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X-ray free-electron lasers (XFELs) as the world's brightest light sources provide ultrashort X-ray pulses with a duration typically in the order of femtoseconds. Recently, they have approached and entered the attosecond regime, which holds…

Bright ultrashort X-ray pulses allow scientists to observe ultrafast motion of atoms and molecules. Coherent light sources, such as the X-ray free electron laser (XFEL), enable remarkable discoveries in cell biology, protein…

We demonstrate the ability to control and shape the spectro-temporal content of extreme-ultraviolet (XUV) pulses produced by a seeded free-electron laser (FEL). The control over the spectro-temporal properties of XUV light was achieved by…

High-intensity, ultrashort, fully coherent X-ray pulses hold great potential for advancing spectroscopic techniques to unprecedented levels. Here, we propose a novel scheme for generating high-brightness and femtosecond-scale soft X-ray…

Accelerator Physics · Physics 2023-06-30 Hanxiang Yang , Jiawei Yan , Haixiao Deng

Accelerator-based X-ray free-electron lasers (XFELs) are the latest addition to the revolutionary tools of discovery for the 21st century. The two major components of an XFEL are an accelerator-produced electron beam and a magnetic…

The advent of isolated and intense sub-femtosecond X-ray pulses enables tracking of quantummechanical motion of electrons in molecules and solids. The combination of X-ray spectroscopy and diffraction imaging is a powerful approach to…

Accelerator-based light sources such as storage rings and free-electron lasers use relativistic electron beams to produce intense radiation over a wide spectral range for fundamental research in physics, chemistry, materials science,…

Accelerator Physics · Physics 2015-06-19 Erik Hemsing , Gennady Stupakov , Dao Xiang , Alexander Zholents

The coupling of laser light to matter can exert sub-cycle coherent control over material properties, with optically induced currents and magnetism shown to be controllable on ultrafast femtosecond time scales. Here, by employing laser light…

Optics · Physics 2024-06-19 Q. Z. Li , S. Shallcross , J. K. Dewhurst , S. Sharma , P. Elliott

Oscillators are at the heart of optical lasers, providing stable transform limited pulses. In contrast, X-ray free electron lasers use self-amplified spontaneous emission (SASE), resulting in large stochastic intensity and spectral…

Accelerator Physics · Physics 2020-02-13 A. Halavanau , A. Benediktovitch , A. A. Lutman , D. DePonte , D. Cocco , N. Rohringer , U. Bergmann , C. Pellegrini

Sub-angstrom spatial resolution of electron density coupled with sub-femtosecond temporal resolution is required to directly observe the dynamics of the electronic structure of a molecule after photoinitiation or some other ultrafast…

Coherent control of quantum dynamics is key to a multitude of fundamental studies and applications alike. In the visible or longer-wavelength domains, near-resonant light fields have become the primary tool to control electron dynamics.…

We investigate the coherent control of the photo\-electron angular distribution in bichromatic atomic ionization. Neon is selected as target since it is one of the most popular systems in current gas-phase experiments with free-electron…

Atomic Physics · Physics 2018-01-31 E. V. Gryzlova , A. N. Grum-Grzhimailo , E. I. Staroselskaya , N. Douguet , K. Bartschat

X-ray beams carrying orbital angular momentum (OAM) are an emerging tool for probing matter. Optical elements, such as spiral phase plates and zone plates, have been widely used to generate OAM light. However, these optics are challenging…

Accelerator Physics · Physics 2022-08-22 Jiawei Yan , Gianluca Geloni

Over the last few years, tremendous progress has been gained in the generation and application of ultrashort radiation pulses. Recently, free-electron lasers generating ultrashort pulses with high peak power from the extreme ultraviolet…

Accelerator Physics · Physics 2023-06-21 Najmeh Mirian

With their brilliance and temporal structure, X-ray free-electron laser can unveil atomic-scale details of ultrafast phenomena. Recent progress in split-and-delay optics (SDO), which produces two X-ray pulses with time-delays, offers bright…

We propose a technique for the production of attosecond X-ray pulses which is based on the use of X-ray SASE FEL combined with a femtosecond laser system. A few-cycle optical pulse from a Ti:sapphire laser interacts with the electron beam…

Accelerator Physics · Physics 2009-11-10 E. L. Saldin , E. A. Schneidmiller , M. V. Yurkov

The ability to arbitrarily dial in amplitudes and phases enables the fundamental quantum state operations pioneered for microwaves and then infrared and visible wavelengths during the second half of the last century. Self-seeded X-ray…

Singly ionized nitrogen molecules in ambient air pumped by near-infrared femtosecond laser give rise to superradiant emission. Here we demonstrate coherent control of this superradiance by injecting a pair of resonant seeding pulses inside…

The features of Betatron x-ray emission produced in a laser-plasma accelerator are closely linked to the properties of the relativistic electrons which are at the origin of the radiation. While in interaction regimes explored previously the…

Plasma Physics · Physics 2011-12-20 S. Corde , K. Ta Phuoc , R. Fitour , J. Faure , A. Tafzi , J. P. Goddet , V. Malka , A. Rousse

High-intensity X-ray sources are essential diagnostic tools for science, technology and medicine. Such X-ray sources can be produced in laser-plasma accelerators, where electrons emit short-wavelength radiation due to their betatron…

Plasma Physics · Physics 2022-03-16 Vojtěch Horný , Miroslav Krůs , Tünde Fülop