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The magnetoelectric coupling, i.e., cross-correlation between electric and magnetic orders, is a very desirable property to combine functionalities of materials for next-generation switchable devices. Multiferroics with spin-driven…

Strongly Correlated Electrons · Physics 2019-01-07 Ian Aupiais , Masahito Mochizuki , Hideaki Sakata , Romain Grasset , Yann Gallais , Alain Sacuto , Maximilien Cazayous

By performing first-principles calculations, we systematically explore the effect of epitaxial strain on the structure and properties of multiferroic TbMnO3. We show that, although the unstrained bulk TbMnO3 displays a non-collinear…

Materials Science · Physics 2015-05-20 Yusheng Hou , Jihui Yang , Xingao Gong , Hongjung Xiang

Extrinsic multiferroic hybrid structures consisting of ferromagnetic and ferroelectric layers elastically coupled to each other are promising due to their robust magnetoelectric effects even at room temperature. For a quantitative analysis…

Materials Science · Physics 2013-01-16 Stephan Gepraegs , Matthias Opel , Sebastian T. B. Goennenwein , Rudolf Gross

Magnetic and magnetoelectric excitations in the multiferroic TbMnO_3 have been investigated at terahertz frequencies. Using different experimental geometries we can clearly separate the electro-active excitations (electromagnons) from the…

Strongly Correlated Electrons · Physics 2009-03-16 A. Pimenov , A. Shuvaev , A. Loidl , F. Schrettle , A. A. Mukhin , V. D. Travkin , V. Yu. Ivanov , A. M. Balbashov

First-principles density functional calculations show that the $\textrm{SrRuO}_{3}/\textrm{PbTiO}_{3}/\textrm{SrRuO}_{3}$ multiferroic junction with asymmetric (RuO$_{2}$/PbO and TiO$_{2}$/SrO) interfaces has a large ferroelectric…

Materials Science · Physics 2013-12-20 Francesco Ricci , Alessio Filippetti , Vincenzo Fiorentini

We present a theoretical examination of the magneto-electric response in the recently discovered multiferroic insulator Cu$_2$OSeO$_3$. Combining Monte Carlo simulation and Ginzburg-Landau analysis we predict the response in each of the…

Strongly Correlated Electrons · Physics 2013-10-22 Ye-Hua Liu , Jung Hoon Han , A. A. Omrani , H. M. Rønnow , You-Quan Li

The magnetic field induced rearrangement of the cycloidal spin structure in ferroelectric mono-domain single crystals of the room-temperature multiferroic BiFeO$_3$ is studied using small-angle neutron scattering (SANS). The cycloid…

Strongly Correlated Electrons · Physics 2018-04-11 S. Bordács , D. G. Farkas , J. S. White , R. Cubitt , L. DeBeer-Schmitt , T. Ito , I. Kézsmárki

Spectrum of coupled spin, acoustic, electro-dipole and electromagnetic waves in orthorhombic perovskite multiferroics placed in external electric and magnetic field has been calculated. Frequency and field dependencies of electric,…

Materials Science · Physics 2013-10-03 Igor V. Bychkov , Dmitry A. Kuzmin , Vladimir G. Shavrov

Magnetodielectric materials are characterized by a strong coupling of magnetic and dielectric properties and in rare cases simultaneously exhibit both, magnetic and polar order. Among other multiferroics, TbMnO3 and GdMnO3 reveal a strong…

Strongly Correlated Electrons · Physics 2015-06-25 A. Pimenov , A. A. Mukhin , V. Yu. Ivanov , V. D. Travkin , A. M. Balbashov , A. Loidl

Terahertz electromagnetic excitations in the multiferroic TbMnO3 at the field-induced magnetic transition are investigated for different orientations of the magnetic cycloid. In addition to the electromagnon along the a-axis, the detailed…

Strongly Correlated Electrons · Physics 2011-03-03 A. M. Shuvaev , V. D. Travkin , V. Yu. Ivanov , A. A. Mukhin , A. Pimenov

The antiferromagnetic domain structure of a multiferroic has been investigated in the presence of a ferroelectric domain structure. It has been demonstrated that an inhomogeneous magnetoelectric (flexomagnetoelectric) interaction leads to…

Materials Science · Physics 2015-05-19 Z. V. Gareeva , A. K. Zvezdin

How the magnetoelectric coupling actually occurs on a microscopic level in multiferroic BiFeO3 is not well known. By using the high-resolution single crystal neutron diffraction techniques, we have determined the electric polarization of…

The control of multiferroic domains through external electric fields has been studied by dielectric measurements and by polarized neutron diffraction on single-crystalline TbMnO$_3$. Full hysteresis cycles were recorded by varying an…

Strongly Correlated Electrons · Physics 2016-02-10 Jonas Stein , Max Baum , Simon Holbein , Vladimir Hutanu , Alexander C. Komarek , Markus Braden

A new type of multiferroicity was experimentally discovered in 2003 in a perovskite manganite TbMnO$_3$ where its ferroelectricity is induced by cycloidally ordered Mn spins. Susequently, such spin-cycloid multiferroic phase was also…

Strongly Correlated Electrons · Physics 2025-02-14 Masahito Mochizuki

The magnetoelectric effect and skyrmions are two fundamental phenomena in the field of condensed-matter physics. Here, using first-principles calculations and Monte-Carlo simulations, we propose that strong magnetoelectric coupling can be…

Materials Science · Physics 2022-06-01 Kaiying Dou , Wenhui Du , Ying Dai , Baibiao Huang , Yandong Ma

We have studied the impact of the magnetic field on the electromagnon excitations in TbMnO3 crystal. Applying magnetic field along the c axis, we show that the electromagnons transform into pure antiferromagnetic modes, losing their polar…

Materials Science · Physics 2011-07-06 P. Rovillain , M. Cazayous , Y. Gallais , M-A. Measson , A. Sacuto , H. Sakata , M. Mochizuki

From magnetic susceptibility, dielectric permittivity, electric polarization and specific heat measurements, we discover spin-induced ferroelectricity and magnetoelectric coupling in Mn3TeO6 and observe two successive magnetic transitions…

Materials Science · Physics 2015-12-01 L. Zhao , Z. Hu , C. Y. Kuo , T. -W. Pi , M. -K. Wu , L. H. Tjeng , A. C. Komarek

A key challenge in antiferromagnetic spintronics is the control of spin configuration on nanometer scales applicable to solid-state technologies. Bismuth ferrite (BiFeO3) is a multiferroic material that exhibits both ferroelectricity and…

We present the microscopic theory of improper multiferroicity in BiMnO3, which can be summarized as follows: (1) the ferroelectric polarization is driven by the hidden antiferromagnetic order in the otherwise centrosymmetric C2/c structure;…

Materials Science · Physics 2010-11-01 I. V. Solovyev , Z. V. Pchelkina

Magnetoelectric multiferroic composite of two types of multiferroic (Type I and II) consisting BiFeO3 and TbMnO3 is studied for enhanced magnetic and transport properties. A narrower band gap is estimated from the UV-visible absorption…

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