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Here we describe the design, single-molecule transport measurements, and theoretical modeling of a ferrocene-based organometallic molecular wire, whose bias-dependent conductance shows a clear Lorentzian form with magnitude exceeding 70% of…

We present consistent results for molecular conduction using two central-complementary approaches: the non-equilibrium Green's function technique and the quantum master equation method. Our model describes electronic conduction in a…

Mesoscale and Nanoscale Physics · Physics 2016-04-13 Bijay Kumar Agarwalla , Dvira Segal

We develop a new general formulation to explore light-driven electron transport through a single-molecule device with multiple pathways. Three individual systems are proposed including (i) a two-terminal molecular junction based on…

Mesoscale and Nanoscale Physics · Physics 2014-01-20 Liang-Yan Hsu , Herschel Rabitz

Effects of relative orientation of the molecules on electron transport in molecular devices are studied by non-equilibrium Green's function method based on density functional theory. In particular, two molecular devices, with the planer…

Mesoscale and Nanoscale Physics · Physics 2009-11-11 Yan-Hong Zhou , Xiao-Hong Zheng , Ying Xu , Zhao Yang Zeng , Zhi Zeng

Electronic transport through a single-molecule magnet Mn$_{12}$ in a two-terminal set up is calculated using the non-equilibrium Green's function method in conjunction with density-functional theory. A single-molecule magnet Mn$_{12}$ is…

Materials Science · Physics 2010-01-28 Salvador Barraza-Lopez , Kyungwha Park , Víctor García-Suárez , Jaime Ferrer

The effects of different contact geometries, bond dimerization, and gate voltage on quantum transport through a C$_{60}$ molecule are studied by the Landauer-B\"{u}ttiker formula based on the Green's function technique. It is shown that the…

Mesoscale and Nanoscale Physics · Physics 2008-08-12 Alireza Saffarzadeh

The effect of thermal structural fluctuations on the modulation of the transfer integrals between close molecules is studied using a combination of molecular dynamics simulations and quantum chemical calculations of the transfer integral.…

Other Condensed Matter · Physics 2007-05-23 Alessandro Troisi , Giorgio Orlandi

The multilayer multiconfiguration time-dependent Hartree theory within second quantization representation of the Fock space is applied to study correlated electron transport in models of single-molecule junctions. Extending previous work,…

Mesoscale and Nanoscale Physics · Physics 2015-06-12 Haobin Wang , Michael Thoss

Transport in molecular electronic devices is different from that in semiconductor mesoscopic devices in two important aspects: (1) the effect of the electronic structure and (2) the effect of the interface to the external contact. A…

Mesoscale and Nanoscale Physics · Physics 2009-11-07 Yongqiang Xue , Supriyo Datta , Mark A. Ratner

We study the dynamics of the electron current in nanodevices where there are time-varying components and interactions. These devices are a nanojunction attached to heat baths and with dynamical electron-phonon interactions and a…

Mesoscale and Nanoscale Physics · Physics 2017-09-13 Eduardo C. Cuansing , Francis A. Bayocboc , Christian M. Laurio

A tight-binding model of electron dynamics in mesoscopic normal rings is studied using boundary conformal field theory. The partition function is calculated in the low energy limit and the persistent current generated as a function of an…

Mesoscale and Nanoscale Physics · Physics 2009-10-31 S. Jaimungal , M. H. S. Amin , G. Rose

The possibility of using single molecule junctions as electron pumps for energy conversion and storage is considered. It is argued that the small dimensions of these systems enable to make use of unique intra-molecular quantum coherences in…

Quantum Physics · Physics 2015-05-20 Roie Volkovich , Uri Peskin

We investigate charge transport in C$_{60}$-based single-molecule junctions with graphene electrodes employing a combination of density functional theory (DFT) electronic structure calculations and Landauer transport theory. In particular,…

Mesoscale and Nanoscale Physics · Physics 2017-01-12 Susanne Leitherer , Pedro B. Coto , Konrad Ullmann , Heiko B. Weber , Michael Thoss

Along with the progress of spin science and spintronics research, the flow of electron spins, (i.e. spin current), has attracted interest. New phenomena and electronic states were explained in succession using the concept of spin current.…

Materials Science · Physics 2023-10-20 Sadamichi Maekawa , Takashi Kikkawa , Hiroyuki Chudo , Jun'ichi Ieda , Eiji Saitoh

Exploring the use of individual molecules as active components in electronic devices has been at the forefront of nanoelectronics research in recent years. Compared to semiconductor microelectronics, modeling transport in single-molecule…

Mesoscale and Nanoscale Physics · Physics 2015-06-24 Yongqiang Xue , Mark A. Ratner

Using molecular dynamics simulation, we investigate transport properties of a classical two-dimensional electron system confined in a microchannel with a narrow constriction. As a function of the confinement strength of the constriction,…

Mesoscale and Nanoscale Physics · Physics 2012-10-18 Moto Araki , Hisao Hayakawa

The single-molecule conductance of a 3-ring, conjugated azomethine was studied using the mechanically controlled breakjunction technique. Charge transport properties are found to be comparable to vinyl-based analogues; findings are…

Mesoscale and Nanoscale Physics · Physics 2016-08-18 Max Koole , Riccardo Frisenda , Michiel L. Petrus , Mickael L. Perrin , Herre S. J. van der Zant , Theo J. Dingemans

We study theoretically how electrons, coherently injected at one point on the boundary of a two-dimensional electron system, are focused by a perpendicular magnetic field $B$ onto another point on the boundary. Using the non-equilibrium…

Mesoscale and Nanoscale Physics · Physics 2013-11-28 Thomas Stegmann , Dietrich E. Wolf , Axel Lorke

The spin dependent charge transport in zigzag graphene nanoribbons (ZGNRs) has been investigated by the nonequilibrium Green's function method combined with the density functional theory at the local spin density approximation. The current…

Mesoscale and Nanoscale Physics · Physics 2015-06-04 Ting-Ting Wu , Xue-Feng Wang , Ming-Xing Zhai , Hua Liu , Liping Zhou , Yong-Jin Jiang

We numerically investigate the electronic transport properties between two mesoscopic graphene disks with a twist by employing the density functional theory coupled with non-equilibrium Green's function technique. By attaching two graphene…

Mesoscale and Nanoscale Physics · Physics 2020-07-01 Yulei Han , Yafei Ren , Xinlong Dong , Junjie Zeng , Wei Ren , Zhenhua Qiao