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We investigate harmonic generation (HG) from ground-state Ar+ aligned with M=1 at a laser wavelength of 390-nm and intensity of 4x10(14) Wcm-2. Using time-dependent R-matrix theory, we find that an initial state with magnetic quantum number…

Atomic Physics · Physics 2013-10-01 A. C. Brown , Hugo W. van der Hart

We apply the time-dependent R-matrix method to investigate harmonic generation from Ne(+) at a wavelength of 390 nm and intensities up to 10(15) Wcm(-2). The 1s(2)2s(2)2p(4) (3)P(e), (1)D(e), and (1)S(e) states of Ne(2+) are included as…

Atomic Physics · Physics 2014-05-14 O. Hassouneh , A. C. Brown , H. W. van der Hart

We investigate the influence of the autoionizing 3s3p(6)nl resonances on the fifth harmonic generated by 200 - 240 nm laser fields interacting with Ar. To determine the influence of a multi-electron response we have developed capability…

Atomic Physics · Physics 2012-04-25 A. C. Brown , S. Hutchinson , M. A. Lysaght , H. W. van der Hart

High-order harmonic generation in multiphoton ionization regime is studied theoretically to examine the resonant effects of the generating particle. We solve the time-dependent Schr\"odinger equation for In+ in the laser field by expanding…

Atomic Physics · Physics 2023-12-12 Alexander I. Magunov , Vasily V. Strelkov

We employ the R-matrix with time-dependence method to investigate extreme-ultraviolet-initiated high-harmonic generation (XIHHG) in Ar$^{+}$. Using a combination of extreme-ultraviolet (XUV, $92\textrm{ nm}$, $3\times…

Atomic Physics · Physics 2018-03-14 D. D. A. Clarke , H. W. van der Hart , A. C. Brown

We report on calculations of harmonic generation by neon in a mixed (800-nm + time-delayed 400-nm) laser pulse scheme. In contrast with previous studies we employ a short (few-cycle) 400-nm pulse, finding that this affords control of the…

Atomic Physics · Physics 2017-01-20 K. R. Hamilton , H. W. van der Hart , A. C. Brown

The below-threshold harmonic generation in the multiphoton ionization regime for a helium atom driven by the elliptically polarized laser field is studied numerically within the framework of two-dimensional (2D) and three-dimensional (3D)…

Optics · Physics 2024-12-11 Mikhail Yu. Emelin , Mikhail Yu. Ryabikin

High-order harmonic generation is investigated for H$_2^+$ and D$_2^+$ with and without Born-Oppenheimer approximation by numerical solution of full dimensional electronic time-dependent Schr\"{o}dinger equation under 4-cycle intense laser…

Atomic Physics · Physics 2014-10-22 Hamed Ahmadi , Ali Maghari , Hassan Sabzyan , Ali Reza Niknam , Mohsen Vafaee

An interesting property of high harmonic generation in solids is its laser polarization dependent nature which in turn provides information about the crystal and band structure of the generation medium. Here we report on the linear…

The high harmonic generation from atoms in the combination of chirped laser pulse and static field is theoretically investigated. For the first time, we explore a further physical mechanism of the significant extension of high harmonic…

Optics · Physics 2015-05-13 Yang Xiang , Yueping Niu , Shangqing Gong

The emission of above-ionization-threshold harmonics results from the recombination of two electron wavepackets moving along a "short" and a "long" trajectory in the atomic continuum. Attosecond pulse train generation has so far been…

Optics · Physics 2015-05-19 J. E. Kruse , P. Tzallas , E. Skantzakis , D. Charalambidis

High-order harmonic generation (HHG) from molecular ion HeH$^{2+}$ in two initial states of $1s\sigma$ (ground state) and $2p\sigma$ (first excited state) is investigated theoretically, in homogeneous and plasmonic-enhanced laser fields.…

Atomic Physics · Physics 2018-07-04 Nehzat Safaei

We present studies of high-order harmonic generation (HHG) at laser intensities well above saturation. We use driving laser pulses which present a particular electron dynamics in the turn-on stage. Our results predict an increasing on the…

Atomic Physics · Physics 2015-06-19 J. A. Pérez-Hernández , M. F. Ciappina , M. Lewenstein , A. Zaïr , L. Roso

Fully quantum treatment explicitly presents the high harmonic generation as a three-stage process: above threshold ionization (ATI) is followed by the continuum electron propagation in a laser field and subsequent stimulated recombination…

Atomic Physics · Physics 2009-10-31 M. Yu. Kuchiev , V. N. Ostrovsky

We study high-order harmonic generation in aligned molecules close to the ionization threshold. Two distinct contributions to the harmonic signal are observed, which show very different responses to molecular alignment and ellipticity of…

Atomic Physics · Physics 2011-09-16 H. Soifer , P. Botheron , D. Shafir , A. Diner , O. Raz , B. D. Bruner , Y. Mairesse , B. Pons , N. Dudovich

We establish how the intensities of the higher harmonics that arise when a photoelectron recombines with a parent ion depend functionally on the parameters of the laser wave and atomic medium, and estimate the limiting values of these…

Optics · Physics 2017-04-19 M. A. Kutlan

When molecules interact with intense light sources of femtosecond or shorter duration the rotational degrees of freedom are frozen during the response to the strong nonperturbative interaction. We show how the frozen degrees of freedom…

Atomic Physics · Physics 2007-09-25 C. B. Madsen , A. S. Mouritzen , T. K. Kjeldsen , L. B. Madsen

In present paper we develop an analytic theory for the harmonic generation of symmetric diatomic molecular ions beyond two-level model, emphasizing the influence of charge-resonance (CR) states those are strongly coupled to electromagnetic…

Atomic Physics · Physics 2009-11-13 Yanjun Chen , Jing Chen , Jie Liu

We have developed the capability to determine accurate harmonic spectra for multielectron atoms within time-dependent R-matrix (TDRM) theory. Harmonic spectra can be calculated using the expectation value of the dipole length, velocity or…

Atomic Physics · Physics 2013-01-03 A. C. Brown , D. J. Robinson , H. W. van der Hart

We present ab initio calculations using the $R$-matrix with time dependence (RMT) method for high-order harmonic generation (HHG) in argon in a short, intense pulse regime. The calculations employ a $6$-cycle $\sin^2$ pulse at $850$ nm with…

Atomic Physics · Physics 2026-04-23 Aaron T. Bondy , Klaus Bartschat
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