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We lay the foundation for determining the microscopic spin interactions in two-dimensional (2D) ferromagnets by combining angle-dependent ferromagnetic resonance (FMR) experiments on high quality CrI$_3$ single crystals with theoretical…

The electronic and magnetic properties of transition metal oxyhalide compound Co2TeO3Cl2 is investigated using first principle calculations within the framework of density functional theory. In order to find underlying spin lattice of this…

Materials Science · Physics 2017-09-13 Jayita Chakraborty

A comparative resonant inelastic x-ray scattering (RIXS) study of three well-known Kitaev materials is presented: $\alpha$-Li$_2$IrO$_3$, Na$_2$IrO$_3$, and $\alpha$-RuCl$_3$. Despite similar low-energy physics, these materials show…

We present a detailed study of the magnetic structure and spin waves in the Fe jarosite compound ${\rm KFe_3(SO_4)_2(OH)_6}$ for the most general Hamiltonian involving one- and two-spin interactions which are allowed by symmetry. We compare…

Materials Science · Physics 2009-11-11 T. Yildirim , A. B. Harris

While the ground state of magnetic materials is in general well described on the basis of spin density functional theory (SDFT), the theoretical description of finite-temperature and non-equilibrium properties require an extension beyond…

Materials Science · Physics 2022-06-22 Sergiy Mankovsky , Hubert Ebert

Given that energy scales associated with crystal field splitting, spin orbit coupling and coulomb correlations in iridates are comparable, hence leading to exotic properties, we investigate the physical properties of orthorhombic SrIrO3…

Materials Science · Physics 2015-07-23 Vijeta Singh , J. J. Pulikkotil

First-principles calculations and simulations are conducted to clarify the nonmagnetic insulating ground state of the honeycomb lattice compound Na2RuO3 with 4d^4 electronic configuration and explore the evolutions of crystal structure and…

Strongly Correlated Electrons · Physics 2023-02-14 Xujia Gong , Wei Wang , Wen Lei , Feng Xiao , Carmine Autieri , Congling Yin , Xing Ming

Electron correlation strength is predicted to be weak in 5d transition metal oxides and hence, various anomalous electronic properties observed in these systems are often attributed to the large spin-orbit interaction strength. Employing…

Strongly Correlated Electrons · Physics 2009-07-17 Kalobaran Maiti

We report the optical and magneto-optical properties of K2V3O8, an S=1/2 quasi-two-dimensional Heisenberg antiferromagnet. Local spin density approximation electronic structure calculations are used to assign the observed excitations and…

Strongly Correlated Electrons · Physics 2009-11-11 R. C. Rai , J. Cao , J. L. Musfeldt , D. J. Singh , R. Jin , Z. X. Zhou , B. C. Sales , D. Mandrus , X. Wei

KTaO$_3$ (KTO) is an incipient ferroelectric, characterized by a softening of the lowest transverse optical (TO) mode with decreasing temperature. Cooper pairing in the recently discovered KTO-based heterostructures has been proposed to be…

Materials Science · Physics 2026-01-29 Giulia Venditti , Francesco Macheda , Paolo Barone , José Lorenzana , Maria N. Gastiasoro

Magnetic order and the underlying magnetic model of the multiferroic pyroxene NaFeGe2O6 are systematically investigated by neutron powder diffraction, thermodynamic measurements, density-functional bandstructure calculations, and…

Strongly Correlated Electrons · Physics 2018-09-19 Lei Ding , Pascal Manuel , Dmitry D. Khalyavin , Fabio Orlandi , Alexander A. Tsirlin

We report on microscopic tight-binding modeling of surface states in Bi$_2$Se$_3$ three-dimensional topological insulator, based on a sp$^3$ Slater-Koster Hamiltonian, with parameters calculated from density functional theory. The effect of…

Mesoscale and Nanoscale Physics · Physics 2014-11-04 A. Pertsova , C. M. Canali

Magnetic properties of the spin-3/2 Heisenberg system Cr2BP3O12 are investigated by magnetic susceptibility chi(T) measurements, electron spin resonance, neutron diffraction, and density functional theory (DFT) calculations, as well as…

Strongly Correlated Electrons · Physics 2013-02-25 O. Janson , S. Chen , A. A. Tsirlin , S. Hoffmann , J. Sichelschmidt , Q. Huang , Z. -J. Zhang , M. -B. Tang , J. -T. Zhao , R. Kniep , H. Rosner

Heterostructures made of transition metal oxides are new tailor-made materials which are attracting much attention. We have constructed a 6-band k.p Hamiltonian and used it within the envelope function method to calculate the subband…

Mesoscale and Nanoscale Physics · Physics 2014-01-09 L. W. van Heeringen , G. A. de Wijs , A. McCollam , J. C. Maan , A. Fasolino

We review recent theoretical developments about the role of spins, electron-electron interactions, and spin-orbit coupling in metal nanoparticles and semiconductor quantum dots. For a closed system, in the absence of spin-orbit coupling or…

Mesoscale and Nanoscale Physics · Physics 2007-05-23 Yuval Oreg , P. W. Brouwer , X. Waintal , Bertrand I. Halperin

The magnetic field response of the Mott-insulating honeycomb iridate Na$_{2}$IrO$_{3}$ is investigated using torque magnetometry measurements in magnetic fields up to 60 tesla. A peak-dip structure is observed in the torque response at…

We address the concomitant metal-insulator transition (MIT) and antiferromagnetic ordering in the novel pyrochlore iridate Eu2Ir2O7 by combining x-ray absorption spectroscopy, x-ray and neutron diffractions and density functional theory…

We present a technique to map an electronic model with local interactions (a generalized multi-orbital Hubbard model) onto an effective model of interacting classical spins, by requiring that the thermodynamic potentials associated to spin…

Strongly Correlated Electrons · Physics 2015-05-27 Andrea Secchi , Alexander I. Lichtenstein , Mikhail I. Katsnelson

The calculations of electronic transport coefficients and optical properties require a very dense interpolation of the electronic band structure in reciprocal space that is computationally expensive and may have issues with band crossing…

Thermomagnetic and inelastic neutron scattering measurements on Na2PrO3 are reported. This material is an antiferromagnetic honeycomb magnet based on the tetravalent lanthanide Pr4+ and has been proposed to host dominant antiferromagnetic…

Strongly Correlated Electrons · Physics 2021-03-17 Marcus J. Daum , Arun Ramanathan , Alexander I. Kolesnikov , Stuart A. Calder , Martin Mourigal , Henry S. La Pierre