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The present work reports the preparation of polycrystalline multiferroic $GdFeO_3$ (GdFO) and characterization with x-ray diffraction (XRD), magnetization, temperature dependent Raman spectroscopy, temperature and magnetic field dependent…

Materials Science · Physics 2021-12-06 Anjali Panchwanee , V. Raghavendra Reddy , Ajay Gupta , V. G. Sathe

The phonon density of states (DOS) and magnetic excitation spectrum of polycrystalline BiFeO$_3$ were measured for temperatures $200 \leq T \leq 750\,$K, using inelastic neutron scattering (INS). Our results indicate that the magnetic…

Materials Science · Physics 2012-02-27 Olivier Delaire , Matthew B. Stone , Jie Ma , Ashfia Huq , Delphine Gout , Craig Brown , Kefeng Wang , Zhifeng Ren

The reflectivity of single-crystalline CoO has been studied by optical spectroscopy for wave numbers ranging from 100 to 28,000\wn and for temperatures 8 $< T <$ 325 K\@. A splitting of the cubic IR-active phonon mode on passing the…

Strongly Correlated Electrons · Physics 2009-01-20 Ch. Kant , T. Rudolf , F. Schrettle , F. Mayr , J. Deisenhofer , P. Lunkenheimer , M. V. Eremin , A. Loidl

Infrared reflectivity spectra of cubic SrMnO$_{3}$ ceramics reveal 18 % stiffening of the lowest-frequency phonon below the antiferromagnetic phase transition occurring at T$_{N}$ = 233 K. Such a large temperature change of the polar phonon…

We present neutron inelastic scattering measurements of the low-energy phonons in single crystal BiFeO3. The dispersions of the three acoustic phonon modes (LA along [100], TA1 along [010] and TA2 along [110]) and two low energy optic…

We present the results of pressure-dependent far-infrared reflectivity measurements on the multiferroic perovskite BiFeO3 at room temperature. The observed behavior of the infrared-active phonon modes as a funtion of pressure clearly…

Other Condensed Matter · Physics 2007-12-06 A. Pashkin , K. Rabia , S. Frank , C. A. Kuntscher , R. Haumont , R. Saint-Martin , J. Kreisel

Spin-phonon coupling, the interaction of spins with surrounding lattice is a key parameter to understand the underlying physics of multiferroics and engineer their magnetization dynamics. Elementary excitations in multiferroic materials are…

Materials Science · Physics 2020-11-05 Bommareddy Poojitha , Anjali Rathore , Ankit Kumar , Surajit Saha

The magnetic susceptibility between 1.5 and 800 K, the infrared reflectivity at room temperature and the temperature dependence of the dielectric constant at mm-wavelengths are reported for single crystalline BiFeO3. A well developed…

Strongly Correlated Electrons · Physics 2010-07-22 Jun Lu , M Schmidt , P Lunkenheimer , A Pimenov , A A Mukhin , V D Travkin , A Loidl

We have measured polarized Raman scattering spectra of the Fe$_{1-x}$Co$_{x}$Sb$_{2}$ and Fe$_{1-x}$Cr$_{x}$Sb$_{2}$ (0$\leq x\leq $0.5) single crystals in the temperature range between 15 K and 300 K. The highest energy $B_{1g}$ symmetry…

Strongly Correlated Electrons · Physics 2016-09-20 N. Lazarević , Z. V. Popović , Rongwei Hu , C. Petrovic

Collective interactions between localized electronic excitations and the crystal lattice are central to many emergent phenomena in materials, including ferroelectricity and quantum magnetism. Despite its importance, the scaling behavior of…

Materials Science · Physics 2025-11-25 Fangliang Wu , Xiaoxuan Ma , Zhongwei Zhang , Motoaki Bamba , Jian Sun , Yuan Wan , Shixun Cao , Qi Zhang

Optical properties of single-crystal monoclinic CuO in the range 70 - 6000 \cm were studied at temperatures from 7 to 300 K. Normal reflection spectra were obtained from the (001) and (010) crystal faces thus giving for the first time…

Strongly Correlated Electrons · Physics 2009-10-31 A. B. Kuz'menko , D. van der Marel , P. J. M. van Bentum , E. A. Tishchenko , C. Presura , A. A. Bush

In bismuth ferrite (BiFeO3), antiferromagnetic and ferroelectric order coexist at room temperature, making it of particular interest for studying magnetoelectric coupling. The mutual control of magnetic and electric properties is very…

Materials Science · Physics 2012-07-23 C. Beekman , A. A. Reijnders , Y. S. Oh , S. W. Cheong , K. S. Burch

We report the complex dielectric function of high-quality Na_3Ir_3O_8 single crystals determined by spectroscopic ellipsometry in the spectral range from 15 meV to 2 eV. The far-infrared phonon spectra exhibit highly asymmetric line shapes…

Strongly Correlated Electrons · Physics 2014-02-28 D. Pröpper , A. N. Yaresko , T. I. Larkin , T. N. Stanislavchuk , A. A. Sirenko , T. Takayama , A. Matsumoto , H. Takagi , B. Keimer , A. V. Boris

We have performed Raman scattering investigations on the high energy magnetic excitations in a BiFeO$_3$ single crystal as a function of both temperature and laser excitation energy. A strong feature observed at 1250 cm$^{-1}$ in the Raman…

Strongly Correlated Electrons · Physics 2018-11-13 M. Cazayous , A. Sacuto , D. Lebeugle , D. Colson

We report inelastic neutron scattering measurements of the phonon spectra in a pure powder sample of the multiferroic material BiFeO3. A high-temperature range was covered to unravel the changes in the phonon dynamics across the Neel (T_N ~…

Materials Science · Physics 2015-03-19 M. Zbiri , H. Schober , N. Choudhury , R. Mittal , S. L. Chaplot , S. J. Patwe , S. N. Achary , A. K. Tyagi

We report plane-polarized Raman scattering spectra of iron oxypnictide superconductor NdFeAsO$_{1-x}$F$_x$ single crystals with varying fluorine $x$ content. The spectra exhibit sharp and symmetrical phonon lines with a weak dependence on…

Superconductivity · Physics 2009-11-13 Y. Gallais , A. Sacuto , M. Cazayous , P. Cheng , L. Fang , H. H. Wen

In this work we present a detailed study of the structural and lattice dynamic properties of Y-doped EuMnO3 ceramics (Eu1-xYxMnO3, with 0<x<0.55). A thorough analysis towards the correlation between both structural and Raman modes…

One- and multi-phonon excitations of the single crystalline LaCoO3 were studied using Raman spectroscopy in the temperature region of 5 K - 300 K. First-order Raman spectra show a larger number of phonon modes than allowed for the…

Strongly Correlated Electrons · Physics 2022-05-31 V. Gnezdilov , K. -Y. Choi , Yu. Pashkevich , P. Lemmens , S. Shiryaev , G. Bychkov , S. Barilo , V. Fomin , A. V. Yeremenko

We have measured far infrared reflectance and transmittance spectra as well as Raman scattering spectra of \alpha'-NaV2O5 single crystals for all the principal polarizations. The temperature range above the phase transition temperature…

Strongly Correlated Electrons · Physics 2019-08-17 M. N. Popova , A. B. Sushkov , S. A. Golubchik , B. N. Mavrin , V. N. Denisov , B. Z. Malkin , A. I. Iskhakova , M. Isobe , Y. Ueda

Rare-earth orthoferrites are a promising platform for antiferromagnetic spintronics with a rich variety of terahertz spin and lattice dynamics phenomena. For instance, it has been experimentally demonstrated that the light-driven optical…