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We present a rigorous and computationally efficient method to do a parameter-free analysis of molecular wires connected to contacts. The self-consistent field approach is coupled with Non-equilibrium Green's Function (NEGF) formalism to…

Mesoscale and Nanoscale Physics · Physics 2016-08-31 Prashant Damle , Avik W. Ghosh , Supriyo Datta

Nonequilibrium Greens function techniques (NEGF) combined with density functional theory (DFT) calculations have become a standard tool for the description of electron transport through single molecule nanojunctions in the coherent…

Mesoscale and Nanoscale Physics · Physics 2015-11-05 Victor Geskin , Robert Stadler , Jérôme Cornil

We aim to provide engineers with an introduction to the non-equilibrium Green's function (NEGF) approach, which provides a powerful conceptual tool and a practical analysis method to treat small electronic devices quantum mechanically and…

Mesoscale and Nanoscale Physics · Physics 2007-05-23 M. P. Anantram , M. S. Lundstrom , D. E. Nikonov

Confined nanoscale spaces, electric fields and tunneling currents make the molecular electronic junction an experimental device for the discovery of new, out-of-equilibrium chemical reactions. Reaction-rate theory for current-activated…

Mesoscale and Nanoscale Physics · Physics 2021-04-27 Riley J. Preston , Maxim F. Gelin , Daniel S. Kosov

The Non-Equilibrium Green's Function (NEGF) method combined with ab initio calculations has been widely used to study charge transport in molecular junctions. However, the significant computational demands of high-resolution calculations…

Computational Physics · Physics 2026-05-19 Xuan Ji , Qiang Qi , Yueqi Chen , Chen Zhou , Xi Yu

We present a novel implementation of the first-principles approach to molecular charge transport using the non-equilibrium Green's function formalism in combination with the ADF/BAND periodic band-structure DFT code, together with results…

Materials Science · Physics 2014-03-18 C. J. O. Verzijl , J. M. Thijssen

Through the Non-Equilibrium Green's Function (NEGF) formalism, quantum-scale device simulation can be performed with the inclusion of electron-phonon scattering. However, the simulation of realistically sized devices under the NEGF…

Mesoscale and Nanoscale Physics · Physics 2015-05-27 Stephen Cauley , Mathieu Luisier , Venkataramanan Balakrishnan , Gerhard Klimeck , Cheng-Kok Koh

In this work, we investigate the transport phenomena in compound semiconductor material based buried channel Quantum Well MOSFET with a view to developing a simple and effective model for the device current. Device simulation has been…

Mesoscale and Nanoscale Physics · Physics 2020-06-14 Ehsanur Rahman , Abir Shadman , Sudipta Romen Biswas , Kanak Datta , Quazi D. M. Khosru

The electrostatic gating effects on molecular transistors are investigated using the density functional theory (DFT) combined with the nonequilibrium Green's function (NEGF) method. When molecular energy levels are away from the Fermi…

Mesoscale and Nanoscale Physics · Physics 2011-09-28 D. Hou , J. H. Wei

Nanoscale electronic transport is of intense technological interest, with applications ranging from semiconducting devices and molecular junctions to charge migration in biological systems. Most explicit theoretical approaches treat…

Mesoscale and Nanoscale Physics · Physics 2014-08-08 Justin E. Elenewski , Hanning Chen

By carrying out density functional theory (DFT) analysis within the Keldysh non-equilibrium Green's function (NEGF) framework, we investigate the quantum transport properties of Au-C60-Au molecular junctions from the first principles. We…

Materials Science · Physics 2007-05-23 N. Sergueev , D. Roubtsov , H. Guo

Since proposed in the 70s, the Non-Equilibrium Green Function (NEGF) method has been recognized as a standard approach to quantum transport simulations. Although it achieves superiority in simulation accuracy, the tremendous computational…

Mesoscale and Nanoscale Physics · Physics 2023-12-05 Yingzhanghao Zhou , Xiang Chen , Peng Zhang , Jun Wang , Lei Wang , Hong Guo

Multi-scale computational approaches are important for studies of novel, low-dimensional electronic devices since they are able to capture the different length-scales involved in the device operation, and at the same time describe critical…

Mesoscale and Nanoscale Physics · Physics 2019-04-04 Gaetano Calogero , Nick R. Papior , Mohammad Koleini , Matthew Helmi Leth Larsen , Mads Brandbyge

We propose a new molecular simulation framework that combines the transferability, robustness and chemical flexibility of an ab initio method with the accuracy and efficiency of a machine learned force field. The key to achieve this mix is…

Computational Physics · Physics 2020-01-08 Sebastian Dick , Marivi Fernandez-Serra

The coherent quantum effect becomes increasingly important in the heat dissipation bottleneck of semiconductor nanoelectronics with the characteristic size shrinking down to few nano-meters scale nowadays. However, the quantum mechanical…

Mesoscale and Nanoscale Physics · Physics 2020-11-18 Yangyu Guo , Marc Bescond , Zhongwei Zhang , Mathieu Luisier , Masahiro Nomura , Sebastian Volz

Orbital-free density functional theory (OFDFT) offers a challenging way of electronic-structure calculations scaled as $\mathcal{O}(N)$ computation for system size $N$. We here develop a scheme of the OFDFT calculations based on the…

Computational Physics · Physics 2021-09-06 Fumihiro Imoto , Masatoshi Imada , Atsushi Oshiyama

While the success of density functional theory (DFT) has led to its use in a wide variety of fields such as physics, chemistry, materials science and biochemistry, it has long been recognised that conventional methods are very inefficient…

Materials Science · Physics 2007-05-23 D. R. Bowler , R. Choudhury , M. J. Gillan , T. Miyazaki

Designing nanoscale electronic devices such as the currently manufactured nanoribbon field-effect transistors (NRFETs) requires advanced modeling tools capturing all relevant quantum mechanical effects. State-of-the-art approaches combine…

While the vast majority of calculations reported on molecular conductance have been based on the static non-equilibrium Green's function formalism combined with density functional theory, in recent years a few time-depedent approaches to…

A theoretical understanding of the experimental electronic transport phenomena in gas sensors based on DNA functionalized graphene is presented by quantitatively investigating the time-dependent electronic transport in these devices using…

Mesoscale and Nanoscale Physics · Physics 2013-09-16 P. Gurung , N. Deo