Related papers: Third harmonic generation in graphene and few-laye…
Graphene is a nonlinear material which can be used as a saturable absorber, frequency mixer and frequency multiplier. We investigate the third harmonic generation from graphene lying on different substrates, consisting of a dielectric…
Optical harmonic generation occurs when high intensity light ($>10^{10}$W/m$^{2}$) interacts with a nonlinear material. Electrical control of the nonlinear optical response enables applications such as gate-tunable switches and frequency…
Due to its linear dispersion, monolayer graphene is expected to generate a third harmonic response at terahertz frequencies. There have been a variety of different models of this effect and recently it has been experimentally observed.…
The nonlinear responses of different materials provide useful mechanisms for optical switching, low noise amplification, and harmonic frequency generation. However, the nonlinear processes usually have an extremely weak nature and require…
Graphene as a zero-bandgap two-dimensional semiconductor with a linear electron band dispersion near the Dirac points has the potential to exhibit very interesting nonlinear optical properties. In particular, third harmonic generation of…
Graphene was shown to have strongly nonlinear electrodynamic properties. In particular, being irradiated by an electromagnetic wave with the frequency $\omega$, it can efficiently generate higher frequency harmonics. Here we predict that in…
We present perturbation theory for analysis of generic third-order nonlinear processes in graphene integrated photonic structures. Optical response of graphene is treated as the nonlinear boundary condition in Maxwell equations. The derived…
We report strong third-harmonic generation (THG) in monolayer graphene grown by chemical vapor deposition (CVD) and transferred to an amorphous silica (glass) substrate; the photon energy is in three-photon resonance with the…
A quantum theory of the third-harmonic generation in graphene is presented. An analytical formula for the nonlinear conductivity tensor $\sigma^{(3)}_{\alpha\beta\gamma\delta}(\omega,\omega,\omega)$ is derived. Resonant maxima of the third…
We consider the linear and nonlinear response of a weighted graphene sheet under the normal incidence of a plane electromagnetic wave in the form of a quasi-monochromatic pulse of long duration with a sharp edge and harmonic filling. The…
The linear energy dispersion of graphene electrons leads to a strongly nonlinear electromagnetic response of this material. We develop a general quantum theory of the third-order nonlinear local dynamic conductivity of graphene…
Synthesis of graphene with reduced use of chemical reagents is essential for manufacturing scale-up and to control its structure and properties. In this paper, we report on a novel chemical-free mechanism of graphene exfoliation from…
We present the first experimental investigation of nonlinear optical properties of graphene flakes. We find that at near infrared frequencies a graphene monolayer exhibits a remarkably high third-order optical nonlinearity which is…
Materials with massless Dirac fermions can possess exceptionally strong and widely tunable optical nonlinearities. Experiments on graphene monolayer have indeed found very large third-order nonlinear responses, but the reported variation of…
Nonlinear optics is an increasingly important field for scientific and technological applications, owing to its relevance and potential for optical and optoelectronic technologies. Currently, there is an active search for suitable nonlinear…
We develop a density matrix formalism in the length gauge to calculate the nonlinear response of intrinsic monolayer graphene at terahertz frequencies. Employing a tight-binding model, we find that the interplay of the interband and…
The second-order nonlinear optical susceptibility $\Pi^{(2)}$ for second harmonic generation is calculated for gapped graphene. The linear and second-order nonlinear plasmon excitations are investigated in context of second harmonic…
We study cascaded harmonic generation of hybrid surface plasmons in integrated planar waveguides composed of a graphene layer and a doped-semiconductor slab. We derive a comprehensive model of cascaded third harmonic generation through…
Nonlinear nanophotonics leverages engineered nanostructures to funnel light into small volumes and intensify nonlinear optical processes with spectral and spatial control. Due to its intrinsically large and electrically tunable nonlinear…
Using a combination of ultraviolet-vacuum ultraviolet reflectivity and spectroscopic ellipsometry, we observe a resonant exciton at an unusually high energy of 6.3eV in epitaxial graphene. Surprisingly, the resonant exciton occurs at room…