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Related papers: The Spin State and Spectroscopic Modes of Multifer…

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The spectroscopic modes of multiferroic BiFeO$_3$ provide detailed information about the very small anisotropy and Dzyaloshinskii-Moriya (DM) interactions responsible for the long-wavelength, distorted cycloid below $\TN = 640$ K. A…

Materials Science · Physics 2015-06-15 Randy S. Fishman

We have identified three of the four magnetoelectric modes of multiferroic BiFeO$_3$ measured using THz spectroscopy. Excellent agreement with the observed peaks is obtained by including the effects of easy-axis anisotropy along the…

Strongly Correlated Electrons · Physics 2015-06-11 Randy S. Fishman , Nobuo Furukawa , Jason T. Haraldsen , Masaaki Matsuda , Shin Miyahara

We have studied the magnetic field dependence of far-infrared active magnetic modes in a single ferroelectric domain \BFO/ crystal at low temperature. The modes soften close to the critical field of 18.8\,T along the [001] (pseudocubic)…

Strongly Correlated Electrons · Physics 2013-06-26 U. Nagel , Randy S. Fishman , T. Katuwal , H. Engelkamp , D. Talbayev , Hee Taek Yi , S. -W. Cheong , T. Rõõm

Low-energy magnon excitations in multiferroic BiFeO$_3$ were measured in detail as a function of temperature around several Brillouin zone centers by inelastic neutron scattering experiments on single crystals. Unique features around 1 meV…

Materials Science · Physics 2014-09-15 Jaehong Jeong , Manh Duc Le , P. Bourges , S. Petit , S. Furukawa , Shin-Ae Kim , Seongsu Lee , S-W. Cheong , Je-Geun Park

We report the direct observation of a "resonance" mode in the lowest-energy optic phonon very near the zone center around (111) in the multiferroic BiFeO$_3$ using neutron scattering methods. The phonon scattering intensity is enhanced when…

We examine the high-frequency optical mode of {\alpha}-Fe2O3 and report that Dzyaloshinskii-Moriya (DM) interaction generates a new type of torque on the magnetic resonance. Using a continuous-wave terahertz interferometer, we measure the…

Materials Science · Physics 2023-07-11 Qiyao Liu , Taeheon Kim , Kyusup Lee , Dongsheng Yang , Dushyant Kumar , Fanrui Hu , Hyunsoo Yang

We have studied spin excitation spectra in the Shastry-Sutherland model compound SrCu$_2$(BO$_3$)$_2$ in magnetic fields using far-infrared Fourier spectroscopy. The transitions from the ground singlet state to the triplet state at 24…

Other Condensed Matter · Physics 2009-11-10 T. Rõõm , D. Hüvonen , U. Nagel , J. Hwang , T. Timusk

Anisotropic spin-spin interactions of the symmetry described by Dzyaloshinsky and Moriya are generally considered weak, as they depend on the spin-orbit couplings. In frustrated spin systems with singlet ground states they can, however,…

Strongly Correlated Electrons · Physics 2009-11-07 O. Cepas , T. Sakai , T. Ziman

We study the effect of magnon interactions on the spin wave spectra of the all-in-all-out phase of the pyrochlore nearest neighbour antiferromagnet with a Dzyaloshinskii-Moriya interaction ($D$). The leading order corrections to spin wave…

Strongly Correlated Electrons · Physics 2025-03-04 V. V. Jyothis , Kallol Mondal , Himanshu Mavani , V. Ravi Chandra

We present a multi-modal spectroscopic paradigm that enables independent measurement of charge and spin degrees of freedom (DOF) in strongly correlated materials. This spin-based technique probes symmetry-specific Hamiltonian parameters by…

Mesoscale and Nanoscale Physics · Physics 2023-09-18 Stephen Carr , Ilija K. Nikolov , Rong Cong , Adrian Del Maestro , Chandrasekhar Ramanathan , V. F. Mitrović

Magnetic excitations in the isostructural spin-dimer systems Sr3Cr2O8 and Ba3Cr2O8 are probed by means of high-field electron spin resonance at sub-terahertz frequencies. Three types of magnetic modes were observed. One mode is gapless and…

The magnetoelectric coupling, i.e., cross-correlation between electric and magnetic orders, is a very desirable property to combine functionalities of materials for next-generation switchable devices. Multiferroics with spin-driven…

Strongly Correlated Electrons · Physics 2019-01-07 Ian Aupiais , Masahito Mochizuki , Hideaki Sakata , Romain Grasset , Yann Gallais , Alain Sacuto , Maximilien Cazayous

The magnon and optical phonon spectrum of an incommensurate multiferroic such as BiFeO3 is considered in the framework of a phenomenological Landau theory. The resulting spin wave spectrum is quite distinct from commensurate substances due…

Strongly Correlated Electrons · Physics 2008-01-24 Rogerio de Sousa , Joel E. Moore

We report the observation of a frequency shift and splitting of the electron spin resonance (ESR) mode of the low-dimensional S=1/2 frustrated antiferromagnet Cs2CuCl4 in the spin-correlated state below the Curie-Weiss temperature 4 K but…

Strongly Correlated Electrons · Physics 2015-03-18 K. Yu. Povarov , A. I. Smirnov , O. A. Starykh , S. V. Petrov , A. Ya. Shapiro

A key challenge in antiferromagnetic spintronics is the control of spin configuration on nanometer scales applicable to solid-state technologies. Bismuth ferrite (BiFeO3) is a multiferroic material that exhibits both ferroelectricity and…

By combining two independent approaches, inelastic neutron scattering measurements and density functional theory calculations, we study the spin-waves in the high-temperature collinear antiferromagnetic phase (AFM2) of Mn$_5$Si$_3$. We…

Mesoscale and Nanoscale Physics · Physics 2021-01-13 F. J. dos Santos , N. Biniskos , S. Raymond , K. Schmalzl , M. dos Santos Dias , P. Steffens , J. Persson , S. Blügel , S. Lounis , T. Brückel

The ZFC and FC magnetization dependence on temperature was measured for BiFeO3 ceramics at the applied magnetic field up to H=10T in 2K-1000K range. The antiferromagnetic order was detected from the hysteresis loops below the Neel…

Materials Science · Physics 2013-05-15 B. Andrzejewski , A. Molak , B. Hilczer , A. Budziak , R. Bujakiewicz-Koronska

A microscopic model for the room-temperature multiferroic BiFeO$_3$ that includes two Dzyaloshinskii-Moriya interactions and single-ion anisotropy along the ferroelectric polarization predicts both the zero-field spectroscopic modes as well…

Strongly Correlated Electrons · Physics 2015-10-28 Randy S. Fishman , Jun Hee Lee , Sándor Bordács , István Kézsmárki , Urmas Nagel , Toomas Rõõm

We present a terahertz spectroscopic study of magnetic excitations in ferroelectric antiferromagnet BiFeO3. We interpret the observed spectrum of long-wavelength magnetic resonance modes in terms of the normal modes of the material's…

Materials Science · Physics 2015-05-27 D. Talbayev , S. A. Trugman , Seongsu Lee , Hee Taek Yi , S. -W. Cheong , A. J. Taylor

We report a comprehensive inelastic neutron scattering study of the hybrid molecule-based multiferroic compound (ND4)2FeCl5D2O in the zero-field incommensurate cycloidal phase and the high-field quasi-collinear phase. The spontaneous…

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