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Thermal expansion in materials can be accurately modeled with careful anharmonic phonon calculations within density functional theory. However, because of interest in controlling thermal expansion and the time consumed evaluating thermal…

Materials Science · Physics 2017-11-03 Joseph T. Schick , Abhijith M. Gopakumar , Andrew M. Rappe

The thermodynamic approach to non-equilibrium dynamics describes the state of macroscopic systems by means of a collection of intensities or intensive variables. The latter are by definition the differentials of the entropy with respect to…

chao-dyn · Physics 2008-02-03 Z. Hens , X. de Hemptinne

Thermal conductivity and interfacial thermal conductance play crucial roles in the design of engineering systems where temperature and thermal stress are of concerns. To date, a variety of measurement techniques are available for both bulk…

Materials Science · Physics 2016-12-09 Dongliang Zhao , Xin Qian , Xiaokun Gu , Saad Ayub Jajja , Ronggui Yang

We discuss what kind of quantum channels can enable thermalization processes. We show that in order to determine a system's temperature, a thermometer needs to dynamically gain information about the system's local Hamiltonian and not just…

Quantum Physics · Physics 2021-11-09 Daniel Grimmer , Robert B. Mann , Eduardo Martin-Martinez

Chemical and biological networks can describe a wide variety of processes, from gene regulatory networks to biochemical oscillations. Modeled by chemical master equations, these processes are inherently stochastic, as fluctuations dominate…

Statistical Mechanics · Physics 2025-12-23 Schuyler B. Nicholson , Luis Pedro García-Pintos

We build a comprehensive methodology for the fast computation of entropy across both solid and liquid phases. The proposed method utilizes a single trajectory of molecular dynamics (MD) to facilitate the calculation of entropy, which is…

Computational Physics · Physics 2024-04-05 Qi-Jun Hong , Zi-Kui Liu

In recent years, the unified theory of information and thermodynamics has been intensively discussed in the context of stochastic thermodynamics. The unified theory reveals that information theory would be useful to understand…

Statistical Mechanics · Physics 2018-07-23 Sosuke Ito

Chemical theories involving thermodynamical equilibrium states invariably utilize statistical mechanical equilibrium density distributions. Here, a definition of heat-work transformation termed thermo mechanical coherence is first made, and…

Chemical Physics · Physics 2007-05-23 Christopher G. Jesudason

While the ongoing search to discover new high-entropy systems is slowly expanding beyond metals, a rational and effective method for predicting "in silico" the solid solution forming ability of multi-component systems remains yet to be…

Materials Science · Physics 2018-07-16 Yoav Lederer , Cormac Toher , Kenneth S. Vecchio , Stefano Curtarolo

Thermoelectric materials can achieve direct energy conversion between electricity and heat, thus can be applied to waste heat harvesting and solid-state cooling. The discovery of new thermoelectric materials is mainly based on experiments…

Materials Science · Physics 2024-05-07 Tao Fan , Artem R. Oganov

The entropy shows an unavoidable tendency of disorder in thermostatistics according to the second thermodynamics law. This provides a minimization entropy principle for quantum thermostatistics with the von Neumann entropy and nonextensive…

Quantum Physics · Physics 2021-04-09 M. X. Luo , X. Wang

Efficiently harvesting thermodynamic resources requires a precise understanding of their structure. This becomes explicit through the lens of information engines -- thermodynamic engines that use information as fuel. Maximizing the work…

Statistical Mechanics · Physics 2024-02-28 Alexander B. Boyd , James P. Crutchfield , Mile Gu , Felix C. Binder

In this work, we report the results of \emph{ab initio} calculations of thermochemical properties of several compounds in the Fe-Nd, B-Nd and B-Fe-Nd systems. We have performed DFT+U calculations to compute the enthalpy of formation of the…

Materials Science · Physics 2020-08-21 Adie Tri Hanindriyo , Soumya Sridar , K. C. Hari Kumar , Kenta Hongo , Ryo Maezono

Fast prediction of the synthesizability conditions of materials remains challenging, even assuming synthesis under thermodynamic equilibrium. Approaches solely based on convex stability hulls neglect finite-temperature effects, while…

Materials Science · Physics 2026-05-27 Finja Tadge , Javier Sanz Rodrigo , Andrea Crovetto

Thermodynamic simulation of chemical and metallurgical systems is the only method to predict their equilibrium composition and is the most important application of chemical thermodynamics. The conventional strategy of simulation is always…

Chemical Physics · Physics 2007-05-23 B. Zilbergleyt

Melting properties are critical for designing novel materials, especially for discovering high-performance, high-melting refractory materials. Experimental measurements of these properties are extremely challenging due to their high melting…

Materials Science · Physics 2024-08-19 Li-Fang Zhu , Fritz Koermann , Qing Chen , Malin Selleby , Joerg Neugebauer , and Blazej Grabowski

A general formulation is presented to derive the equation of motion and to demonstrate thermodynamic consistency for several classes of phase field models at once. It applies to models with a conserved phase field, describing either uniform…

Materials Science · Physics 2011-05-06 Mowei Cheng , Stefaan Cottenier , Heike Emmerich

Topological phases of matter$\unicode{x2013}$comprising both insulators and semimetals$\unicode{x2013}$offer great potential for quantum applications, but identifying new candidates remains challenging due to expensive first-principles…

Materials Science · Physics 2026-04-08 Xinyu Xu , Arif Ullah , Ming Yang

Thermoelectric materials can generate clean energy by transforming waste heat into electricity. The effectiveness of thermoelectric materials is measured by the dimensionless figure of merit, ZT. The quest for high ZT materials has drawn…

Materials Science · Physics 2025-09-03 Chung T. Ma , S. Joseph Poon

Chemical modelling serves two purposes in dynamical models: accounting for the effect of microphysics on the dynamics and providing observable signatures. Ideally, the former must be done as part of the hydrodynamic simulation but this…

Computational Physics · Physics 2021-09-15 J. Holdship , S. Viti , T. J. Haworth , J. D. Ilee