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Ultrasound and magnetization studies of bond-frustrated ZnCr2S4 spinel are performed in static magnetic fields up to 18 T and in pulsed fields up to 62 T. At temperatures below the antiferromagnetic transition at T_N1 14 K the sound…

Strongly Correlated Electrons · Physics 2015-03-19 V. Tsurkan , S. Zherlitsyn , V. Felea , S. Yasin , Yu. Skourski , J. Deisenhofer , H. -A. Krug von Nidda , P. Lemmens , J. Wosnitza , A. Loidl

Co10Ge3O16 crystallizes in an intergrowth structure featuring alternating layers of spinel and rock salt. Variable-temperature powder synchrotron X-ray and neutron diffraction, magnetometry, and heat capacity experiments reveal a…

Materials Science · Physics 2013-07-12 Phillip T. Barton , Ram Seshadri , Anna Llobet , Matthew R. Suchomel

We studied temperature and magnetic field dependence of magnetization, $M(T)$ and $M(B)$, on thiospinel FeCr$_{2}$S$_{4}$. We observed a step-like anomaly at $T_{OO} \sim$ 9 K for $M$($T$) attributed to an orbital order transition in…

Strongly Correlated Electrons · Physics 2015-05-28 Masakazu Ito , Yuji Nagi , Naotoshi Kado , Shinpei Urakawa , Takuro Ogawa , Akihiro Kondo , Keiichi Koyama , Kazuo Watanabe , Koichi Kindo

We present temperature-dependent x-ray diffraction and temperature- and field-dependent Raman scattering studies of single crystal Mn3O4, which reveal the novel magnetostructural phases that evolve in the spinels due to the interplay…

Strongly Correlated Electrons · Physics 2015-05-14 M. Kim , X. M. Chen , E. Fradkin , P. Abbamonte , S. L. Cooper

We have measured the magnetization and specific heat of multiferroic CoCr2O4 in magnetic fields up to 14 T. The high-field magnetization measurements indicate a new phase transition at T* = 5 - 6 K. The phase between T* and the lock-in…

Cubic spinel GeNi2O4 exhibits intriguing magnetic properties with two successive antiferromagnetic phase transitions (TN1 12.1 and TN2 11.4 K) with the absence of any structural transition. We have performed detailed heat capacity and…

Strongly Correlated Electrons · Physics 2020-12-02 T. Basu , T. Zou , Z. Dun , C. Q. Xu , C. R. Dela Cruz , Tao Hong , H. B. Cao , K. M. Taddei , H. D. Zhou , X. Ke

We have investigated the structural, magnetic, thermodynamic, and dielectric properties of polycrystalline CoCr$_2$O$_4$, an insulating spinel exhibiting both ferrimagnetic and spiral magnetic structures. Below $T_c$ = 94 K the sample…

Materials Science · Physics 2007-05-23 G. Lawes , B. Melot , K. Page , C. Ederer , M. A. Hayward , Th. Proffen , R. Seshadri

We have carried out $^{63,65}$Cu NMR spectra measurements in magnetic field up to about 45~T on single crystal of a multiferroic triangular antiferromagnet CuCrO$_2$. The measurements were performed for magnetic fields aligned along the…

Strongly Correlated Electrons · Physics 2016-12-21 Yu. A. Sakhratov , L. E. Svistov , P. L. Kuhns , H. D. Zhou , A. P. Reyes

We report on neutron diffraction, thermal expansion, magnetostriction, dielectric, and specific heat measurements on polycrystalline FeCr2S4 in external magnetic fields. The ferrimagnetic ordering temperatures $T_{\mathrm{C}}\approx 170$ K…

MnCr2O4 that exhibits spin frustration and complex spiral spin order is of great interest from both fundamental as well as application-oriented perspectives. Unlike CoCr2O4 whose ground state presents the coexistence of commensurate spiral…

High-field phase diagram of a chiral-lattice antiferromagnet Sr(TiO)Cu4(PO4)4 is studied by means of the ultrasound, dielectric, and magnetocaloric-effect measurements. These experimental techniques reveal two new phase transitions at high…

CuCrO2 offers insights into the different types of spiral magnetic orderings that can form spontaneously due to frustration in triangular-lattice antiferromagnets. We explore the magnetic phase diagram up to 65 T along all the principle…

Materials Science · Physics 2015-06-18 Eundeok Mun , M. Frontzek , A. Podlesnyak , G. Ehlers , S. Barilo , S. V. Shiryaev , Vivien S. Zapf

The crystal and magnetic structures of the spinel compounds ZnCr$_2$S$_4$ and ZnCr$_2$Se$_4$ were investigated by high resolution powder synchrotron and neutron diffraction. ZnCr$_2$Se$_4$ exhibits a first order phase transition at $T_N=21$…

Strongly Correlated Electrons · Physics 2009-11-13 F. Yokaichiya , A. Krimmel , V. Tsurkan , I. Margiolaki , P. Thompson , H. N. Bordallo , A. Buchsteiner , N. Stüßer , D. N. Argyriou , A. Loidl

We present the magnetic properties of complete solid solutions of ZnCr$_2$O$_4$ and CoCr$_2$O$_4$: two well-studied oxide spinels with very different magnetic ground states. ZnCr$_2$O$_4$, with non-magnetic $d^{10}$ cations occupying the A…

Materials Science · Physics 2009-06-04 Brent C. Melot , Jennifer E. Drewes , Ram Seshadri , Arthur P. Ramirez

The temperature evolution of the electron spin resonance is studied at cooling the crystal samples of Cs2CuCl4 through the Neel point 0.62 K. A coexistence of the high-frequency spinon type resonance developed in the spin-liquid phase and…

Strongly Correlated Electrons · Physics 2013-05-30 A. I. Smirnov , K. Yu. Povarov , S. V. Petrov , A. Ya. Shapiro

We investigated magnetization, muon spin rotation ($\mu$SR), and $^{119}Sn$ M\"{o}ssbauer spectroscopy on Sn substituted $CuCr_{2-x}Sn_xS_4$ (x=0.03 and 0.08) spinel compounds. The magnetization and $\mu$SR results reveal similar additional…

We examine the evolution of magnetic properties in the normal spinel oxides Mg(1-x)Cu(x)Cr2O4 using magnetization and heat capacity measurements. The end-member compounds of the solid solution series have been studied in some detail because…

Materials Science · Physics 2012-09-11 Moureen C. Kemei , Stephanie L. Moffitt , Daniel P. Shoemaker , Ram Seshadri

The magnetization processes of the spin-3/2 antiferromagnet LiInCr4O8 comprising a "breathing" pyrochlore lattice, which is an alternating array of small and large tetrahedra, are studied under ultrahigh magnetic fields of up to 130 T using…

We have performed a resonant x-ray scattering study at the Co pre-K edge on a single crystal of Ca3Co2O6. The measurements reveal an abrupt transition to a magnetically ordered state immediately below T_N = 25 K, with a magnetic correlation…

Other Condensed Matter · Physics 2008-05-10 S. Agrestini , C. Mazzoli , A. Bombardi , M. R. Lees

Exploring the uncharacterized magnetic phases of Co$^{2+}$ chain compounds is critical for finding new low-dimensional magnets hosting quantized excitations. We map the unexplored magnetic phases of the Co$^{2+}$ chain compound…

Strongly Correlated Electrons · Physics 2023-10-18 Zachary W. Riedel , Zhihao Jiang , Maxim Avdeev , André Schleife , Daniel P. Shoemaker
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