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Related papers: Magnetisation process in Er2Ti2O7 and Tb2Ti2O7 at …

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The pyrochlore insulator Yb2Ti2O7 has attracted the attention of experimentalists and theoreticians alike for about 15 years. Conflicting neutron diffraction data on the possible existence of magnetic Bragg reflections at low temperature…

Strongly Correlated Electrons · Physics 2016-08-26 A. Yaouanc , P. Dalmas de Reotier , L. Keller , B. Roessli , A. Forget

The XY pyrochlore Yb$_2$Ti$_2$O$_7$, with pseudo spin 1/2 at the Yb$^{3+}$ site, has been celebrated as potential host for the quantum spin ice state. The substitution of non-magnetic Ti with Pt gives Yb$_2$Pt$_2$O$_7$, a system with…

Strongly Correlated Electrons · Physics 2018-10-03 S. K. Takahashi , A. Arsenault , C. Mauws , A. M. Hallas , C. Sarkis , K. A. Ross , C. R. Wiebe , M. Tachibana , G. M. Luke , T. Imai

In frustrated magnetic systems, geometric constraints or the competition amongst interactions introduce extremely high degeneracy and prevent the system from readily selecting a low-temperature ground state. The most frustrated known spin…

Strongly Correlated Electrons · Physics 2016-11-23 Darren C. Peets , Hasung Sim , Maxim Avdeev , Je-Geun Park

The quantum spin ice model applied to Tb2Ti2O7 predicts that magnetic fields applied along the [111] axis will induce a partial magnetization plateau [H. R. Molavian and M. J. P. Gingras, J. Phys.: Condens. Matter 21, 172201 (2009)]. We…

Strongly Correlated Electrons · Physics 2011-05-12 P. J. Baker , M. J. Matthews , S. R. Giblin , P. Schiffer , C. Baines , D. Prabhakaran

We derive an effective spin-1/2 exchange model for non-Kramers Tb$^{3+}$ states in the pyrochlore Tb$_2$Ti$_2$O$_7$. The four anisotropic nearest-neighbour exchange constants, as well as next-neighbour exchange constants are derived for the…

Strongly Correlated Electrons · Physics 2014-12-02 S. P. Mukherjee , S. H. Curnoe

Reliable and profound studies of actual magnetic domain structure in rare-earth A2Ir2O7 pyrochlore iridates are frequently limited by insufficient sample quality or lack of single crystals. We report the magnetic properties of the…

The pyrochlore compounds Ho2Ti2O7 and Dy2Ti2O7 show an exotic form of magnetism called the spin ice state, resulting from the interplay between geometrical frustration and ferromagnetic coupling. A fascinating feature of this state is the…

Materials Science · Physics 2013-09-11 D. P. Leusink , F. Coneri , M. Hoek , S. Turner , H. Idrissi , G. Van Tendeloo , H. Hilgenkamp

Electron spin resonance study of frustrated pyrochlore Gd2Ti2O7 is performed in a wide frequency band for a temperature range 0.4-30 K, which covers paramagnetic and magnetically ordered phases. The paramagnetic resonance reveals the…

Strongly Correlated Electrons · Physics 2012-02-02 S. S. Sosin , A. I. Smirnov , L. A. Prozorova , G. Balakrishnan , M. E. Zhitomirsky

The ground state of the quantum spin ice candidate magnet Yb2Ti2O7 is known to be sensitive to weak disorder at the 1 percent level which occurs in single crystals grown from the melt. Powders produced by solid state synthesis tend to be…

Strongly Correlated Electrons · Physics 2016-03-09 J. Gaudet , K. A. Ross , E. Kermarrec , N. P. Butch , G. Ehlers , H. A. Dabkowska , B. D. Gaulin

Pyrochlore erbium titanate samples in the form of powders (with nominal compositions of Er2Ti2+xO7) and bulk single crystals were prepared to elucidate the effect of synthesis and growth conditions on their composition, structure, and…

Materials Science · Physics 2018-12-14 Q. Wang , A. Ghasemi , A. Scheie , S. M. Koohpayeh

Dy$_{2}$Zr$_{2}$O$_{7}$ a disordered pyrochlore system, exhibits the spin ice freezing under the application of magnetic field. Our studies suggest the stabilization of pyrochlore phase in Dy$_{2-x}$La$_{x}$Zr$_{2}$O$_{7}$ with the…

Strongly Correlated Electrons · Physics 2021-10-12 Sheetal , C. S. Yadav

A spin-ice compound dysprosium titanate, Dy2Ti2O7, is studied by specific heat measurements in magnetic fields applied along the [110] direction of the cubic unit cell. Above a magnetic field of 0.4 T a relatively sharp peak at T = 1.1 K in…

Materials Science · Physics 2009-11-10 Zenji Hiroi , Kazuyuki Matsuhira , Masao Ogata

The XY pyrochlore antiferromagnet Er$_2$Ti$_2$O$_7$ exhibits a rare case of $Z_6$ discrete symmetry breaking in its $\psi_2$ magnetic ground state. Despite being well-studied theoretically, systems with high discrete symmetry breakings are…

Strongly Correlated Electrons · Physics 2017-02-15 J. Gaudet , A. M. Hallas , J. Thibault , N. P. Butch , H. A. Dabkowska , B. D. Gaulin

We have studied the low energy spin dynamics between 4.6K and 0.07K in a Tb2Ti2O7 single crystal sample, by means of inelastic neutron scattering experiments. The spectra consist in a dual response, with a static and an inelastic…

Strongly Correlated Electrons · Physics 2015-06-11 Sylvain Petit , Pierre Bonville , Julien Robert , Claudia Decorse , Isabelle Mirebeau

We report high-frequency/high-field electron spin resonance (ESR) and high-field magnetization studies on single crystals of the bond-disordered pyrochlore NaCaCo$_2$F$_7$. Frequency- and temperature-dependent ESR investigations above the…

At low temperatures, Tb$_2$Ti$_2$O$_7$ enters a spin liquid state, despite expectations of magnetic order and/or a structural distortion. Using neutron scattering, we have discovered that in this spin liquid state an excited crystal field…

Strongly Correlated Electrons · Physics 2014-01-16 T. Fennell , M. Kenzelmann , B. Roessli , H. Mutka , J. Ollivier , M. Ruminy , U. Stuhr , O. Zaharko , L. Bovo , A. Cervellino , M. K. Haas , R. J. Cava

The recent identification of the dysprosium titanate compound $Dy_2 Ti_2 O_7$ as a ``Spin-Ice'', i.e. the spin analog of regular entropic ice of Pauling, has created considerable excitement. The ability to manipulate spins using magnetic…

Statistical Mechanics · Physics 2009-11-07 B. Sriram Shastry

In this work we present a neutron Larmor diffraction study of the rare earth pyrochlores $R_2$Ti$_2$O$_7$, with $R$ = Tb, Dy, Ho. We measured the temperature dependence of the lattice parameter with precision $10^{-5}$, between 0.5 K and…

Strongly Correlated Electrons · Physics 2016-11-09 M Ruminy , F Groitl , T Keller , T Fennell

The origin of the lowest-temperature anomaly reported several years ago using a polycrystalline sample of the spin ice compound Dy2Ti2O7 had remained unresolved. Here we finally clarify its origin by susceptibility measurements down to 65…

Strongly Correlated Electrons · Physics 2009-11-11 Ryuji Higashinaka , Yoshiteru Maeno

Here we present experimental evidence of the pseudo-doublet ground state of the non-Kramers compound SrTm2O4, based on specific heat, magnetic entropy and electron paramagnetic resonance. We demonstrate that the two crystallographic Tm3+…