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Detecting and controlling nuclear spin nano-ensembles is crucial for the further development of nuclear magnetic resonance (NMR) spectroscopy and for the emerging solid state quantum technology. Here we present the fabrication of a…

This study investigates spin squeezed states in nuclear magnetic resonance (NMR) quadrupolar systems with spins $I=3/2$ and $I=7/2$ at room temperature, taking into account the effects of relaxation on the dynamics. The origin of spin…

Nuclear magnetic resonance (NMR) is a powerful tool for applications ranging from chemical analysis to quantum information processing. Achieving optical initialization and detection of molecular nuclear spins promises new opportunities -…

We have characterized spin-squeezed states produced at a temperature of $26^\circ{\mathrm C}$ on a Nuclear Magnetic Resonance (NMR) quadrupolar system. The implementation is carried out in an ensemble of $^{133}$Cs nuclei with spin $I=7/2$…

Coherent oscillations between any two levels from four nuclear spin states of I=3/2 have been demonstrated in a nanometre-scale NMR semiconductor device, where nuclear spins are all-electrically controlled. Using this device, we discuss…

Quantum Physics · Physics 2009-08-04 S. K. Ozdemir , A. Miranowicz , T. Ota , G. Yusa , N. Imoto , Y. Hirayama

We analyze a quantum computer (QC) design based on nuclear spin qubits in a quasi-one-dimensional (1D) chain of non-Kramers doublet atoms. We explore the use of spatial symmetry breaking to obtain control over the local dynamics of a qubit.…

Other Condensed Matter · Physics 2009-11-10 E. Novais , A. H. Castro Neto

Spin cat states are superpositions of two or more coherent spin states (CSSs) that are distinctly separated over the Bloch sphere. Additionally, the nuclei with angular momenta greater than 1/2 possess a quadrupolar charge distribution. At…

Quantum Physics · Physics 2017-08-08 Ceyhun Bulutay

Nuclear spins are highly coherent quantum objects. In large ensembles, their control and detection via magnetic resonance is widely exploited, e.g. in chemistry, medicine, materials science and mining. Nuclear spins also featured in early…

Spin defects in solids, such as the nitrogen-vacancy (NV) center in diamond, have emerged as a key tool for detecting nuclear spins at the nanoscale. While active nuclear spin control via radio-frequency (RF) irradiation is often…

Electron spins in quantum dots under coherent control exhibit a number of novel feedback processes. Here, we present experimental and theoretical evidence of a feedback process between nuclear spins and a single electron spin in a single…

We propose a new approach to the measurement of a single spin state, based on nuclear magnetic resonance (NMR) techniques and inspired by the coherent control over many-body systems envisaged by Quantum Information Processing (QIP). A…

We theoretically consider solid state nuclear spins in a semiconductor nanostructure environment as long-lived, high-fidelity quantum memory. In particular, we calculate, in the limit of a strong applied magnetic field, the fidelity versus…

Mesoscale and Nanoscale Physics · Physics 2009-11-13 W. M. Witzel , S. Das Sarma

This paper surveys our recent research on quantum information processing by nuclear magnetic resonance (NMR) spectroscopy. We begin with a geometric introduction to the NMR of an ensemble of indistinguishable spins, and then show how this…

Quantum Physics · Physics 2007-05-23 T. F. Havel , S. S. Somaroo , C. -H. Tseng , D. G. Cory

Spin/magnetisation relaxation and coherence times, respectively T_1 and T_2, initially defined in the context of nuclear magnetic resonance (NMR), are general concepts applicable to a wide range of systems, including quantum bits [1-4]. At…

Superconductivity · Physics 2015-11-10 C. H. L. Quay , Y. Chiffaudel , C. Strunk , M. Aprili

We investigate numerically the Multiple Quantum (MQ) NMR dynamics in systems of nuclear spins 1/2 coupled by the dipole-dipole interactions in the case of the pseudopure initial state. Simulations of the MQ NMR with the real molecular…

Other Condensed Matter · Physics 2009-11-13 G. B. Furman

We have developed semiconductor point contact devices in which nuclear spins in a nanoscale region are coherently controlled by all-electrical methods. Different from the standard nuclear-magnetic resonance technique, the longitudinal…

Quantum Physics · Physics 2009-11-13 Y. Hirayama , A. Miranowicz , T. Ota , G. Yusa , K. Muraki , S. K. Ozdemir , N. Imoto

Zero-field nuclear magnetic resonance (NMR) provides complementary analysis modalities to those of high-field NMR and allows for ultra-high-resolution spectroscopy and measurement of untruncated spin-spin interactions. Unlike for the…

Quantum Physics · Physics 2022-03-01 Min Jiang , Teng Wu , John W. Blanchard , Guanru Feng , Xinhua Peng , Dmitry Budker

The nuclear spin, being much more isolated from the environment than its electronic counterpart, enables quantum experiments with prolonged coherence times and presents a gateway towards uncovering the intricate dynamics within an atom.…

Mesoscale and Nanoscale Physics · Physics 2023-09-08 Lukas M. Veldman , Evert W. Stolte , Mark P. Canavan , Rik Broekhoven , Philip Willke , Laëtitia Farinacci , Sander Otte

We implement several non-binary logic systems using the spin dynamics of nuclear spins in nuclear magnetic resonance (NMR). The NMR system is a suitable test system because of its high degree of experimental control; findings from NMR…

Emerging Technologies · Computer Science 2015-12-03 Pedro M. Aguiar , Robert Hornby , Cameron McGarry , Simon O'Keefe , Angelika Sebald

Pulsed magnetic resonance is a wide-reaching technology allowing the quantum state of electronic and nuclear spins to be controlled on the timescale of nanoseconds and microseconds respectively. The time required to flip either dilute…

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