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We experimentally disentangle the contributions of different quantum paths in high-order harmonic generation (HHG) from the spectrally and spatially resolved harmonic spectra. By adjusting the laser intensity and focusing position, we…

Atomic Physics · Physics 2015-10-08 Lixin He , Pengfei Lan , Qingbin Zhang , Chunyang Zhai , Feng Wang , Wenjing Shi , Peixiang Lu

The optical phase of the driving field in the process of high harmonic generation and the coherence properties of the harmonics are fundamental concepts in attosecond physics. Here, we consider to drive the process by incoherent classical…

Quantum Physics · Physics 2024-09-16 Philipp Stammer

We generate high-order harmonics in gaseous medium with tunable photon energy using time domain interferometry of double pulses in a non-collinear generation geometry. The method is based on the fact that the generated harmonics inherit…

Accurate molecular imaging via high-order harmonic generation relies on comparing the harmonic emission from a molecule and an adequate reference system. However, an ideal reference atom with the same ionization properties as the molecule…

Atomic Physics · Physics 2015-05-28 Elmar V. van der Zwan , Manfred Lein

It is shown that under optimal conditions, the generation of the 3rd, 5th, 7th, and 9th harmonics of the short-wave, ultraviolet or vacuum ultraviolet, laser field by helium atoms is mainly due to transitions between bound states, and the…

High-harmonic generation (HHG) in solids has typically been explored in transparent dielectrics and semiconductors. Metals have long been dismissed due to their strong reflectivity at infrared wavelengths. Here, we demonstrate HHG from…

We analyze third-harmonic generation from high-index dielectric nanoparticles and discuss the basic features and multipolar nature of the parametrically generated electromagnetic fields near the Mie-type optical resonances. By combining…

High-harmonic generation (HHG) involves the up-conversion of a high-intensity driving field into its harmonic orders. This process is intrinsically non-classical, requiring from quantum mechanics for a complete explanation as, under…

Quantum Physics · Physics 2024-09-25 Javier Rivera-Dean

We apply the theory of high-order harmonic generation by low-frequency laser fields in the strong field approximation to the study of the spatial and temporal coherence properties of the harmonics. We discuss the role of dynamically induced…

Quantum Physics · Physics 2007-05-23 Pascal Salières , Anne L'Huillier , Philippe Antoine , Maciej Lewenstein

We show that spatially structured radiation generates second harmonic in a two-dimensional system even if the system is homogeneous and isotropic. The effect originates from non-locality of electric response to structured electromagnetic…

Mesoscale and Nanoscale Physics · Physics 2025-04-23 A. A. Gunyaga , M. V. Durnev , S. A. Tarasenko

Layered NbOX$_2$ ($X=\mathrm{Cl,\,Br,\,I}$), a member of the van der Waals ferroelectric family, exhibits intrinsic ferroelectricity and pronounced nonlinear optical responses, making it a promising candidate for integrated nanophotonics…

We investigated the giant resonance in Xenon by high-order harmonic generation spectroscopy driven by a two-color field. The addition of a non-perturbative second harmonic component parallel to the driving field breaks the symmetry between…

High-harmonic generation in solids allows probing and controlling electron dynamics in crystals on few femtosecond timescales, paving the way to lightwave electronics. In the spatial domain, recent advances in the real-space interpretation…

We present theoretical studies of high-order harmonic generation (HHG) driven by plasmonic fields in two-electron atomic systems. Comparing the two-active electron and single-active electron approximation models of the negative hydrogen ion…

Atomic Physics · Physics 2016-11-03 A. Chacón , M. F. Ciappina , M. Lewenstein

Using numerical simulations, we show that atomic high order harmonic generation, HHG, with a circularly polarized laser field offers an ideal framework for quantum-classical correspondence in strong field physics. With an appropriate…

Atomic Physics · Physics 2014-02-06 Francois Mauger , A. D. Bandrauk , Adam Kamor , Turgay Uzer , Cristel Chandre

It is well known that when two types of perturbations interact in cosmological perturbation theory, the interaction may lead to the generation of a third type. In this article we discuss the generation of magnetic fields from such…

General Relativity and Quantum Cosmology · Physics 2014-03-24 Bob Osano

High harmonic generation in benzene is studied using a mixed quantum-classical approach in which the electrons are described using time-dependent density functional theory while the ions move classically. The interaction with both…

Atomic Physics · Physics 2016-03-02 Abigail Wardlow , Daniel Dundas

The interaction of intense mid-infrared laser fields with atoms and molecules leads to a range of new opportunities, from the production of bright, coherent radiation in the soft x-ray range to imaging molecular structures and dynamics with…

We extend a model of two-center interference to include the superposition of opposite orientations in aligned polar molecules. We show that the position of the minimum in the harmonic spectrum from both aligned and oriented CO depends…

Atomic Physics · Physics 2011-09-07 Adam Etches , Mette B. Gaarde , Lars Bojer Madsen

A quantum optical model for the high-order harmonic generation is presented, in which both the exciting field and the high harmonic modes are quantized, while the target material appears via parameters only. As a consequence, the model is…