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We investigate optical second-harmonic generation (SHG) from metasurfaces where noncentrosymmetric V-shaped gold nanoparticles are ordered into regular array configurations. In contrast to expectations, a substantial enhancement of the SHG…

We theoretically demonstrate x-ray second harmonic generation (SHG) with strong-field-driven high harmonic generation (HHG) from core electrons in gas-phase atoms, highlighting its potential as a powerful spectroscopic tool for studying…

Atomic Physics · Physics 2025-03-31 Xinhua Xie

Optical-field sampling using second-harmonic generation (SHG) from strong-field ionization enables ultrabroadband terahertz detection, but the microscopic origin of the SHG signal and its ultrabroadband response have been unclear. Here we…

We demonstrate a simple and scalable approach to increase conversion efficiencies of nonlinear metasurfaces by incorporating them into multipass cells and by letting the pump beam to interact with the metasurfaces multiple times. We…

We demonstrate phase-matched second-harmonic generation (SHG) from three-dimensional metamaterials consisting of stacked metasurfaces. To achieve phase matching, we utilize a novel mechanism based on phase engineering of the metasurfaces at…

The resonance effects on the optical second harmonic generation from 140 nm silver nanoparticles is studied experimentally by hyper-Rayleigh scattering and numerically by finite element method calculations. We find that the interferences…

In the currently accepted models of the nonlinear optics, the nonlinear radiation was treated as the result of an infinitesimally thin polarization sheet layer, and a three layer model was generally employed. The direct consequence of this…

Chemical Physics · Physics 2016-08-29 De-sheng Zheng , Yuan Wang , An-an Liu , Hong-fei Wang

The second harmonic generation is one of the most important applications of nonlinear effect, which has attracted great interests in nonlinear optics and microwave in the past decades. To the best of our knowledge, however, generating the…

A computational method for the scattering of light by multiple nonclassical plasmonic nanospheres, each of which has multiple (non-)concentric dielectric or metallic layers, is presented. The electromagnetic (EM) response of the free…

Computational Physics · Physics 2025-09-08 Xin Zheng , Christos Mystilidis , Christos Tserkezis , Guy A. E. Vandenbosch , Xuezhi Zheng

Directional harmonic generation is an important property characterizing the ability of nonlinear optical antennas to diffuse the signal in well-defined region of space. Herein, we show how sub-wavelength facets of an organic molecular…

We present a novel spectroscopic technique for second harmonic generation (SHG) using femtosecond laser pulses at 30~kHz repetition rate, which nevertheless provides high spectral resolution limited only by the spectrometer. The potential…

Second harmonic generation (SHG) is prohibited in centrosymmetric crystals such as silicon or germanium due to the presence of inversion symmetry. However, the structuring of such materials makes it possible to break the inversion symmetry,…

Electromagnetic wave scattering from planar dielectric films deposited on one-dimensional, randomly rough, perfectly conducting substrates is studied by numerical simulations for both p- and s-polarization. The reduced Rayleigh equation,…

Condensed Matter · Physics 2024-03-25 I. Simonsen , A. A. Maradudin

We present Floquet calculations of high harmonic generation (HHG) for the lowest two electronic states of the $\mbox{H}_2^+$ ion by strong continuous-wave laser fields. We solve the non-Hermitian matrix problem to get accurate solutions to…

Atomic Physics · Physics 2015-06-18 Ts Tsogbayar , M Horbatsch

Optical second harmonic generation (SHG) is studied from multilayer graphene films in the presence of DC electric current flowing in the sample plane. Graphene layers are manufactured by chemical vapour deposition (CVD) technique and…

Mesoscale and Nanoscale Physics · Physics 2015-06-04 Anton Y. Bykov , Tatiana V. Murzina , Maxim G. Rybin , Elena D. Obraztsova

We present HELIOS (HomogEneous and Layered medIa Optical Scattering), an open-source surface integral equation (SIE) software designed for modeling light scattering by particles embedded in homogeneous or layered media and periodic…

Optics · Physics 2026-02-27 Parmenion S. Mavrikakis , Olivier J. F. Martin

We introduce a new concept of split-ball resonator and demonstrate a strong magnetic dipole response for both gold and silver spherical plasmonic nanoparticles with nanometer-scale cuts. Tunability of the magnetic dipole resonance…

I present a direct and intuitive eigenmode method that evaluates the near-field enhancement around the surface of metallic nanoparticles of arbitrary shape. The method is based on the boundary integral equation in the electrostatic limit.…

Mesoscale and Nanoscale Physics · Physics 2013-05-30 Titus Sandu

It is found that for objects possessing small surface structures with differing radii of curvature the secondary electron emission (SEE) yield may be significantly higher than for objects with smooth surfaces of the same material. The…

Mesoscale and Nanoscale Physics · Physics 2016-05-03 A. R. Dzhanoev , F. Spahn , V. Yaroshenko , H. Lühr , J. Schmidt

Super-resolution microscopy in the visible is an established powerful tool in several disciplines. In the infrared (IR) spectral range, however, no comparable schemes have been demonstrated to date. In this work, we experimentally…