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In our review we focus on the quantum spin liquid, defining the thermodynamic, transport and relaxation properties of geometrically frustrated magnets (insulators) represented by herbertsmithite $\rm ZnCu_{3}(OH)_6Cl_2$.

Strongly Correlated Electrons · Physics 2019-08-29 V. R. Shaginyan , A. Z. Msezane , M. Ya. Amusia , J. W. Clark , G. S. Japaridze , V. A. Stephanovich , Y. S. Leevik

Quantum spin liquids (QSLs) host a variety of fractionalized particles. In Kitaev's paradigmatic honeycomb model a spin-$\tfrac{1}{2}$ fractionalizes into $Z_2$ flux due to emergent $Z_2$ gauge field and matter Majorana fermions. Although…

Strongly Correlated Electrons · Physics 2026-01-22 Shi Feng , Nandini Trivedi

A quantum spin liquid is a novel ground state that can support long-range entanglement between magnetic moments, resulting in exotic spin excitations involving fractionalized $S=\frac{1}{2}$ spinons. Here, we measure the excitations in…

Pursuing the exotic quantum spin liquid (QSL) state in the Kitaev material $\alpha$-RuCl$_3$ has intrigued great research interest recently. A fascinating question is on the possible existence of field-induced QSL phase in this compound.…

Strongly Correlated Electrons · Physics 2023-09-14 Xu-Guang Zhou , Han Li , Yasuhiro H. Matsuda , Akira Matsuo , Wei Li , Nobuyuki Kurita , Gang Su , Koichi Kindo , Hidekazu Tanaka

Finding distinct signatures of a quantum spin liquid (QSL) is an ongoing quest in condensed matter physics, invariably complicated by the presence of disorder in real materials. In this regard the 2D Kagome system…

Strongly Correlated Electrons · Physics 2024-01-22 B. S. Shivaram , J. Prestigiacomo , Aini Xu , Zhenyuan Zeng , Trevor D. Ford , Itamar Kimchi , Shiliang Li , Patrick A. Lee

The pursuit of quantum spin liquid (QSL) in the Kitaev honeycomb magnets has drawn intensive attention recently. In particular, $\alpha$-RuCl$_3$ has been widely recognized as a promising candidate for the Kitaev QSL. Although the compound…

Strongly Correlated Electrons · Physics 2023-03-29 Han Li , Wei Li , Gang Su

The search for Kitaev's quantum spin liquid (KQSL) state in real materials has recently expanded with the prediction that honeycomb lattices of divalent, high-spin cobalt ions could host the dominant bond-dependent exchange interactions…

Despite tremendous investigations, a quantum spin liquid state realized in spin-1/2 kagome Heisenberg antiferromagnet remains largely elusive. In herbertsmithite ZnCu$_3$(OH)$_6$Cl$_2$, a quantum spin liquid candidate on the perfect kagome…

Strongly Correlated Electrons · Physics 2021-06-15 H. Murayama , T. Tominaga , T. Asaba , A. de Oliveira Silva , Y. Sato , H. Suzuki , Y. Ukai , S. Suetsugu , Y. Kasahara , R. Okuma , I. Kimchi , Y. Matsuda

The spin-$\frac{1}{2}$ kagome antiferromagnet is considered an ideal host for a quantum spin liquid ground state. We find that when the bonds of the kagome lattice are modulated with a periodic pattern, new quantum ground states emerge.…

At sufficiently low temperatures, condensed-matter systems tend to develop order. An exception are quantum spin-liquids, where fluctuations prevent a transition to an ordered state down to the lowest temperatures. While such states are…

Strongly Correlated Electrons · Physics 2010-04-15 Z. Y. Meng , T. C. Lang , S. Wessel , F. F. Assaad , A. Muramatsu

New physics can emerge in magnetic materials where quantum fluctuations are enhanced due to reduced dimensionality and strong frustration. One long sought example is the resonating-valence-bond (RVB) state, where atomic magnetic moments are…

Strongly Correlated Electrons · Physics 2013-07-19 Tian-Heng Han , Joel S. Helton , Shaoyan Chu , Daniel G. Nocera , Jose A. Rodriguez-Rivera , Collin Broholm , Young S. Lee

Unambiguous identification of the Kitaev quantum spin liquid (QSL) in materials remains a huge challenge despite many encouraging signs from various measurements. To facilitate the experimental detection of the Kitaev QSL, here we propose…

Strongly Correlated Electrons · Physics 2023-05-24 Saikat Banerjee , Shi-Zeng Lin

A quantum spin liquid (QSL) is a novel phase of matter with long-range entanglement where localized spins are highly correlated with the vanishing of magnetic order. Such exotic quantum states provide the opportunities to develop new…

Strongly Correlated Electrons · Physics 2022-09-21 Wen-Yuan Liu , Juraj Hasik , Shou-Shu Gong , Didier Poilblanc , Wei-Qiang Chen , Zheng-Cheng Gu

Strongly correlated Fermi systems are among the most intriguing and fundamental systems in physics. We show that the herbertsmithite ZnCu3(OH)6Cl2 can be viewed as a new type of strongly correlated electrical insulator that possesses…

Strongly Correlated Electrons · Physics 2013-06-24 V. R. Shaginyan , K. G. Popov , V. A. Khodel

The Kitaev quantum spin liquid (QSL) on the two-dimensional honeycomb lattice epitomizes an entangled topological state, where the spins fractionalize into Majorana fermions. This state has aroused tremendous interest because it harbors…

Strongly Correlated Electrons · Physics 2022-12-12 S. Suetsugu , Y. Ukai , M. Shimomura , M. Kamimura , T. Asaba , Y. Kasahara , N. Kurita , H. Tanaka , T. Shibauchi , J. Nasu , Y. Motome , Y. Matsuda

The spiral spin liquid (SSL) is a highly degenerate state characterized by a continuous contour or surface in reciprocal space spanned by a spiral propagation vector. Although the SSL state has been predicted in a number of various…

Barlowite $Cu_4(OH)_6FBr$ is a newly found mineral containing $Cu^{2+}$ kagome planes. Despite similarities in many aspects to Herbertsmithite $Cu_3Zn(OH)_6Cl_2$, the well-known quantum spin liquid (QSL) candidate, intrinsic Barlowite turns…

Materials Science · Physics 2015-12-23 Zheng Liu , Xiaolong Zou , Jia-Wei Mei , Feng Liu

Quantum Spin Liquids (QSLs) are phases of interacting spins that do not order even at the absolute zero temperature, making it impossible to characterize them by a local order parameter. In this article, we review the unique view provided…

Strongly Correlated Electrons · Physics 2013-02-06 Tarun Grover , Yi Zhang , Ashvin Vishwanath

Alpha-phase (a-) RuCl_3 has emerged as a prime candidate for a quantum spin liquid (QSL) that promises exotic quasiparticles relevant for fault-tolerant quantum computation. Here, we report spin sensitive transport measurements to probe…

Strongly Correlated Electrons · Physics 2026-04-27 H. Idzuchi , M. Kimata , S. Okamoto , P. Laurell , N. Mohanta , M. Cothrine , S. E. Nagler , D. Mandrus , A. Banerjee , Y. P. Chen

We report the structural transformation of hexagonal Ba3YIr2O9 to a cubic double perovskite form (stable in ambient conditions) under an applied pressure of 8GPa at 1273K. While the ambient pressure (AP) synthesized sample undergoes…

Strongly Correlated Electrons · Physics 2013-10-28 Tusharkanti Dey , A. V. Mahajan , R. Kumar , B. Koteswararao , F. C. Chou , A. A. Omrani , H. M. Ronnow