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Mid-infrared (mid-IR) spectroscopy provides a way to study structures and dynamics of complicated molecules in condensed phases. Therefore, developing compact and broadband mid-IR spectrometer has been a long-standing challenge. Here, we…
Two semiconductor optical frequency combs consuming less than 1 W of electrical power are used to demonstrate high-sensitivity mid-infrared dual-comb spectroscopy in the important 3-4 $\mu$m spectral region. The devices are 4 millimeters…
We present a versatile mid-infrared frequency comb spectroscopy system based on a doubly resonant optical parametric oscillator tunable in the 3-5.4 {\mu}m range and two detection methods, a Fourier transform spectrometer (FTS) and a…
Infrared spectroscopy is a powerful tool for basic and applied science. The molecular spectral fingerprints in the 3 um to 20 um region provide a means to uniquely identify molecular structure for fundamental spectroscopy, atmospheric…
While mid-infrared radiation can be used to identify and quantify numerous chemical species, contemporary broadband mid-IR spectroscopic systems are often hindered by large footprints, moving parts and high power consumption. In this work,…
Cavity-enhanced direct frequency comb spectroscopy combines broad spectral bandwidth, high spectral resolution, precise frequency calibration, and ultrahigh detection sensitivity, all in one experimental platform based on an optical…
Dual-frequency comb spectroscopy has emerged as a disruptive technique for measuring wide-spanning spectra with high resolution, yielding a particularly powerful technique for sensitive multi-component gas analysis. We present a…
We demonstrate a compact continuous-wave single-frequency doubly-resonant optical parametric oscillator (DRO) in a double-pass pump configuration with a control of the relative phase between the reflected waves. The nested DRO cavity allows…
Breath analysis enables rapid, non-invasive diagnostics, as well as long-term monitoring, of human health through the identification and quantification of exhaled biomarkers. Here, for the first time, we demonstrate the remarkable…
Electro-optic frequency combs were employed to rapidly interrogate an optomechanical sensor, demonstrating spectral resolution substantially exceeding that possible with a mode-locked frequency comb. Frequency combs were generated using an…
We demonstrate coherent dual frequency-comb spectroscopy for detecting variations in greenhouse gases. High signal-to-noise spectra are acquired spanning 5990 to 6260 cm^-1 (1600 to 1670 nm) covering ~700 absorption features from CO2, CH4,…
We present the detection of molecular oxygen with Odin toward the dense molecular core rho Oph A, which is part of a region of active star formation. The observed spectral line is the (N,J = 1,1-1,0) ground state transition of molecular…
We report a photoacoustic spectroscopy setup with a high-power mid-infrared frequency comb as the light source. The setup is used in broadband spectroscopy of radiocarbon methane. Due to the high sensitivity of a cantilever-enhanced…
We report a femtosecond optical parametric oscillator (OPO) based on the new semiconductor gain material orientation patterned gallium phosphide (OP-GaP), which enables the production of high-repetition-rate femtosecond pulses spanning 5-12…
Molecular spectroscopy in the mid-infrared portion of the electromagnetic spectrum (3--25 um) has been a cornerstone interdisciplinary analytical technique widely adapted across the biological, chemical, and physical sciences. Applications…
We report on a comb-locked cavity ring-down spectrometer developed for high-precision, SI-traceable, molecular spectroscopy of air-broadened CO2 gas samples. The experimental setup relies on the use of a singly-resonant optical parametric…
Glyoxal CHOCHO is a trace gas in the atmosphere, often used as an indicator of biogenic emissions. It is frequently compared to formaldehyde concentrations, which serve as indicators of anthropogenic emissions, to gain insights into the…
We measure the fluorescence spectrum of broadband emitters in an open optical microcavity with radius of curvature R = 17.7(3) um and finesse F ~= 1000. This geometry enables a combined measurement of emission spectra versus cavity length,…
We use optical frequency comb Fourier transform spectroscopy to measure high-resolution spectra of iodomethane, CH$_3$I in the C-H stretch region from 2800 to 3160 cm$^{-1}$. The fast-scanning Fourier transform spectrometer with…
Developing compact, broadband mid-infrared coherent sources for applications in spectroscopy and sensing remains a pressing challenge in photonics. However, material limitations and integration constraints have restricted the accessible…