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Quantum spin liquids have been at the forefront of correlated electron research ever since their original proposal in 1973, and the realization that they belong to the broader class of intrinsic topological orders, along with the fractional…

Strongly Correlated Electrons · Physics 2018-04-26 Ioannis Rousochatzakis , Yuriy Sizyuk , Natalia B. Perkins

A quantum spin liquid (QSL) arises from a highly entangled superposition of many degenerate classical ground states in a frustrated magnet, and is characterized by emergent gauge fields and deconfined fractionalized excitations (spinons).…

Strongly Correlated Electrons · Physics 2025-06-24 Bin Gao , Félix Desrochers , David W. Tam , Paul Steffens , Arno Hiess , Yixi Su , Sang-Wook Cheong , Yong Baek Kim , Pengcheng Dai

Spin liquids are exotic phases of quantum matter challenging Landau's paradigm of symmetry-breaking phase transitions. Despite strong exchange interactions, spins do not order or freeze down to zero temperature. While well-established for…

Strongly Correlated Electrons · Physics 2020-04-22 P. Khuntia , M. Velazquez , Q. Barthélemy , F. Bert , E. Kermarrec , A. Legros , B. Bernu , L. Messio , A. Zorko , P. Mendels

The "spin ice" state found in the rare earth pyrochlore magnets Ho2Ti2O7 and Dy2Ti2O7 offers a beautiful realisation of classical magnetostatics, complete with magnetic monopole excitations. It has been suggested that in "quantum spin ice"…

Strongly Correlated Electrons · Physics 2015-06-04 Owen Benton , Olga Sikora , Nic Shannon

Conventional wisdom dictates that quantum effects become unimportant at high temperatures. In magnets, when the thermal energy exceeds interactions between atomic magnetic moments, the moments are usually uncorrelated, and classical…

$\rm{Sr_2CuTe_{0.5}W_{0.5}O_6}$ is a square-lattice magnet with super-exchange between S=1/2 $\rm{Cu^{2+}}$ spins mediated by randomly distributed Te and W ions. Here, using sub-K temperature and 20 $\rm{\mu}$eV energy resolution neutron…

Quantum fluctuations are expected to lead to highly entangled spin-liquid states in certain two-dimensional spin-1/2 compounds. We have synthesized and measured thermodynamic properties and muon spin relaxation rates in the copper-based…

Quantum spin liquids (QSL) have generated considerable excitement as phases of matter with emergent gauge structures and fractionalized excitations. In this context, phase transitions out of QSLs have been widely discussed as Higgs…

Strongly Correlated Electrons · Physics 2021-09-15 Hyeok-Jun Yang , Nic Shannon , SungBin Lee

At low temperatures, a spin ice enters a Coulomb phase - a state with algebraic correlations and topologically constrained spin configurations. In Ho2Ti2O7, we have observed experimentally that this process is accompanied by a non-standard…

Quantum spin liquids (QSLs) are fluid-like states of quantum spins where its long-range ordered state is destroyed by quantum fluctuations. The ground state of QSL and its exotic phenomena, which have been extensively discussed for decades,…

Strongly Correlated Electrons · Physics 2011-10-25 Minoru Yamashita , Takasada Shibauchi , Yuji Matsuda

This article is an introductory review of the physics of quantum spin liquid (QSL) states. Quantum magnetism is a rapidly evolving field, and recent developments reveal that the ground states and low-energy physics of frustrated spin…

Strongly Correlated Electrons · Physics 2017-04-21 Yi Zhou , Kazushi Kanoda , Tai-Kai Ng

Quantum spin liquids are exotic phases of matter whose low-energy physics is described as the deconfined phase of an emergent gauge theory. With recent theory proposals and an experiment showing preliminary signs of $\mathbb{Z}_2$…

Quantum Gases · Physics 2025-04-14 Jeet Shah , Gautam Nambiar , Alexey V. Gorshkov , Victor Galitski

We use numerical linked cluster (NLC) expansions to compute the specific heat, C(T), and entropy, S(T), of a quantum spin ice model of Yb2Ti2O7 using anisotropic exchange interactions recently determined from inelastic neutron scattering…

Strongly Correlated Electrons · Physics 2012-10-11 R. Applegate , N. R. Hayre , R. R. P. Singh , T. Lin , A. G. R. Day , M. J. P. Gingras

Neutron scattering experiments on a polycrystalline sample of the frustrated pyrochlore magnet Tb2Ti2O7, which does not show any magnetic order down to 50 mK, have revealed that it shows condensation behavior below 0.4 K from a thermally…

Disordered Systems and Neural Networks · Physics 2011-12-13 Hiroshi Takatsu , Hiroaki Kadowaki , Taku J. Sato , Jeffrey W. Lynn , Yoshikazu Tabata , Teruo Yamazaki , Kazuyuki Matsuhira

The long-sought quantum spin liquid is a quantum-entangled magnetic state leading to the fractionalization of spin degrees of freedom. Quasiparticles emergent from the fractionalization affect not only the ground state properties but also…

Strongly Correlated Electrons · Physics 2017-09-06 Junki Yoshitake , Joji Nasu , Yukitoshi Motome

While phase transitions between magnetic analogs of three states of matter --- a long-range ordered state, paramagnet, and spin liquid --- have been extensively studied, the possibility of "liquid-liquid" transitions, namely, between…

Strongly Correlated Electrons · Physics 2017-04-05 Joji Nasu , Yasuyuki Kato , Junki Yoshitake , Yoshitomo Kamiya , Yukitoshi Motome

Topological phases of spin liquids with constrained disorder can host a kinetics of fractionalized excitations. However, spin-liquid phases with distinct kinetic regimes have proven difficult to observe experimentally. Here we present a…

The quantum antiferromagnet on the pyrochlore lattice offers an archetypal frustrated system, which potentially realizes a quantum spin liquid characterized by the absence of standard spontaneous symmetry breaking even at zero temperature,…

Strongly Correlated Electrons · Physics 2023-11-21 Rico Pohle , Youhei Yamaji , Masatoshi Imada

Electronic spins can form long-range entangled phases of condensed matter named quantum spin liquids. Their existence is conceptualized in models of two- or three-dimensional frustrated magnets that evade symmetry-breaking order down to…

Artificial spin ices are frustrated spin systems that can be engineered, wherein fine tuning of geometry and topology has allowed the design and characterization of exotic emergent phenomena at the constituent level. Here we report a…