS) free electron laser. Molecular…
Nonlinear radio waves modulate the plasma, scatter on the modulations, and develop an intermittent power spectrum -- perhaps. Rudiments of theory, numerical simulations, and qualitative modeling of nonlinear scattering are presented.…
We study the resonance fluorescence properties of an optically active spin 1/2 system, elucidating the effects of a magnetic field on the coherence of the scattered light. We derive a master equation model for this system that reproduces…
Raman spectroscopy uses light scattering to extract information on low-energy excitations of solids. The Raman process is described by diagrams which are fourth order in the light-matter interaction, and in particular the resonant…
The influence of the laser pulse temporal shape on the Nonlinear Thomson Scattering on-axis photon spectrum is analyzed in detail. Using the classical description, analytical expressions for the temporal and spectral structure of the…
An optical four-level atomic discrete system through optical induction is proposed. A theoretical scheme to produce nonclassical lattice solitons (NLS) in the system is presented with the use of the effects of enhanced self-phase modulation…
Propagation of light in a highly scattering medium is among the most fascinating optical effect that everyone experiences on an everyday basis and possesses a number of fundamental problems which have yet to be solved. Conventional wisdom…
A century ago, J. J. Thomson showed that the scattering of low-intensity light by electrons was a linear process (i.e., the scattered light frequency was identical to that of the incident light) and that light's magnetic field played no…
Nonresonant inelastic light and X-ray scattering is investigated for the spinless Falicov-Kimball model on an infinite-dimensional hypercubic lattice with a charge-density-wave phase at half filling. The many-body density of states (DOS) is…
Inelastic light scattering from electrons is a symmetry-selective probe of the charge dynamics within correlated materials. Many measurements have been made on correlated insulators, and recent exact solutions in large dimensions explain a…