Related papers: On the Saturation of the Nonlinear Refractive Inde…
The higher-order Kerr effect (HOKE) has been recently advocated to explain measurements of the saturation of the nonlinear refractive index in gases. Here we show that cascaded third-harmonic generation results in an effective fifth order…
Br\'ee, Demircan, and Steinmeyer [Phys. Rev. Lett. 106, 183902 (2011)] recently calculated higher-order Kerr effect (HOKE) coefficients using the nonlinear Kramers-Kronig relations. We show that the saturated and negative nonlinear index of…
According to a recent experiment, the instantaneous electronic Kerr effect in air exhibits a strong intensity dependence, the nonlinear refractive index switching sign and crossing over from a self-focusing to a de-focusing nonlinearity. A…
We demonstrate that Freeman resonances have a strong impact on the nonlinear optical response in femtosecond filaments. These resonances decrease the transient refractive index within a narrow intensity window and strongly affect the…
The recent measurement of negative higher-order Kerr effect (HOKE) terms in gases has given rise to a controversial debate, fed by its impact on short laser pulse propagation. By comparing the experimentally measured yield of the third and…
As a contribution to the ongoing controversy about the role of higher-order Kerr effect (HOKE) in laser filamentation, we first provide thorough details about the protocol that has been employed to infer the HOKE indices from the…
We test numerical filamentation models against experimental data about the peak intensity and filament density in laser filaments. We show that the consideration of the higher-order Kerr effect (HOKE) improves the quantitative agreement…
We investigate numerically the propagation and the Anderson localization of plane waves in a one-dimensional lattice chain, where disorder and saturable nonlinearity are simultaneously present. Using a calculation scheme for solving the…
We report a novel experimental technique to investigate ultrafast dynamics in photoexcited molecules by probing the third-order nonlinear optical susceptibility. A non-colinear 3-pulse scheme is developed to probe the ultrafast dynamics of…
While filaments are generally interpreted as a dynamic balance between Kerr focusing and plasma defocusing, the role of the higher-order Kerr effect (HOKE) is actively debated as a potentially dominant defocusing contribution to filament…
Polarization dependence on clamping intensity inside femtosecond filament was experimentally measured in air. By tuning the laser pulse ellipse from linear polarization to circular polarization, the measured clamping intensity inside laser…
We find the atomic response to the intense femtosecond laser pulse via solving numerically the three-dimensional non-stationary Schr\"odinger equation (TDSE) for a model atom and calculating its dipole moment. For weak quasi-static fields,…
We develop an approach describing nonlinear-optical processes in the strong-field domain characterized by the nonperturbative field-with-matter interaction. The polarization of an isolated atom in the external field calculated via the…
We numerically investigate the conical emission (CE) from ultrashort laser filaments, both considering and disregarding the higher-order Kerr effect (HOKE). While the consideration of HOKE has almost no influence on the predicted CE from…
The axial dependence of femtosecond filamentation in air is measured under conditions of varying laser pulsewidth, energy, and focusing f-number. Filaments are characterized by the ultrafast z-dependent absorption of energy from the laser…
An electrodynamic response of graphene to a strong electromagnetic radiation is considered. A hot electron model (HEM) is introduced and a corresponding system of nonlinear equations is formulated. Solutions of this system are found and…
A study is made of the saturation mechanism of a single superradiant spike of radiation in a Free Electron Laser. A one-dimensional (1D) computer model is developed using the Puffin, un-averaged FEL simulation code, which allows…
Using Time-Dependent Density Functional Theory (TDDFT) nonlinear nonperturbative response of the molecular system is studied for photoisomerization reaction. The 1,3-cyclohexadiene photoisomerization is probed by the high-harmonic…
A theoretical calculation is performed for the ultrafast spin dynamics in nickel using an exact diagonalization method. The present theory mainly focuses on a situation where the intrinsic charge and spin dynamics is probed by the nonlinear…
We directly measure the nonlinear optical response in argon and nitrogen in a thin gas target to laser intensities near the ionization threshold. No instantaneous negative nonlinear refractive index is observed, nor is saturation, in…