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We analyze the role of coherent, non-perturbative system-bath interactions in a photosynthetic heat engine. Using the reaction-coordinate formalism to describe the vibrational phonon-environment in the engine, we analyze the efficiency…

Chemical Physics · Physics 2018-09-19 Melina Wertnik , Alex Chin , Franco Nori , Neill Lambert

Experimental/theoretical evidence for sustained vibration-assisted electronic (vibronic) coherence in the Photosystem II Reaction Center (PSII RC) indicates that photosynthetic solar-energy conversion might be optimized through the…

Timing requirements for long-range quantum networking are driven by the necessity of synchronizing the arrival of photons, from independent sources, for Bell-state measurements. Thus, characteristics such as repetition rate and pulse…

Quantum Physics · Physics 2023-07-03 Randy Lafler , R. Nicholas Lanning

The work is devoted to the investigation of the influence of a heat bath on the physical processes in a quantum system. We use the density matrix theory as one of the most powerfool tool for investigation of quantum relaxation. In the…

Quantum Physics · Physics 2007-05-23 Dmitri S. Kilin

Noise is widely understood to be something that interferes with a signal or process. Thus, it is generally thought to be destructive, obscuring signals and interfering with function. However, early in the 20th century, mechanical engineers…

Biological Physics · Physics 2019-06-10 Steven Weinstein , Theodore P. Pavlic

Transport phenomena on a quantum scale appear in a variety of systems, ranging from photosynthetic complexes to engineered quantum devices. It has been predicted that the efficiency of quantum transport can be enhanced through dynamic…

It is shown that quantum sustainability is a universal phenomenon which emerges during environment-assisted electronic excitation energy transfer (EET) in photobiological complexes (PBCs), such as photosynthetic reaction centers and centers…

Biological Physics · Physics 2018-07-09 Konstantin G. Zloshchastiev

At low temperatures when the phonon modes are effectively frozen, photon transport is the dominating mechanism of thermal relaxation in metallic systems. Starting from a microscopic many-body Hamiltonian, we develop a nonequilibrium Green's…

Mesoscale and Nanoscale Physics · Physics 2009-11-13 Teemu Ojanen , Tero T. Heikkila

Photosystem II (PSII) reaction center is a unique protein-chromophore complex that is capable of efficiently separating electronic charges across the membrane after photoexcitation. In the PSII reaction center, the primary energy- and…

Charge transfer is a fundamental process that underlies a multitude of phenomena in chemistry and biology. Recent advances in observing and manipulating charge and heat transport at the nanoscale, and recently developed techniques for…

Mesoscale and Nanoscale Physics · Physics 2016-07-26 Galen T. Craven , Abraham Nitzan

We describe a method for simulating exciton dynamics in protein-pigment complexes, including effects from charge transfer as well as fluorescence. The method combines the hierarchical equations of motion, which are used to describe quantum…

Chemical Physics · Physics 2022-11-23 Thomas P. Fay , David T. Limmer

Understanding energy dissipation and transport in nanoscale structures is of great importance for the design of energy-efficient circuits and energy-conversion systems. This is also a rich domain for fundamental discoveries at the…

Mesoscale and Nanoscale Physics · Physics 2010-03-23 Eric Pop

Under nonequilibrium conditions, quantum optical systems reveal unusual properties that might be distinct from those in condensed matter. The fundamental reason is that photonic eigenstates can have arbitrary occupation numbers, whereas in…

Quantum Physics · Physics 2021-07-06 Dmitriy S. Shapiro

In this article, a low noise amplifier is quantum mechanically analyzed to study the behavior of the noise figure. The analysis view is changed from the classic to quantum, because using quantum theory produces some degrees of freedom,…

Quantum Physics · Physics 2021-08-12 Ahmad Salmanogli

Photons excited into ground state modes at finite temperature display partitioning among photon phases, lifetimes and distances travelled since creation. These distributions set the distance from an interface a created photon has some…

Optics · Physics 2022-04-28 Geoff B Smith , Angus R Gentle , Matthew D Arnold

The Wigner-Weisskopf-type model describing the energy transfer between two centers mediated by a continuum of energy levels is studied. This work is motivated by the recent interest in transport phenomena at nanoscale in biology and quantum…

Quantum Physics · Physics 2015-05-27 Robert Alicki , Filippo Giraldi

Efficient energy transport is highly desirable for organic semiconductor (OSC) devices such as photovoltaics, photodetectors, and photocatalytic systems. However, photo-generated excitons in OSC films mostly occupy highly localized states…

Photosynthetic organisms harvest light energy, utilizing the absorption and energy transfer properties of protein-bound chromophores. Controlling the harvesting efficiency is critical for the optimal function of the photosynthetic…

We analyze the problem of directed quantum transport induced by external exponentially correlated telegraphic noise. In addition to quantum nature of the heat bath, nonlinearity of the periodic system potential brings in quantum…

Statistical Mechanics · Physics 2007-05-23 Pulak Kumar Ghosh , Debashis Barik , Deb Shankar Ray

Research into the efficiency of photosynthetic light harvesting has focused on two factors: (1) entanglement of chromophores, and (2) environmental noise. While chromophores are conjugated $\pi$-bonding molecules with strongly correlated…

Biological Physics · Physics 2013-03-29 David A. Mazziotti