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We report on the optical spectroscopy of the spin of two magnetic atoms (Mn) embedded in an individual quantum dot interacting with either a single electron, a single exciton and single trion. As a result of their interaction to a common…

Mesoscale and Nanoscale Physics · Physics 2015-06-05 L. Besombes , C. L. Cao , S. Jamet , H. Boukari , J. Fernandez-Rossier

We report on the observation of spin dependent optically dressed states and optical Stark effect on an individual Mn spin in a semiconductor quantum dot. The vacuum-to-exciton or the exciton-to-biexciton transitions in a Mn-doped quantum…

Mesoscale and Nanoscale Physics · Physics 2012-06-18 C. Le Gall , A. Brunetti , H. Boukari , L. Besombes

We analyze the spin dynamics of an individual magnetic atom (Mn) inserted in a II-VI semiconductor quantum dot under resonant optical excitation. In addition to standard optical pumping expected for a resonant excitation, we show that for…

Mesoscale and Nanoscale Physics · Physics 2015-06-15 S. Jamet , H. Boukari , L. Besombes

In order to explain the recently observed phenomenon of optical orientation of a single Mn spin residing inside a quantum dot, a process of Mn spin relaxation with characteristic timescale of tens of nanoseconds had been invoked. We show…

Mesoscale and Nanoscale Physics · Physics 2010-08-24 Lukasz Cywinski

Using the emission of the positively charged exciton as a probe, we analyze the dynamics of the optical pumping and the dynamics of the relaxation of a Mn spin exchange-coupled with a confined hole spin in a II-VI semiconductor quantum dot.…

Mesoscale and Nanoscale Physics · Physics 2015-06-22 B. Varghese , H. Boukari , L. Besombes

A system of two coupled CdTe quantum dots, one of them containing a single Mn ion, was studied in continuous wave and modulated photoluminescence, photoluminescence excitation, and photon correlation experiments. Optical writing of…

Other Condensed Matter · Physics 2011-01-13 M. Goryca , T. Kazimierczuk , M. Nawrocki , A. Golnik , J. A. Gaj , P. Kossacki , P. Wojnar , G. Karczewski

For future quantum technologies the combination of a long quantum state lifetime and an efficient interface with external optical excitation are required. In solids, the former is for example achieved by individual spins, while the latter…

When a detuned and strong laser pulse acts on an optical transition, a Stark shift of the corresponding energies occurs. We analyze how this optical Stark effect can be used to prepare and control the dark exciton occupation in a…

We report on the coherent dynamics of the spin of an individual magnetic atom coupled to carriers in a semiconductor quantum dot which has been investigated by resonant photoluminescence of the positively charged exciton (X+). We…

Mesoscale and Nanoscale Physics · Physics 2015-09-02 A. Lafuente-Sampietro , H. Boukari , L. Besombes

The ability to discriminate between simultaneously occurring noise sources in the local environment of semiconductor InGaAs quantum dots, such as electric and magnetic field fluctuations, is key to understanding their respective dynamics…

Mesoscale and Nanoscale Physics · Physics 2014-11-18 Megan J. Stanley , Clemens Matthiesen , Jack Hansom , Claire Le Gall , Carsten H. H. Schulte , Edmund Clarke , Mete Atatüre

This study explores the optical properties of quantum dots doped with a Ni$^{2+}$ ion that interacts with a charged exciton. Systematic magneto-optical analysis reveals that the strain distribution at the Ni$^{2+}$ site significantly…

Mesoscale and Nanoscale Physics · Physics 2025-08-21 K. E. Polczynska , S. Karouaz , W. Pacuski , L. Besombes

A Cr atom in a semiconductor host carries a localized spin with an intrinsic large spin to strain coupling particularly promising for the development of hybrid spin-mechanical systems and coherent mechanical spin driving. We demonstrate…

Mesoscale and Nanoscale Physics · Physics 2017-02-01 A. Lafuente-Sampietro , H. Utsumi , H. Boukari , S. Kuroda , L. Besombes

A hight degree of spin polarization is achieved for a Mn atom localized in a semiconductor quantum dot using quasi-resonant optical excitation at zero magnetic field. Optically created spin polarized carriers generate an energy splitting of…

Other Condensed Matter · Physics 2012-06-18 C. Le Gall , L. Besombes , H. Boukari , R. Kolodka , H. Mariette , J. Cibert

We investigate the effect of spin-orbit interaction on the intra- and interdot particle dynamics of a double quantum dot under ac electric fields. The former is modeled as an effective ac magnetic field that produces electric-dipole spin…

Mesoscale and Nanoscale Physics · Physics 2023-05-10 David Fernández-Fernández , Jordi Picó-Cortés , Sergio Vela Liñán , Gloria Platero

We have investigated the spin preparation efficiency by optical pumping of individual Mn atoms embedded in CdTe/ZnTe quantum dots. Monitoring the time dependence of the intensity of the fluorescence during the resonant optical pumping…

Mesoscale and Nanoscale Physics · Physics 2012-06-18 C. Le Gall , R. S. Kolodka , C. Cao , H. Boukari , H. Mariette , J. Fernández-Rossier , L. Besombes

We present the results of a comprehensive magneto-optical characterization of single CdTe quantum dots containing a few Mn2+ ions. We find that some quantum dots exhibit an unexpected evolution of excitonic photoluminescence spectrum with…

Mesoscale and Nanoscale Physics · Physics 2017-01-04 Maciej Koperski , Tomasz Smoleński , Mateusz Goryca , Piotr Wojnar , Marek Potemski , Piotr Kossacki

The spin-flip rate that couples dark and bright excitons in self-assembled quantum dots is obtained from time-resolved spontaneous emission measurements in a modified local density of optical states. Employing this technique, we can…

Other Condensed Matter · Physics 2010-03-18 Jeppe Johansen , Brian Julsgaard , Søren Stobbe , Jørn M. Hvam , Peter Lodahl

A photo-excited II-VI semiconductor nanocrystal doped with a few Mn spins is considered. The effects of spin-exciton interactions and the resulting multi-spin correlations on the photoluminescence are calculated by numerical diagonalization…

Mesoscale and Nanoscale Physics · Physics 2009-11-11 J. Fernández-Rossier

We show how a spin interaction between electrons localized in neighboring quantum dots can be induced and controlled optically. The coupling is generated via virtual excitation of delocalized excitons and provides an efficient coherent…

Condensed Matter · Physics 2009-11-07 C. Piermarocchi , Pochung Chen , L. J. Sham , D. G. Steel

We studied the spin dynamics of a Cr atom incorporated in a II-VI semiconductor quantum dot using photon correlation techniques. We used recently developed singly Cr-doped CdTe/ZnTe quantum dots (A. Lafuente-Sampietro {\it et al.}, [1]) to…

Mesoscale and Nanoscale Physics · Physics 2016-08-24 A. Lafuente-Sampietro , H. Utsumi , H. Boukari , S. Kuroda , L. Besombes
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