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Interfaces are ubiquitous in Li-ion battery electrodes, occurring across compositional gradients, regions of multiphase intergrowths, and between electrodes and solid electrolyte interphases or protective coatings. However, the impact of…

Materials Science · Physics 2017-04-05 Shenzhen Xu , Ryan Jacobs , Chris Wolverton , Thomas Kuech , Dane Morgan

BAs is III-V semiconductor with ultra-high thermal conductivity, but many of its electronic properties are unknown. This work applies predictive atomistic calculations to investigate the properties of BAs heterostructures, such as strain…

Materials Science · Physics 2019-09-05 Kyle Bushick , Sieun Chae , Zihao Deng , John Heron , Emmanouil Kioupakis

The interrelationship between a material's structure and its properties lies at the heart of materials-related research. Finding how the changes of one affect the other is of primary importance in theoretical and computational materials…

Mesoscale and Nanoscale Physics · Physics 2024-06-14 Hao Wang , Kah-Meng Yam , Zhuoling Jiang , Na Guo , Chun Zhang

Magnetoelectric (ME) interactions in layered structures of magnetostrictive and piezoelectric phases are mediated by mechanical deformation. Here we discuss the frequency dependence of ME coupling in bilayers and trilayers of Permendur, a…

Materials Science · Physics 2009-11-10 U. Laletsin , N. Padubnaya , G. Srinivasan , C. P. DeVreugd

The ability to directly observe electronic band structure in modern nanoscale field-effect devices could transform understanding of their physics and function. One could, for example, visualize local changes in the electrical and chemical…

We report a proof-of-concept demonstration of negative capacitance effect in a nanoscale ferroelectric-dielectric heterostructure. In a bilayer of ferroelectric, Pb(Zr0.2Ti0.8)O3 and dielectric, SrTiO3, the composite capacitance was…

Mesoscale and Nanoscale Physics · Physics 2014-09-15 Asif Islam Khan , Debanjan Bhowmik , Pu Yu , Sung Joo Kim , Xiaoqing Pan , Ramamoorthy Ramesh , Sayeef Salahuddin

Electronic phase behavior in correlated-electron systems is a fundamental problem of condensed matter physics. We argue here that the change in the phase behavior near the surface and interface, i.e., {\em electronic reconstruction}, is the…

Strongly Correlated Electrons · Physics 2015-06-25 Satoshi Okamoto , Andrew J. Millis

The physical origin of Fermi level pinning (FLP) at metal/Ge interfaces has been argued over a long period. Using the Fe$_{3}$Si/Ge(111) heterostructure developed originally, we can explore electrical transport properties through atomically…

Mesoscale and Nanoscale Physics · Physics 2012-01-31 K. Kasahara , S. Yamada , K. Sawano , M. Miyao , K. Hamaya

The conducting interface of LaAlO$_3$/SrTiO$_3$ heterostructures has been studied by hard X-ray photoelectron spectroscopy. From the Ti~2$p$ signal and its angle-dependence we derive that the thickness of the electron gas is much smaller…

We propose that one of the best grounds for the materials design from the viewpoint of {\it electron correlation} such as ferromagnetism, superconductivity is the atomically controlled nanostructures and heterointerfaces, as theoretically…

Materials Science · Physics 2009-11-10 Hideo Aoki

The physical nature of the ferroelectric (FE), ferrielectric (FEI) and antiferroelectric (AFE) phases, their coexistence and spatial distributions underpin the functionality of antiferrodistortive (AFD) multiferroics in the vicinity of…

We study the electron-phonon coupling strength near the interface of monolayer and bilayer FeSe thin films on SrTiO$_3$, BaTiO$_3$, and oxygen-vacant SrTiO$_3$ substrates, using ab initio methods. The calculated total electron-phonon…

Superconductivity · Physics 2016-05-04 Yan Wang , Andreas Linscheid , Tom Berlijn , Steve Johnston

Photoemission spectroscopy is used to investigate the electronic structure of the newly discovered iron-based superconductors LaFeAsO_{1-x}F_x and LaFePO_{1-x}F_x. Line shapes of the Fe 2p core-level spectra suggest an itinerant character…

Interface engineering is an extremely useful tool for systematically investigating materials and the various ways materials interact with each other. We describe different interface engineering strategies designed to reveal the origin of…

Materials Science · Physics 2016-09-19 Hans Boschker , Zhaoliang Liao , Mark Huijben , Gertjan Koster , Guus Rijnders

We report on surface effects on the electronic properties of interfaces in epitaxial LaAlO$_3$/SrTiO$_3$ heterostructures. Our results are based on first-principles electronic structure calculations for well-relaxed multilayer…

Materials Science · Physics 2009-11-13 U. Schwingenschloegl , C. Schuster

Tunneling between two parallel, two-dimensional electron gases (2DEGs) in a complex oxide heterostructure containing a large, mobile electron density of ~ 3x10^14 cm^-2 is used to probe the subband structure of the 2DEGs.…

Mesoscale and Nanoscale Physics · Physics 2013-11-26 Santosh Raghavan , S. James Allen , Susanne Stemmer

Amongst the iron-based superconductors, LiFeAs is unrivalled in the simplicity of its crystal structure and phase diagram. However, our understanding of this canonical compound suffers from conflict between mutually incompatible…

Using metal-ferroelectric junctions as switchable diodes was proposed several decades ago. This was shown to actually work in PbZr(1-x)TixO3 (PZT) by Blom et al. [P.W. M. Blom et al., Phys. Rev. Lett. 73, 2107 (1994)], who reported…

Materials Science · Physics 2012-12-04 Saeedeh Farokhipoor , Beatriz Noheda

By the first-principles electronic structure calculations, we have studied electronic structures of FeSe monolayer and bilayer thin films on SrTiO$_3$ (001) with SrO-termination or TiO$_2$ termination. We find that both FeSe monolayer and…

Superconductivity · Physics 2012-06-18 Kai Liu , Zhong-Yi LU , Tao Xiang

To resolve the microscopic origin of magnetism in the Fe2O3/FeTiO3-system, we have performed density functional theory calculations taking into account on-site Coulomb repulsion. By varying systematically the concentration, distribution and…

Materials Science · Physics 2009-09-23 Rossitza Pentcheva , Hasan Sadat Nabi