Related papers: Second harmonic microscopy of monolayer MoS2
We theoretically predict efficient optical second-harmonic generation (SHG) from a few hundred nanometer thick slab consisting of a quadratic nonlinear anisotropic medium whose linear principal permittivities are, at the fundamental…
Second and third harmonic generation in the opaque region of a GaAs wafer is experimentally observed both in transmission and reflection. These harmonic components can propagate through an opaque material as long as the pump is tuned to a…
Two-dimensional molybdenum disulfide (MoS$_2$) featuring atomically thin thickness and unique electronic structure with favorable bandgap has been widely recognized as an attractive new material for the development of the next generation of…
We perform an optical spectroscopy study to investigate the properties of different artificial MoS$_2$ bi- and trilayer stacks created from individual monolayers by a deterministic transfer process. These twisted bi- and trilayers differ…
The effective nonlinear response of films of random composites consisting of a binary composite with nonlinear particles randomly embedded in a linear host is theoretically and numerically studied. A theoretical expression for the effective…
Second-harmonic and sum-frequency mixing phenomena associated with 3D-localized photonic modes are studied in InP-based planar photonic crystal microcavities excited by short-pulse radiation near 1550 nm. Three-missing-hole microcavities…
The two-dimensional ferroelectrics GeS, GeSe, SnS and SnSe are expected to have large spontaneous in-plane electric polarization and enhanced shift-current response. Using density functional methods, we show that these materials also…
We exploit a slightly noncollinear second-harmonic cross-correlation scheme to map the 3D space-time intensity distribution of an unknown complex-shaped ultrashort optical pulse. We show the capability of the technique to reconstruct both…
We compute the nonlinear optical response of an Fe monolayer placed on top of 1 to 4 monolayers of Cu(001). Our calculation is based on ab initio eigenstates of the slab, which are obtained within the full-potential linearized augmented…
Nonlinear optical generation from a crystalline material can reveal the symmetries of both its lattice structure and underlying ordered electronic phases and can therefore be exploited as a complementary technique to diffraction based…
Nano-resonator integrated with two-dimensional materials (e.g. transition metal dichalcogenides) have recently emerged as a promising nano-optoelectronic platform. Here we demonstrate resonatorenhanced second-harmonic generation (SHG) in…
Hyperbolic plasmonic metamaterials provide numerous opportunities for designing unusual linear and nonlinear optical properties. We show that the modal overlap of fundamental and second-harmonic light in an anisotropic plasmonic…
We discuss a novel method for generating octave-spanning supercontinua and few-cycle pulses in the important mid-IR wavelength range. The technique relies on strongly phase-mismatched cascaded second-harmonic generation (SHG) in mid-IR…
We describe a compact and stable setup for detecting the optical second harmonics, in which the incident plane rotates with respect to the sample. The setup is composed of rotating Fresnel-rhomb optics and a femtosecond ytterbium-doped…
We conduct a theoretical and numerical study on the second-harmonic (SH) optical response of a nano-structured metamaterial composed of a periodic array of inclusions. Both the inclusions and their surrounding matrix are made of…
We analytically investigate the effect of a non-centrosymmetric geometry in the optical second harmonic (SH) generation from a particle made of a centrosymmetric material, in the interior of which quadratic optical processes are suppressed.…
Second harmonic generation is considered in lossy negative-index metamaterials. It is shown that energy transfer from fundamental to harmonic takes place in the entire sample for the range of phase mismatch values. Note that in conventional…
In this letter we report on the synthesis of monolayers of MoS$_2$ via chemical vapor deposition directly on thin films of Al$_2$O$_3$ grown by spatial atomic layer deposition. The synthesized monolayers are characterized by atomic force…
Nonlinear metasurface holography shows the great potential of metasurfaces to control the phase, amplitude, and polarization of light while simultaneously converting the frequency of the light. The possibility of tailoring the scattering…
Optical second harmonic generation (SHG) is a nonlinear optical effect widely used for nonlinear optical microscopy and laser frequency conversion. Closed-form analytical solution of the nonlinear optical responses is essential for…