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Mid-infrared dual-comb spectroscopy has the potential to supplant conventional high-resolution Fourier transform spectroscopy in applications that require high resolution, accuracy, signal-to-noise ratio, and speed. Until now, dual-comb…

Dual-comb spectroscopy is a powerful technique to measure optical spectra in a wide spectral range with high-frequency resolution. The development of compact systems operating in the long-wave infrared wavelength range is of high interest…

Over the last two decades, frequency combs have brought breakthroughs in length metrology with traceability to length standards. In particular, frequency-comb-based spectral interferometry is regarded as a promising technology for…

Optics · Physics 2025-01-20 Yoon-Soo Jang , Heulbi Ahn , Sunghoon Eom , Jungjae Park , Jonghan Jin

A new method, FM-FTS, combining Frequency Modulation heterodyne laser spectroscopy and Fourier Transform Spectroscopy is presented. It provides simultaneous sensitive measurement of absorption and dispersion profiles with broadband spectral…

Optics · Physics 2007-09-24 Julien Mandon , Guy Guelachvili , Nathalie Picqué

Frequency combs represent exceptionally precise measurement tools due to the coherence of their spectral lines. While optical frequency comb sources constitute a well-established technology, superconducting circuits provide a relatively…

Superconductivity · Physics 2025-12-12 Angelo Greco , Xavier Ballu , Francesco Giazotto , Alessandro Crippa

We demonstrate single-photon time-domain interference in a new realm. We observe interferences in the photon counting statistics with two separate mode-locked femtosecond lasers of slightly different repetition frequencies, each emitting a…

Optics · Physics 2020-12-01 Nathalie Picqué , Theodor W. Hänsch

We report the development of a new instrument for cavity-enhanced absorption spectroscopy of the fundamental rovibrational transitions of molecules in the long-wave mid-infrared (LWIR) region from 6500 to 10000 nm. Our setup combines a LWIR…

Optical frequency combs provide equidistant frequency markers in the infrared, visible and ultra-violet and can link an unknown optical frequency to a radio or microwave frequency reference. Since their inception frequency combs have…

Dual-comb spectroscopy has demonstrated remarkable capabilities for rapid and sensitive measurements; however, significant challenges still exist in generating high-power, mutually coherent mid-infrared combs. Here we demonstrate that a…

We use optical frequency comb Fourier transform spectroscopy to measure high-resolution spectra of iodomethane, CH$_3$I in the C-H stretch region from 2800 to 3160 cm$^{-1}$. The fast-scanning Fourier transform spectrometer with…

We achieve a quantum-noise-limited absorption sensitivity of 1.7/times10$^{-12}$ cm$^{-1}$ per spectral element at 400 s of acquisition time with cavity-enhanced frequency comb spectroscopy, the highest demonstrated for a comb-based…

An optical frequency comb generated with an electro-optic phase modulator and a chirped radiofrequency waveform is used to perform saturation and pump-probe spectroscopy on the $D_1$ and $D_2$ transitions of atomic potassium. With a comb…

Atomic Physics · Physics 2016-12-21 David A. Long , Adam J. Fleisher , David F. Plusquellic , Joseph T. Hodges

Optical frequency combs are key to optical precision measurements. While most frequency combs operate in the near-infrared regime, many applications require combs at mid-infrared, visible or even ultra-violet wavelengths. Frequency combs…

The sensitivity of molecular fingerprinting is dramatically improved when placing the absorbing sample in a high-finesse optical cavity, thanks to the large increase of the effective path-length. As demonstrated recently, when the…

Optical frequency combs are broadband sources that offer mutually-coherent, equidistant spectral lines with unprecedented precision in frequency and timing for an array of applications. Kerr frequency combs in microresonators require a…

A compact and robust coherent laser light source that provides spectral coverage from the ultraviolet to infrared is desirable for numerous applications, including heterodyne super resolution imaging[1], broadband infrared microscopy[2],…

Dual-comb spectroscopy has been proven a powerful tool in molecular characterization, which remains challenging to implement in the mid-infrared region due to difficulties in the realization of two mutually locked comb sources and efficient…

Mid-infrared (mid-IR) spectroscopy offers unparalleled sensitivity for the detection of trace gases, solids and liquids, which is based on the existence of strong telltale vibrational bands in this part of the spectrum. It was shown more…

Optics · Physics 2016-08-29 Viktor O. Smolski , Honglei Yang , Jia Xu , Konstantin L. Vodopyanov

Historically, there has been a trade-off in spectroscopic measurements between high spectral resolution, broadband coverage, and acquisition time. Optical frequency combs, initially envisioned for precision spectroscopy of the hydrogen atom…

Optics · Physics 2020-06-04 A. V. Muraviev , D. Konnov , K. L. Vodopyanov

Optical cavities provide high sensitivity to dispersion since their resonance frequencies depend on the index of refraction. We present a direct, broadband, and accurate measurement of the modes of a high finesse cavity using an optical…