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Recently developed quantum mechanical theory of inelastic He atom scattering (HAS) from solid surfaces is employed to analyze the energy transfer between projectile particles (thermal energy He-atoms) and vibrational degrees of freedom…

Statistical Mechanics · Physics 2007-05-23 A. Siber , B. Gumhalter , J. P. Toennies

The wave function of an atom passed through a diffraction grating acquires a regular space structure and the interaction of another particle with this atom can be thought of as scattering on a 'quantum grating' composed of a single atom.…

Quantum Physics · Physics 2020-02-24 S. F. Zhang , B. Najjari , X. Ma , A. B. Voitkiv

We here report coherent reflection of thermal He atom beams from various microscopically rough surfaces at grazing incidence. For a sufficiently small normal component $k_z$ of the incident wave-vector of the atom the reflection probability…

Atomic Physics · Physics 2010-09-28 Bum Suk Zhao , H. Christian Schewe , Gerard Meijer , Wieland Schöllkopf

Diffraction of atoms from surfaces provides detailed insights into structures, interactions, and dynamical processes. However, currently the method is limited to measurements in reflection - diffraction through materials has only been…

The diffraction of fast atoms at crystal surfaces is ideal for a detailed investigation of the surface electronic density. However, instead of sharp diffraction spots, most experiments show elongated streaks characteristic of inelastic…

Atomic Physics · Physics 2017-08-02 Philippe Roncin , Maxime Debiossac

The diffraction of fast atoms at grazing incidence on crystal surfaces (GIFAD) was first interpreted only in terms of elastic diffraction from a perfectly periodic rigid surface with atoms fixed at equilibrium position. Recently, a new…

Materials Science · Physics 2022-09-23 Philippe Roncin , Maxime Debiossac , Hanene Oueslati , Fayçal Raouafi

Quantum reflection is a universal property of atoms and molecules when scattered from surfaces in ultracold collisions. Recent experimental work has documented the quantum reflection and diffraction of He atoms, dimers, trimers and Neon…

Quantum Physics · Physics 2018-12-12 G. Rojas-Lorenzo , J. Rubayo-Soneira , S. Miret-Artés , E. Pollak

The Sudden Approximation (SA) for scattering of atoms from surfaces is generalized to allow for double collision events and scattering from time-dependent quantum liquid surfaces. The resulting new schemes retain the simplicity of the…

Materials Science · Physics 2015-06-25 Daniel A. Lidar

We have applied small angle scattering in grazing incidence beam geometry on a time-of-flight neutron instrument. Due to the broad wavelength distribution provided for a specific incident beam angle the penetration depth of the neutron beam…

Soft Condensed Matter · Physics 2020-06-09 Max Wolff , Peter Kuhns , Andrew J C Dennison , Georg Liesche , Philipp Gutfreund , Sarah Rogers

We develop a versatile theoretical approach to the study of cold-atom diffractive scattering from light-field gratings by combining calculations of the optical near-field, generated by evanescent waves close to the surface of periodic…

Atomic Physics · Physics 2009-11-07 G. Leveque , C. Meier , R. Mathevet , C. Robiliiard , J. Weiner , C. Girard , J. C. Weeber

Recent measurements of the scattering of He and Ne atoms at Rh(110) suggest that these two rare-gas atoms measure a qualitatively different surface corrugation: While Ne atom scattering seemingly reflects the electron-density undulation of…

Grazing incidence X-ray scattering experiments are designed to achieve strong scattering signals from materials, such as molecular monolayers, island films, or thin films that are localized to the surfaces of flat substrates. Optimal…

Instrumentation and Detectors · Physics 2025-07-01 Edward Tortorici , Charles T. Rogers

The activated surface diffusion of interacting adsorbates is described in terms of the so-called interacting single adsorbate approximation, which is applied to the diffusion of Na atoms on Cu(001) for coverages up to 20% in quasielastic He…

Statistical Mechanics · Physics 2008-03-11 R. Martinez-Casado , J. L. Vega , A. S. Sanz , S. Miret-Artes

Using density-functional theory we compute the energy barriers and attempt frequencies for surface diffusion of Ag on Ag(111) with different lattice constants, and on an Ag adsorbate monolayer on Pt(111). We find that the attempt frequency…

Condensed Matter · Physics 2009-10-31 C. Ratsch , M. Scheffler

We review recent theoretical models and experiments dealing with the diffraction of neutral atoms from a reflection grating, formed by a standing evanescent wave. We analyze diffraction mechanisms proposed for normal and grazing incidence,…

Six-dimensional quantum dynamical calculations of the scattering of H_2 from a Pd(100) surface using a potential energy surface derived from density-functional theory calculations are presented. Due to the corrugation and anisotropy of the…

mtrl-th · Physics 2009-10-30 Axel Gross , Matthias Scheffler

We report fast atom diffraction through single-layer graphene using hydrogen atoms at kinetic energies from 150 to 1200 eV. High-resolution images reveal overlapping hexagonal patterns from coexisting monocrystalline domains. Time-of-flight…

Grazing incidence interferometry has been applied to rough planar and cylindrical surfaces. As suitable beam splitters diffractive optical phase elements are quite common because these allow for the same test sensitivity for all surface…

To describe the grazing scattering of keV atoms at surface, a new quantum binary collision model have been proposed where the dynamical properties of the surface atoms are considered via the wave-function of the local Debye harmonic…

Atomic Physics · Physics 2018-07-25 Philippe Roncin , Maxime Debiossac

Projected momentum distributions of electrons, i.e. Compton profiles above the topmost atomic layer have recently become experimentally accessible by kinetic electron emission in grazing-incidence scattering of atoms at atomically flat…

Other Condensed Matter · Physics 2009-11-11 Christoph Lemell , Andres Arnau , Joachim Burgdörfer