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Building upon past work on the phase diagram of Janus fluids [Sciortino et al., Phys. Rev. Lett. \textbf{103}, 237801 (2009)], we perform a detailed study of integral equation theory of the Kern-Frenkel potential with coverage that is tuned…

The equilibrium properties of a Janus fluid confined to a one-dimensional channel are exactly derived. The fluid is made of particles with two faces (active and passive), so that the pair interaction is that of hard spheres, except if the…

Statistical Mechanics · Physics 2020-07-01 M. A. G. Maestre , A. Santos

We study the Kern-Frenkel model for patchy colloids using Barker-Henderson second-order thermodynamic perturbation theory. The model describes a fluid where hard sphere particles are decorated with one patch, so that they interact via a…

Soft Condensed Matter · Physics 2012-03-27 Christoph Gögelein , Flavio Romano , Francesco Sciortino , Achille Giacometti

We investigate the orientational properties of a homogeneous and inhomogeneous tetrahedral 4-patch fluid (Kern--Frenkel model). Using integral equations, either (i) HNC or (ii) a modified HNC scheme with simulation input, the full…

Soft Condensed Matter · Physics 2025-01-07 Alessandro Simon , Luc Belloni , Daniel Borgis , Martin Oettel

We use molecular dynamics simulations to study the dynamics of Janus particles, micro- or nanoparticles which are not spherically symmetric, in the uniform flow of a simple liquid. In particular we consider spheres with an asymmetry in the…

Fluid Dynamics · Physics 2016-06-10 Aurelien Y. M. Archereau , Shaun C. Hendy , Geoff. R. Willmott

A class of binary mixtures of Janus fluids formed by colloidal spheres with the hydrophobic hemispheres constrained to point either up or down are studied by means of Gibbs ensemble Monte Carlo simulations and simple analytical…

Soft Condensed Matter · Physics 2013-11-14 Riccardo Fantoni , Achille Giacometti , Miguel Ángel G. Maestre , Andrés Santos

Anisotropic patchy particles have become an archetypical statistical model system for associating fluids. Here we formulate an approach to the Kern-Frenkel model via classical density functional theory to describe the positionally and…

Statistical Mechanics · Physics 2024-06-12 Alessandro Simon , Jens Weimar , Georg Martius , Martin Oettel

We investigate the structure formation of amphiphilic molecules at planar walls using density functional theory. The molecules are modeled as (hard) spheres composed of a hydrophilic and hydrophobic part. The orientation of the resulting…

Soft Condensed Matter · Physics 2015-05-20 Gerald Rosenthal , Sabine H. L. Klapp

Self-assembly of Janus (or `patchy') particles is dependent on the precise interaction between neighbouring particles. Here, the orientations of two amphiphilic Janus spheres within a dimer in an explicit fluid are studied with high…

Soft Condensed Matter · Physics 2021-08-18 Sina Safaei , Caleb Todd , Jack Yarndley , Shaun Hendy , Geoff R. Willmott

Molecular dynamics simulations are carried out to study the translational and rotational diffusion of a single Janus particle immersed in a dense Lennard-Jones fluid. We consider a spherical particle with two hemispheres of different…

Soft Condensed Matter · Physics 2015-06-18 Ali Kharazmi , Nikolai V. Priezjev

Using large scale molecular dynamics simulations we study the orientational dynamics of a heated Janus particle which exhibits self-propulsion. The asymmetry in the microscopic interaction of the colloid with the solvent is implemented by…

Soft Condensed Matter · Physics 2018-11-14 Dipanjan Chakraborty

The force and torque on a Janus sphere moving in a rarefied gas with a thermal gradient are calculated. The regime of large Knudsen number is considered, with the momenta of impinging gas molecules either obtained from a Chapman-Enskog…

Fluid Dynamics · Physics 2018-09-14 Tobias Baier , Sudarshan Tiwari , Samir Shrestha , Axel Klar , Steffen Hardt

Colloidal Janus spheres in water (one hemisphere attractive and the other repulsive) assemble into two-dimensional hexagonal crystals with orientational order controlled by anisotropic interactions. We exploit the decoupled translational…

Soft Condensed Matter · Physics 2014-06-11 Shan Jiang , Jing Yan , Jonathan K. Whitmer , Stephen M. Anthony , Erik Luijten , Steve Granick

We perform numerical simulations of a simple model of one-patch colloidal particles to investigate: (i) the behavior of the gas-liquid phase diagram on moving from a spherical attractive potential to a Janus potential and (ii) the…

Soft Condensed Matter · Physics 2017-08-23 Francesco Sciortino , Achille Giacometti , Giorgio Pastore

The statistical-mechanical study of the equilibrium properties of fluids, starting from the knowledge of the interparticle interaction potential, is essential to understand the role that microscopic interaction between individual particles…

Soft Condensed Matter · Physics 2025-10-07 Ana M. Montero

We develop a new model, to our knowledge, for the many-body hydrodynamics of amphiphilic Janus particles suspended in a viscous background flow. The Janus particles interact through a hydrophobic attraction potential that leads to…

Soft Condensed Matter · Physics 2021-10-05 Szu-Pei Fu , Bryan Quaife , Rolf Ryham , Yuan-Nan Young

We consider a simple fluid confined between two parallel walls (substrates), separated by a distance L. The walls exert competing surface fields so that one wall is attractive and may be completely wet by liquid (it is solvophilic) while…

Soft Condensed Matter · Physics 2014-09-01 Maria C. Stewart , Robert Evans

We investigate the equilibrium orientation and adsorption process of a single, ellipsoidal Janus particle at a fluid-fluid interface. The particle surface comprises equally sized parts that are hydrophobic or hydrophilic. We present free…

Soft Condensed Matter · Physics 2020-09-30 Florian Günther , Qingguang Xie , Jens Harting

We perform molecular dynamics simulations to understand the translational and rotational diffusion of Janus nanoparticles at the interface between two immiscible fluids. Considering spherical particles with different affinity to fluid…

Fluid Dynamics · Physics 2016-05-04 Hossein Rezvantalab , German Drazer , Shahab Shojaei-Zadeh

The diffusion of a Janus rod-shaped nanoparticle in a dense Lennard-Jones fluid is studied using molecular dynamics (MD) simulations. The Janus particle is modeled as a rigid cylinder whose atoms on each half-side have different interaction…

Soft Condensed Matter · Physics 2017-07-31 Ali Kharazmi , Nikolai V. Priezjev
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